Methane conversion to higher alkanes over ruthenium and cobalt loaded Zr3(PO4)4
Identifieur interne :
000115 ( PascalFrancis/Curation );
précédent :
000114;
suivant :
000116
Methane conversion to higher alkanes over ruthenium and cobalt loaded Zr3(PO4)4
Auteurs : N. Cheikhi [
Maroc] ;
M. Zivad [
Maroc]
Source :
-
Journal de physique. IV [ 1155-4339 ] ; 2005.
RBID : Pascal:05-0363864
Descripteurs français
- Pascal (Inist)
- Catalyseur sur support,
Métal transition,
Platinoïde,
Zirconium Phosphate,
Ruthénium,
Cobalt,
Oligomérisation,
Méthane,
Catalyse hétérogène,
Hydrocarbure,
Alcane.
- Wicri :
English descriptors
- KwdEn :
- Alkane,
Cobalt,
Heterogeneous catalysis,
Hydrocarbon,
Methane,
Oligomerization,
Platinoid,
Ruthenium,
Supported catalyst,
Transition metal,
Zirconium Phosphates.
Abstract
The catalyst Ru-Co/Zr3(PO4)4 was synthesized by impregnation and was tested in the reaction of oligomerization of methane into higher hydrocarbon. The reaction was carried out using a two-steps procedure consisting of: - Methane adsorption. - Hydrogenation of the adsorbed entities and formation of higher hydrocarbons. The production of these alkanes extends from ethane to pentane and could schematically be described by the following pathways: CH4 ⇄ (CHx)ads + (4-X)/2H2 CHx, CHy ⇄ CnHm The results showed that addition of cobalt to ruthenium improved the global activity. This promoter effect was attributed to the synergy brought in by cobalt and to the formation of Ru-CO2+species which are more active than ruthenium alone. These species were identified by EDX-STEM and XPS analyses.
| pA |
| A01 | 01 | 1 | | @0 1155-4339 |
|---|
| A03 | | 1 | | @0 J. phys., IV |
|---|
| A05 | | | | @2 123 |
|---|
| A08 | 01 | 1 | ENG | @1 Methane conversion to higher alkanes over ruthenium and cobalt loaded Zr3(PO4)4 |
|---|
| A09 | 01 | 1 | ENG | @1 REMCES IX: Proceedings of the 9th International Seminar on the Physical Chemistry of Solid State Materials |
|---|
| A11 | 01 | 1 | | @1 CHEIKHI (N.) |
|---|
| A11 | 02 | 1 | | @1 ZIVAD (M.) |
|---|
| A12 | 01 | 1 | | @1 BENLHACHEMI (Abdeljalil) @9 ed. |
|---|
| A12 | 02 | 1 | | @1 BENYAICH (H.) @9 ed. |
|---|
| A12 | 03 | 1 | | @1 BOUABID (Khalid) @9 ed. |
|---|
| A12 | 04 | 1 | | @1 BOUKHARI (A.) @9 ed. |
|---|
| A12 | 05 | 1 | | @1 ELAATMANI (M.) @9 ed. |
|---|
| A12 | 06 | 1 | | @1 ES-SAKHI (B.) @9 ed. |
|---|
| A12 | 07 | 1 | | @1 IHLAL (A.) @9 ed. |
|---|
| A12 | 08 | 1 | | @1 KHAIROUNE (S.) @9 ed. |
|---|
| A12 | 09 | 1 | | @1 MANSOURI (I.) @9 ed. |
|---|
| A12 | 10 | 1 | | @1 NOUNAH (Abderrahman) @9 ed. |
|---|
| A12 | 11 | 1 | | @1 TAHA (Mohamed) @9 ed. |
|---|
| A12 | 12 | 1 | | @1 ZAHIDI (E.) @9 ed. |
|---|
| A14 | 01 | | | @1 Faculté des Sciences, Laboratoire de Physico-Chimie des Matériaux et Catalyse, Département de Chimie, BP. 1014 @2 Rabat @3 MAR @Z 1 aut. @Z 2 aut. |
|---|
| A15 | 01 | | | @1 Faculté des Sciences, Cité Dakhla @2 Agadir @3 MAR @Z 1 aut. @Z 3 aut. @Z 11 aut. |
|---|
| A15 | 02 | | | @1 Ecole Supérieure de Technologie @2 Salé Médina @3 MAR @Z 10 aut. |
|---|
| A18 | 01 | 1 | | @1 IBN ZOHR University. Faculty of Sciences @2 Agadir @3 MAR @9 patr. |
|---|
| A20 | | | | @1 301-305 |
|---|
| A21 | | | | @1 2005 |
|---|
| A23 | 01 | | | @0 ENG |
|---|
| A43 | 01 | | | @1 INIST @2 125C @5 354000126872900540 |
|---|
| A44 | | | | @0 0000 @1 © 2005 INIST-CNRS. All rights reserved. |
|---|
| A45 | | | | @0 16 ref. |
|---|
| A47 | 01 | 1 | | @0 05-0363864 |
|---|
| A60 | | | | @1 P @2 C |
|---|
| A61 | | | | @0 A |
|---|
| A64 | 01 | 1 | | @0 Journal de physique. IV |
|---|
| A66 | 01 | | | @0 FRA |
|---|
| C01 | 01 | | ENG | @0 The catalyst Ru-Co/Zr3(PO4)4 was synthesized by impregnation and was tested in the reaction of oligomerization of methane into higher hydrocarbon. The reaction was carried out using a two-steps procedure consisting of: - Methane adsorption. - Hydrogenation of the adsorbed entities and formation of higher hydrocarbons. The production of these alkanes extends from ethane to pentane and could schematically be described by the following pathways: CH4 ⇄ (CHx)ads + (4-X)/2H2 CHx, CHy ⇄ CnHm The results showed that addition of cobalt to ruthenium improved the global activity. This promoter effect was attributed to the synergy brought in by cobalt and to the formation of Ru-CO2+species which are more active than ruthenium alone. These species were identified by EDX-STEM and XPS analyses. |
|---|
| C02 | 01 | X | | @0 001C01A03 |
|---|
| C03 | 01 | X | FRE | @0 Catalyseur sur support @5 01 |
|---|
| C03 | 01 | X | ENG | @0 Supported catalyst @5 01 |
|---|
| C03 | 01 | X | SPA | @0 Catalizador sobre soporte @5 01 |
|---|
| C03 | 02 | X | FRE | @0 Métal transition @2 NC @5 02 |
|---|
| C03 | 02 | X | ENG | @0 Transition metal @2 NC @5 02 |
|---|
| C03 | 02 | X | SPA | @0 Metal transición @2 NC @5 02 |
|---|
| C03 | 03 | X | FRE | @0 Platinoïde @2 NC @5 03 |
|---|
| C03 | 03 | X | ENG | @0 Platinoid @2 NC @5 03 |
|---|
| C03 | 03 | X | SPA | @0 Platinoide @2 NC @5 03 |
|---|
| C03 | 04 | X | FRE | @0 Zirconium Phosphate @2 NC @2 NA @5 04 |
|---|
| C03 | 04 | X | ENG | @0 Zirconium Phosphates @2 NC @2 NA @5 04 |
|---|
| C03 | 04 | X | SPA | @0 Zirconio Fosfato @2 NC @2 NA @5 04 |
|---|
| C03 | 05 | X | FRE | @0 Ruthénium @2 NC @5 05 |
|---|
| C03 | 05 | X | ENG | @0 Ruthenium @2 NC @5 05 |
|---|
| C03 | 05 | X | SPA | @0 Rutenio @2 NC @5 05 |
|---|
| C03 | 06 | X | FRE | @0 Cobalt @2 NC @5 06 |
|---|
| C03 | 06 | X | ENG | @0 Cobalt @2 NC @5 06 |
|---|
| C03 | 06 | X | SPA | @0 Cobalto @2 NC @5 06 |
|---|
| C03 | 07 | X | FRE | @0 Oligomérisation @5 07 |
|---|
| C03 | 07 | X | ENG | @0 Oligomerization @5 07 |
|---|
| C03 | 07 | X | SPA | @0 Oligomerización @5 07 |
|---|
| C03 | 08 | X | FRE | @0 Méthane @2 NK @2 FX @5 08 |
|---|
| C03 | 08 | X | ENG | @0 Methane @2 NK @2 FX @5 08 |
|---|
| C03 | 08 | X | SPA | @0 Metano @2 NK @2 FX @5 08 |
|---|
| C03 | 09 | X | FRE | @0 Catalyse hétérogène @5 09 |
|---|
| C03 | 09 | X | ENG | @0 Heterogeneous catalysis @5 09 |
|---|
| C03 | 09 | X | SPA | @0 Catálisis heterogénea @5 09 |
|---|
| C03 | 10 | X | FRE | @0 Hydrocarbure @2 FX @5 10 |
|---|
| C03 | 10 | X | ENG | @0 Hydrocarbon @2 FX @5 10 |
|---|
| C03 | 10 | X | SPA | @0 Hidrocarburo @2 FX @5 10 |
|---|
| C03 | 11 | X | FRE | @0 Alcane @5 11 |
|---|
| C03 | 11 | X | ENG | @0 Alkane @5 11 |
|---|
| C03 | 11 | X | SPA | @0 Alcano @5 11 |
|---|
| N21 | | | | @1 255 |
|---|
|
|---|
| pR |
| A30 | 01 | 1 | ENG | @1 REMCES International Seminar on the Physical Chemistry of Solid State Materials @2 9 @3 Agadir MAR @4 2002-10-30 |
|---|
|
|---|
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Le document en format XML
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(PO<sub>4</sub>
)<sub>4</sub>
</title><author><name sortKey="Cheikhi, N" sort="Cheikhi, N" uniqKey="Cheikhi N" first="N." last="Cheikhi">N. Cheikhi</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculté des Sciences, Laboratoire de Physico-Chimie des Matériaux et Catalyse, Département de Chimie, BP. 1014</s1>
<s2>Rabat</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14><country>Maroc</country>
</affiliation><author><name sortKey="Zivad, M" sort="Zivad, M" uniqKey="Zivad M" first="M." last="Zivad">M. Zivad</name>
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<s2>Rabat</s2>
<s3>MAR</s3>
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<sZ>2 aut.</sZ>
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</publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Methane conversion to higher alkanes over ruthenium and cobalt loaded Zr<sub>3</sub>
(PO<sub>4</sub>
)<sub>4</sub>
</title><author><name sortKey="Cheikhi, N" sort="Cheikhi, N" uniqKey="Cheikhi N" first="N." last="Cheikhi">N. Cheikhi</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculté des Sciences, Laboratoire de Physico-Chimie des Matériaux et Catalyse, Département de Chimie, BP. 1014</s1>
<s2>Rabat</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14><country>Maroc</country>
</affiliation><author><name sortKey="Zivad, M" sort="Zivad, M" uniqKey="Zivad M" first="M." last="Zivad">M. Zivad</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Faculté des Sciences, Laboratoire de Physico-Chimie des Matériaux et Catalyse, Département de Chimie, BP. 1014</s1>
<s2>Rabat</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14><country>Maroc</country>
</affiliation><series><title level="j" type="main">Journal de physique. IV</title>
<title level="j" type="abbreviated">J. phys., IV</title>
<idno type="ISSN">1155-4339</idno>
<imprint><date when="2005">2005</date>
</imprint><seriesStmt><title level="j" type="main">Journal de physique. IV</title>
<title level="j" type="abbreviated">J. phys., IV</title>
<idno type="ISSN">1155-4339</idno>
</seriesStmt><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Alkane</term>
<term>Cobalt</term>
<term>Heterogeneous catalysis</term>
<term>Hydrocarbon</term>
<term>Methane</term>
<term>Oligomerization</term>
<term>Platinoid</term>
<term>Ruthenium</term>
<term>Supported catalyst</term>
<term>Transition metal</term>
<term>Zirconium Phosphates</term>
</keywords><keywords scheme="Pascal" xml:lang="fr"><term>Catalyseur sur support</term>
<term>Métal transition</term>
<term>Platinoïde</term>
<term>Zirconium Phosphate</term>
<term>Ruthénium</term>
<term>Cobalt</term>
<term>Oligomérisation</term>
<term>Méthane</term>
<term>Catalyse hétérogène</term>
<term>Hydrocarbure</term>
<term>Alcane</term>
</keywords><keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Cobalt</term>
<term>Hydrocarbure</term>
</keywords><front><div type="abstract" xml:lang="en">The catalyst Ru-Co/Zr<sub>3</sub>
(PO<sub>4</sub>
)<sub>4</sub>
was synthesized by impregnation and was tested in the reaction of oligomerization of methane into higher hydrocarbon. The reaction was carried out using a two-steps procedure consisting of: - Methane adsorption. - Hydrogenation of the adsorbed entities and formation of higher hydrocarbons. The production of these alkanes extends from ethane to pentane and could schematically be described by the following pathways: CH<sub>4</sub>
⇄ (CH<sub>x</sub>
)<sub>ads</sub>
+ (4-X)/2H<sub>2</sub>
CH<sub>x</sub>
, CH<sub>y</sub>
⇄ C<sub>n</sub>
H<sub>m</sub>
The results showed that addition of cobalt to ruthenium improved the global activity. This promoter effect was attributed to the synergy brought in by cobalt and to the formation of Ru-CO<sup>2+</sup>
species which are more active than ruthenium alone. These species were identified by EDX-STEM and XPS analyses.</div><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>1155-4339</s0>
</fA01><fA03 i2="1"><s0>J. phys., IV</s0>
</fA03><fA05><s2>123</s2>
</fA05><fA08 i1="01" i2="1" l="ENG"><s1>Methane conversion to higher alkanes over ruthenium and cobalt loaded Zr<sub>3</sub>
(PO<sub>4</sub>
)<sub>4</sub>
</s1><fA09 i1="01" i2="1" l="ENG"><s1>REMCES IX: Proceedings of the 9th International Seminar on the Physical Chemistry of Solid State Materials</s1>
</fA09><fA11 i1="01" i2="1"><s1>CHEIKHI (N.)</s1>
</fA11><fA11 i1="02" i2="1"><s1>ZIVAD (M.)</s1>
</fA11><fA12 i1="01" i2="1"><s1>BENLHACHEMI (Abdeljalil)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="02" i2="1"><s1>BENYAICH (H.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="03" i2="1"><s1>BOUABID (Khalid)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="04" i2="1"><s1>BOUKHARI (A.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="05" i2="1"><s1>ELAATMANI (M.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="06" i2="1"><s1>ES-SAKHI (B.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="07" i2="1"><s1>IHLAL (A.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="08" i2="1"><s1>KHAIROUNE (S.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="09" i2="1"><s1>MANSOURI (I.)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="10" i2="1"><s1>NOUNAH (Abderrahman)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="11" i2="1"><s1>TAHA (Mohamed)</s1>
<s9>ed.</s9>
</fA12><fA12 i1="12" i2="1"><s1>ZAHIDI (E.)</s1>
<s9>ed.</s9>
</fA12><fA14 i1="01"><s1>Faculté des Sciences, Laboratoire de Physico-Chimie des Matériaux et Catalyse, Département de Chimie, BP. 1014</s1>
<s2>Rabat</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</fA14><fA15 i1="01"><s1>Faculté des Sciences, Cité Dakhla</s1>
<s2>Agadir</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>11 aut.</sZ>
</fA15><fA15 i1="02"><s1>Ecole Supérieure de Technologie</s1>
<s2>Salé Médina</s2>
<s3>MAR</s3>
<sZ>10 aut.</sZ>
</fA15><fA18 i1="01" i2="1"><s1>IBN ZOHR University. Faculty of Sciences</s1>
<s2>Agadir</s2>
<s3>MAR</s3>
<s9>patr.</s9>
</fA18><fA20><s1>301-305</s1>
</fA20><fA21><s1>2005</s1>
</fA21><fA23 i1="01"><s0>ENG</s0>
</fA23><fA43 i1="01"><s1>INIST</s1>
<s2>125C</s2>
<s5>354000126872900540</s5>
</fA43><fA44><s0>0000</s0>
<s1>© 2005 INIST-CNRS. All rights reserved.</s1>
</fA44><fA45><s0>16 ref.</s0>
</fA45><fA47 i1="01" i2="1"><s0>05-0363864</s0>
</fA47><fA60><s1>P</s1>
<s2>C</s2>
</fA60><fA64 i1="01" i2="1"><s0>Journal de physique. IV</s0>
</fA64><fA66 i1="01"><s0>FRA</s0>
</fA66><fC01 i1="01" l="ENG"><s0>The catalyst Ru-Co/Zr<sub>3</sub>
(PO<sub>4</sub>
)<sub>4</sub>
was synthesized by impregnation and was tested in the reaction of oligomerization of methane into higher hydrocarbon. The reaction was carried out using a two-steps procedure consisting of: - Methane adsorption. - Hydrogenation of the adsorbed entities and formation of higher hydrocarbons. The production of these alkanes extends from ethane to pentane and could schematically be described by the following pathways: CH<sub>4</sub>
⇄ (CH<sub>x</sub>
)<sub>ads</sub>
+ (4-X)/2H<sub>2</sub>
CH<sub>x</sub>
, CH<sub>y</sub>
⇄ C<sub>n</sub>
H<sub>m</sub>
The results showed that addition of cobalt to ruthenium improved the global activity. This promoter effect was attributed to the synergy brought in by cobalt and to the formation of Ru-CO<sup>2+</sup>
species which are more active than ruthenium alone. These species were identified by EDX-STEM and XPS analyses.</s0><fC02 i1="01" i2="X"><s0>001C01A03</s0>
</fC02><fC03 i1="01" i2="X" l="FRE"><s0>Catalyseur sur support</s0>
<s5>01</s5>
</fC03><fC03 i1="01" i2="X" l="ENG"><s0>Supported catalyst</s0>
<s5>01</s5>
</fC03><fC03 i1="01" i2="X" l="SPA"><s0>Catalizador sobre soporte</s0>
<s5>01</s5>
</fC03><fC03 i1="02" i2="X" l="FRE"><s0>Métal transition</s0>
<s2>NC</s2>
<s5>02</s5>
</fC03><fC03 i1="02" i2="X" l="ENG"><s0>Transition metal</s0>
<s2>NC</s2>
<s5>02</s5>
</fC03><fC03 i1="02" i2="X" l="SPA"><s0>Metal transición</s0>
<s2>NC</s2>
<s5>02</s5>
</fC03><fC03 i1="03" i2="X" l="FRE"><s0>Platinoïde</s0>
<s2>NC</s2>
<s5>03</s5>
</fC03><fC03 i1="03" i2="X" l="ENG"><s0>Platinoid</s0>
<s2>NC</s2>
<s5>03</s5>
</fC03><fC03 i1="03" i2="X" l="SPA"><s0>Platinoide</s0>
<s2>NC</s2>
<s5>03</s5>
</fC03><fC03 i1="04" i2="X" l="FRE"><s0>Zirconium Phosphate</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>04</s5>
</fC03><fC03 i1="04" i2="X" l="ENG"><s0>Zirconium Phosphates</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>04</s5>
</fC03><fC03 i1="04" i2="X" l="SPA"><s0>Zirconio Fosfato</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>04</s5>
</fC03><fC03 i1="05" i2="X" l="FRE"><s0>Ruthénium</s0>
<s2>NC</s2>
<s5>05</s5>
</fC03><fC03 i1="05" i2="X" l="ENG"><s0>Ruthenium</s0>
<s2>NC</s2>
<s5>05</s5>
</fC03><fC03 i1="05" i2="X" l="SPA"><s0>Rutenio</s0>
<s2>NC</s2>
<s5>05</s5>
</fC03><fC03 i1="06" i2="X" l="FRE"><s0>Cobalt</s0>
<s2>NC</s2>
<s5>06</s5>
</fC03><fC03 i1="06" i2="X" l="ENG"><s0>Cobalt</s0>
<s2>NC</s2>
<s5>06</s5>
</fC03><fC03 i1="06" i2="X" l="SPA"><s0>Cobalto</s0>
<s2>NC</s2>
<s5>06</s5>
</fC03><fC03 i1="07" i2="X" l="FRE"><s0>Oligomérisation</s0>
<s5>07</s5>
</fC03><fC03 i1="07" i2="X" l="ENG"><s0>Oligomerization</s0>
<s5>07</s5>
</fC03><fC03 i1="07" i2="X" l="SPA"><s0>Oligomerización</s0>
<s5>07</s5>
</fC03><fC03 i1="08" i2="X" l="FRE"><s0>Méthane</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>08</s5>
</fC03><fC03 i1="08" i2="X" l="ENG"><s0>Methane</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>08</s5>
</fC03><fC03 i1="08" i2="X" l="SPA"><s0>Metano</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>08</s5>
</fC03><fC03 i1="09" i2="X" l="FRE"><s0>Catalyse hétérogène</s0>
<s5>09</s5>
</fC03><fC03 i1="09" i2="X" l="ENG"><s0>Heterogeneous catalysis</s0>
<s5>09</s5>
</fC03><fC03 i1="09" i2="X" l="SPA"><s0>Catálisis heterogénea</s0>
<s5>09</s5>
</fC03><fC03 i1="10" i2="X" l="FRE"><s0>Hydrocarbure</s0>
<s2>FX</s2>
<s5>10</s5>
</fC03><fC03 i1="10" i2="X" l="ENG"><s0>Hydrocarbon</s0>
<s2>FX</s2>
<s5>10</s5>
</fC03><fC03 i1="10" i2="X" l="SPA"><s0>Hidrocarburo</s0>
<s2>FX</s2>
<s5>10</s5>
</fC03><fC03 i1="11" i2="X" l="FRE"><s0>Alcane</s0>
<s5>11</s5>
</fC03><fC03 i1="11" i2="X" l="ENG"><s0>Alkane</s0>
<s5>11</s5>
</fC03><fC03 i1="11" i2="X" l="SPA"><s0>Alcano</s0>
<s5>11</s5>
</fC03><fN21><s1>255</s1>
</fN21><pR><fA30 i1="01" i2="1" l="ENG"><s1>REMCES International Seminar on the Physical Chemistry of Solid State Materials</s1>
<s2>9</s2>
<s3>Agadir MAR</s3>
<s4>2002-10-30</s4>
</fA30>
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