LrgpV1, Hal, Checkpoint, bibRecord, 000B82

High carbon dioxide solubilities in imidazolium based ionic liquids and in poly(ethylene glycol) dimethyl ether

Identifieur interne : 000B82 ( Hal/Checkpoint ); précédent : 000B81; suivant : 000B83

High carbon dioxide solubilities in imidazolium based ionic liquids and in poly(ethylene glycol) dimethyl ether

Auteurs : A. L. Revelli [France] ; F. Mutelet [France] ; J. N. Jaubert [France]

Source :

Journal of Physical Chemistry B [ 1520-6106 ] ; 2010.

RBID : Hal:hal-00611077

Abstract

This work is focused on the possible capture of carbon dioxide using ionic liquids (ILs). Such solvents are gaining special attention because the efficiency of many processes can be enhanced by the judicious manipulation of their properties. The absorption of greenhouse gases can be enhanced by the basic character of the IL. In this work, these characteristics are evaluated through the study of the gas-liquid equilibrium of four imidazolium-based ILs: 1-butyl-3-methylimidazolium tetrafluoroborate BMIMBF(4), 1-butyl-3-methylimidazolium thiocyanate BMIMSCN, 1,3-dimethylimidazolium methylphosphonate DMIMMP, and 1,3-diethoxyimidazolium (ETO)(2)IMTf(2)N with CO(2) at temperatures up to 373 K and pressures up to 300 bar. Solubility of carbon dioxide in poly(ethylene glycol) dimethyl ether, component of selexol, was also measured to evaluate the capture's efficiency of ionic liquids. Experimental data indicate that 67 to 123 g of CO(2) can be absorbed per kg of ionic liquid and 198 g per kg of poly(ethylene glycol) dimethyl ether.

Url:

https://hal.archives-ouvertes.fr/hal-00611077

DOI: 10.1021/jp1057989

Links toward previous steps (curation, corpus...)

to stream Hal, to step Corpus: 000563
to stream Hal, to step Curation: 000563

Links to Exploration step

Hal:hal-00611077

Le document en format XML

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<abstract xml:lang="en">This work is focused on the possible capture of carbon dioxide using ionic liquids (ILs). Such solvents are gaining special attention because the efficiency of many processes can be enhanced by the judicious manipulation of their properties. The absorption of greenhouse gases can be enhanced by the basic character of the IL. In this work, these characteristics are evaluated through the study of the gas-liquid equilibrium of four imidazolium-based ILs: 1-butyl-3-methylimidazolium tetrafluoroborate BMIMBF(4), 1-butyl-3-methylimidazolium thiocyanate BMIMSCN, 1,3-dimethylimidazolium methylphosphonate DMIMMP, and 1,3-diethoxyimidazolium (ETO)(2)IMTf(2)N with CO(2) at temperatures up to 373 K and pressures up to 300 bar. Solubility of carbon dioxide in poly(ethylene glycol) dimethyl ether, component of selexol, was also measured to evaluate the capture's efficiency of ionic liquids. Experimental data indicate that 67 to 123 g of CO(2) can be absorbed per kg of ionic liquid and 198 g per kg of poly(ethylene glycol) dimethyl ether.</abstract>
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High carbon dioxide solubilities in imidazolium based ionic liquids and in poly(ethylene glycol) dimethyl ether

High carbon dioxide solubilities in imidazolium based ionic liquids and in poly(ethylene glycol) dimethyl ether

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