Syntheses, structure and properties of three-dimensional pillared-layer Ag(I)-Ln(III) heterometallic coordination polymers based on mixed isonicotinate and hemimellitate ligands
Identifieur interne : 000395 ( Chine/Analysis ); précédent : 000394; suivant : 000396Syntheses, structure and properties of three-dimensional pillared-layer Ag(I)-Ln(III) heterometallic coordination polymers based on mixed isonicotinate and hemimellitate ligands
Auteurs : RBID : Pascal:12-0448070Descripteurs français
- Pascal (Inist)
- Structure à pilier, Polymère coordination, Structure cristalline, Structure moléculaire, Ligand, Arséniure d'indium, Semiconducteur III-V, Composé III-V, Dérivé de l'acide isonicotinique, Croissance cristalline en solution, Diffraction RX, Structure lamellaire, Lanthanide, Liaison coordination, Argent, Monocristal, Photoluminescence, Substrat polymère, InAs, 6166H, 7855Q, 8105L, 8110D.
- Wicri :
- concept : Argent.
English descriptors
- KwdEn :
Abstract
Three pillared-layer 4d-4f Ag(I)-Ln(III) heterometallic coordination polymers (HCPs), formulated as [Ln2Ag(hma)2(ina)(H2O)2]n nH20 [Ln=La(1), Pr(2), Nd(3); Hina=isonicotinic acid, H3hma=hemimellitic acid], have been synthesized under hydrothermal conditions. Single-crystal and powder X-ray diffractions confirm that they are isostructural, which features a three-dimensional (3D) pillared-layer heterometallic structure built upon the strictly alternate arrangement of lanthanide-organic layers and [Ag(ina)] pillars. The layers and pillars are connected to each other by Ln-0 and Ag-O coordination bonds. The photoluminescent property of the Nd derivative (3) has also been investigated.
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Pascal:12-0448070Le document en format XML
<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Syntheses, structure and properties of three-dimensional pillared-layer Ag(I)-Ln(III) heterometallic coordination polymers based on mixed isonicotinate and hemimellitate ligands</title>
<author><name>XINFA LI</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Chemistry, Zunyi Normal College</s1>
<s2>Zunyi 563002</s2>
<s3>CHN</s3>
<sZ>1 aut.</sZ>
</inist:fA14>
<country>République populaire de Chine</country>
<wicri:noRegion>Zunyi 563002</wicri:noRegion>
</affiliation>
</author>
<author><name>RONG CAO</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences</s1>
<s2>Fuzhou 350002</s2>
<s3>CHN</s3>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>République populaire de Chine</country>
<wicri:noRegion>Fuzhou 350002</wicri:noRegion>
</affiliation>
</author>
</titleStmt>
<publicationStmt><idno type="inist">12-0448070</idno>
<date when="2012">2012</date>
<idno type="stanalyst">PASCAL 12-0448070 INIST</idno>
<idno type="RBID">Pascal:12-0448070</idno>
<idno type="wicri:Area/Main/Corpus">001557</idno>
<idno type="wicri:Area/Main/Repository">001451</idno>
<idno type="wicri:Area/Chine/Extraction">000395</idno>
</publicationStmt>
<seriesStmt><idno type="ISSN">0022-4596</idno>
<title level="j" type="abbreviated">J. solid state chem. : (Print)</title>
<title level="j" type="main">Journal of solid state chemistry : (Print)</title>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Coordination bond</term>
<term>Crystal growth from solutions</term>
<term>Crystal structure</term>
<term>III-V compound</term>
<term>III-V semiconductors</term>
<term>Indium arsenides</term>
<term>Isonicotinic acid derivatives</term>
<term>Lamellar structure</term>
<term>Ligands</term>
<term>Molecular structure</term>
<term>Monocrystals</term>
<term>Photoluminescence</term>
<term>Pillared structure</term>
<term>Polychelate</term>
<term>Rare earths</term>
<term>Silver</term>
<term>XRD</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Structure à pilier</term>
<term>Polymère coordination</term>
<term>Structure cristalline</term>
<term>Structure moléculaire</term>
<term>Ligand</term>
<term>Arséniure d'indium</term>
<term>Semiconducteur III-V</term>
<term>Composé III-V</term>
<term>Dérivé de l'acide isonicotinique</term>
<term>Croissance cristalline en solution</term>
<term>Diffraction RX</term>
<term>Structure lamellaire</term>
<term>Lanthanide</term>
<term>Liaison coordination</term>
<term>Argent</term>
<term>Monocristal</term>
<term>Photoluminescence</term>
<term>Substrat polymère</term>
<term>InAs</term>
<term>6166H</term>
<term>7855Q</term>
<term>8105L</term>
<term>8110D</term>
</keywords>
<keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Argent</term>
</keywords>
</textClass>
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<front><div type="abstract" xml:lang="en">Three pillared-layer 4d-4f Ag(I)-Ln(III) heterometallic coordination polymers (HCPs), formulated as [Ln<sub>2</sub>
Ag(hma)<sub>2</sub>
(ina)(H<sub>2</sub>
O)<sub>2</sub>
]<sub>n</sub>
nH<sub>2</sub>
0 [Ln=La(1), Pr(2), Nd(3); Hina=isonicotinic acid, H<sub>3</sub>
hma=hemimellitic acid], have been synthesized under hydrothermal conditions. Single-crystal and powder X-ray diffractions confirm that they are isostructural, which features a three-dimensional (3D) pillared-layer heterometallic structure built upon the strictly alternate arrangement of lanthanide-organic layers and [Ag(ina)] pillars. The layers and pillars are connected to each other by Ln-0 and Ag-O coordination bonds. The photoluminescent property of the Nd derivative (3) has also been investigated.</div>
</front>
</TEI>
<inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0022-4596</s0>
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<fA03 i2="1"><s0>J. solid state chem. : (Print)</s0>
</fA03>
<fA05><s2>196</s2>
</fA05>
<fA08 i1="01" i2="1" l="ENG"><s1>Syntheses, structure and properties of three-dimensional pillared-layer Ag(I)-Ln(III) heterometallic coordination polymers based on mixed isonicotinate and hemimellitate ligands</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>XINFA LI</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>RONG CAO</s1>
</fA11>
<fA14 i1="01"><s1>Department of Chemistry, Zunyi Normal College</s1>
<s2>Zunyi 563002</s2>
<s3>CHN</s3>
<sZ>1 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences</s1>
<s2>Fuzhou 350002</s2>
<s3>CHN</s3>
<sZ>2 aut.</sZ>
</fA14>
<fA20><s1>182-186</s1>
</fA20>
<fA21><s1>2012</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>14677</s2>
<s5>354000506857270270</s5>
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<fA44><s0>0000</s0>
<s1>© 2012 INIST-CNRS. All rights reserved.</s1>
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<fA60><s1>P</s1>
</fA60>
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<fA64 i1="01" i2="1"><s0>Journal of solid state chemistry : (Print)</s0>
</fA64>
<fA66 i1="01"><s0>NLD</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Three pillared-layer 4d-4f Ag(I)-Ln(III) heterometallic coordination polymers (HCPs), formulated as [Ln<sub>2</sub>
Ag(hma)<sub>2</sub>
(ina)(H<sub>2</sub>
O)<sub>2</sub>
]<sub>n</sub>
nH<sub>2</sub>
0 [Ln=La(1), Pr(2), Nd(3); Hina=isonicotinic acid, H<sub>3</sub>
hma=hemimellitic acid], have been synthesized under hydrothermal conditions. Single-crystal and powder X-ray diffractions confirm that they are isostructural, which features a three-dimensional (3D) pillared-layer heterometallic structure built upon the strictly alternate arrangement of lanthanide-organic layers and [Ag(ina)] pillars. The layers and pillars are connected to each other by Ln-0 and Ag-O coordination bonds. The photoluminescent property of the Nd derivative (3) has also been investigated.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B60A66H</s0>
</fC02>
<fC02 i1="02" i2="3"><s0>001B80A10D</s0>
</fC02>
<fC02 i1="03" i2="3"><s0>001B70H55Q</s0>
</fC02>
<fC02 i1="04" i2="3"><s0>001B80A05Z</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Structure à pilier</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Pillared structure</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Estructura con pilares</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE"><s0>Polymère coordination</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG"><s0>Polychelate</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA"><s0>Polímero coordinación</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="3" l="FRE"><s0>Structure cristalline</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="3" l="ENG"><s0>Crystal structure</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Structure moléculaire</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Molecular structure</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="3" l="FRE"><s0>Ligand</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Ligands</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="3" l="FRE"><s0>Arséniure d'indium</s0>
<s2>NK</s2>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="3" l="ENG"><s0>Indium arsenides</s0>
<s2>NK</s2>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="3" l="FRE"><s0>Semiconducteur III-V</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="3" l="ENG"><s0>III-V semiconductors</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Composé III-V</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>III-V compound</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Compuesto III-V</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Dérivé de l'acide isonicotinique</s0>
<s2>FR</s2>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Isonicotinic acid derivatives</s0>
<s2>FR</s2>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Croissance cristalline en solution</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Crystal growth from solutions</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="3" l="FRE"><s0>Diffraction RX</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="3" l="ENG"><s0>XRD</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Structure lamellaire</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Lamellar structure</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Estructura lamelar</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="3" l="FRE"><s0>Lanthanide</s0>
<s2>NC</s2>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="3" l="ENG"><s0>Rare earths</s0>
<s2>NC</s2>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Liaison coordination</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Coordination bond</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Enlace coordinación</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Argent</s0>
<s2>NC</s2>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Silver</s0>
<s2>NC</s2>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="3" l="FRE"><s0>Monocristal</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="3" l="ENG"><s0>Monocrystals</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="3" l="FRE"><s0>Photoluminescence</s0>
<s5>29</s5>
</fC03>
<fC03 i1="17" i2="3" l="ENG"><s0>Photoluminescence</s0>
<s5>29</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Substrat polymère</s0>
<s4>INC</s4>
<s5>46</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>InAs</s0>
<s4>INC</s4>
<s5>47</s5>
</fC03>
<fC03 i1="20" i2="3" l="FRE"><s0>6166H</s0>
<s4>INC</s4>
<s5>65</s5>
</fC03>
<fC03 i1="21" i2="3" l="FRE"><s0>7855Q</s0>
<s4>INC</s4>
<s5>66</s5>
</fC03>
<fC03 i1="22" i2="3" l="FRE"><s0>8105L</s0>
<s4>INC</s4>
<s5>67</s5>
</fC03>
<fC03 i1="23" i2="3" l="FRE"><s0>8110D</s0>
<s4>INC</s4>
<s5>72</s5>
</fC03>
<fN21><s1>345</s1>
</fN21>
</pA>
</standard>
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