CobaltMaghrebV1, PascalFrancis, Checkpoint, bibRecord, 000341

On the NaxNi0.6Co0.4O2 system : Physical and electrochemical studies

Identifieur interne : 000341 ( PascalFrancis/Checkpoint ); précédent : 000340; suivant : 000342

On the NaxNi0.6Co0.4O2 system : Physical and electrochemical studies

Auteurs : I. Saadoune [Maroc] ; A. Maazaz [Maroc] ; M. Menetrier [France] ; C. Delmas [France]

Source :

Journal of solid state chemistry [ 0022-4596 ] ; 1996.

RBID : Pascal:96-0185253

Descripteurs français

Pascal (Inist)
- Sodium Oxyde, Nickel Oxyde, Cobalt Oxyde, Composé quaternaire, Réaction électrochimique, Composé insertion, Désinsertion, Iode, Matériau électrode, Accumulateur électrochimique, Coefficient diffusion, Cinétique, Solution électrolyte, Solution non aqueuse, XRD, Paramètre cristallin, Propriété magnétique, NaxNi0,6Co0,4O2, Co Na Ni O.
Wicri :
- topic : Iode.

English descriptors

KwdEn :
- Cobalt Oxides, Desinsertion, Diffusion coefficient, Electrochemical reaction, Electrode material, Electrolyte solution, Intercalation compound, Iodine, Kinetics, Lattice parameters, Magnetic properties, Nickel Oxides, Non aqueous solution, Quaternary compound, Secondary cell, Sodium Oxides, XRD.

Abstract

Sodium chemical deintercalation from the NaNi_0.6Co_0.4O₂ phase was realized by using iodine as oxidizing agent. The Na_0.58Ni_0.6Co_0.4O₂ phase obtained was used as the positive electrode in sodium batteries. Several structural transformations were observed during discharge (intercalation reaction). The magnetic and electrical study of the Na_xNi_0.6Co_0.4O₂ (x = 1, 0.80, 0.58) phases shows clearly that Ni^III (t₂⁶e¹ in LS configuration) is preferentially oxidized to the tetravalent state compared to CO^III (t₂⁶e⁰ in LS configuration). The sodium diffusion coefficient was also calculated in the solid solution domains. It shows that the diffusion kinetics is faster when sodium ions are situated in a prismatic environment.

Affiliations:

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Le document en format XML

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Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 system : Physical and electrochemical studies</title>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">On the Na<sub>x</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 system : Physical and electrochemical studies</title>
<author><name sortKey="Saadoune, I" sort="Saadoune, I" uniqKey="Saadoune I" first="I." last="Saadoune">I. Saadoune</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Université Cadi-Ayyad, Laboratoire de Chimie du Solide Minéral, Faculté des Sciences-Semlalia, B. P. S15</s1>
<s2>Marrakesh</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>Maroc</country>
<wicri:noRegion>Marrakesh</wicri:noRegion>
</affiliation>
</author>
<author><name sortKey="Maazaz, A" sort="Maazaz, A" uniqKey="Maazaz A" first="A." last="Maazaz">A. Maazaz</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Université Cadi-Ayyad, Laboratoire de Chimie du Solide Minéral, Faculté des Sciences-Semlalia, B. P. S15</s1>
<s2>Marrakesh</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>Maroc</country>
<wicri:noRegion>Marrakesh</wicri:noRegion>
</affiliation>
</author>
<author><name sortKey="Menetrier, M" sort="Menetrier, M" uniqKey="Menetrier M" first="M." last="Menetrier">M. Menetrier</name>
<affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Institut de Chimie de la Matière Condensée de Bordeaux and Ecole Nationale Supérieure de Chimie et Physique de Bordeaux, Avenue Dr. A. Schweitzer</s1>
<s2>33608 Pessac</s2>
<s3>FRA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Nouvelle-Aquitaine</region>
<region type="old region" nuts="2">Aquitaine</region>
<settlement type="city">Pessac</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Delmas, C" sort="Delmas, C" uniqKey="Delmas C" first="C." last="Delmas">C. Delmas</name>
<affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Institut de Chimie de la Matière Condensée de Bordeaux and Ecole Nationale Supérieure de Chimie et Physique de Bordeaux, Avenue Dr. A. Schweitzer</s1>
<s2>33608 Pessac</s2>
<s3>FRA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>France</country>
<placeName><region type="region" nuts="2">Nouvelle-Aquitaine</region>
<region type="old region" nuts="2">Aquitaine</region>
<settlement type="city">Pessac</settlement>
</placeName>
</affiliation>
</author>
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<series><title level="j" type="main">Journal of solid state chemistry</title>
<title level="j" type="abbreviated">J. solid state chem.</title>
<idno type="ISSN">0022-4596</idno>
<imprint><date when="1996">1996</date>
</imprint>
</series>
</biblStruct>
</sourceDesc>
<seriesStmt><title level="j" type="main">Journal of solid state chemistry</title>
<title level="j" type="abbreviated">J. solid state chem.</title>
<idno type="ISSN">0022-4596</idno>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Cobalt Oxides</term>
<term>Desinsertion</term>
<term>Diffusion coefficient</term>
<term>Electrochemical reaction</term>
<term>Electrode material</term>
<term>Electrolyte solution</term>
<term>Intercalation compound</term>
<term>Iodine</term>
<term>Kinetics</term>
<term>Lattice parameters</term>
<term>Magnetic properties</term>
<term>Nickel Oxides</term>
<term>Non aqueous solution</term>
<term>Quaternary compound</term>
<term>Secondary cell</term>
<term>Sodium Oxides</term>
<term>XRD</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Sodium Oxyde</term>
<term>Nickel Oxyde</term>
<term>Cobalt Oxyde</term>
<term>Composé quaternaire</term>
<term>Réaction électrochimique</term>
<term>Composé insertion</term>
<term>Désinsertion</term>
<term>Iode</term>
<term>Matériau électrode</term>
<term>Accumulateur électrochimique</term>
<term>Coefficient diffusion</term>
<term>Cinétique</term>
<term>Solution électrolyte</term>
<term>Solution non aqueuse</term>
<term>XRD</term>
<term>Paramètre cristallin</term>
<term>Propriété magnétique</term>
<term>NaxNi0,6Co0,4O2</term>
<term>Co Na Ni O</term>
</keywords>
<keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Iode</term>
</keywords>
</textClass>
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<front><div type="abstract" xml:lang="en">Sodium chemical deintercalation from the NaNi<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 phase was realized by using iodine as oxidizing agent. The Na<sub>0.58</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 phase obtained was used as the positive electrode in sodium batteries. Several structural transformations were observed during discharge (intercalation reaction). The magnetic and electrical study of the Na<sub>x</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 (x = 1, 0.80, 0.58) phases shows clearly that Ni<sup>III</sup>
 (t<sub>2</sub>
<sup>6</sup>
e<sup>1</sup>
 in LS configuration) is preferentially oxidized to the tetravalent state compared to CO<sup>III</sup>
 (t<sub>2</sub>
<sup>6</sup>
e<sup>0</sup>
 in LS configuration). The sodium diffusion coefficient was also calculated in the solid solution domains. It shows that the diffusion kinetics is faster when sodium ions are situated in a prismatic environment.</div>
</front>
</TEI>
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</fA01>
<fA02 i1="01"><s0>JSSCBI</s0>
</fA02>
<fA03 i2="1"><s0>J. solid state chem.</s0>
</fA03>
<fA05><s2>122</s2>
</fA05>
<fA06><s2>1</s2>
</fA06>
<fA08 i1="01" i2="1" l="ENG"><s1>On the Na<sub>x</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 system : Physical and electrochemical studies</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>SAADOUNE (I.)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>MAAZAZ (A.)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>MENETRIER (M.)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>DELMAS (C.)</s1>
</fA11>
<fA14 i1="01"><s1>Université Cadi-Ayyad, Laboratoire de Chimie du Solide Minéral, Faculté des Sciences-Semlalia, B. P. S15</s1>
<s2>Marrakesh</s2>
<s3>MAR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Institut de Chimie de la Matière Condensée de Bordeaux and Ecole Nationale Supérieure de Chimie et Physique de Bordeaux, Avenue Dr. A. Schweitzer</s1>
<s2>33608 Pessac</s2>
<s3>FRA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</fA14>
<fA20><s1>111-117</s1>
</fA20>
<fA21><s1>1996</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>14677</s2>
<s5>354000053351700190</s5>
</fA43>
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</fA60>
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</fA64>
<fA66 i1="01"><s0>USA</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Sodium chemical deintercalation from the NaNi<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 phase was realized by using iodine as oxidizing agent. The Na<sub>0.58</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 phase obtained was used as the positive electrode in sodium batteries. Several structural transformations were observed during discharge (intercalation reaction). The magnetic and electrical study of the Na<sub>x</sub>
Ni<sub>0.6</sub>
Co<sub>0.4</sub>
O<sub>2</sub>
 (x = 1, 0.80, 0.58) phases shows clearly that Ni<sup>III</sup>
 (t<sub>2</sub>
<sup>6</sup>
e<sup>1</sup>
 in LS configuration) is preferentially oxidized to the tetravalent state compared to CO<sup>III</sup>
 (t<sub>2</sub>
<sup>6</sup>
e<sup>0</sup>
 in LS configuration). The sodium diffusion coefficient was also calculated in the solid solution domains. It shows that the diffusion kinetics is faster when sodium ions are situated in a prismatic environment.</s0>
</fC01>
<fC02 i1="01" i2="X"><s0>001C01H05</s0>
</fC02>
<fC02 i1="02" i2="X"><s0>001D05I03E</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Sodium Oxyde</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Sodium Oxides</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Sodio Óxido</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE"><s0>Nickel Oxyde</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>FX</s2>
<s2>NA</s2>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG"><s0>Nickel Oxides</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>FX</s2>
<s2>NA</s2>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA"><s0>Niquel Óxido</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>FX</s2>
<s2>NA</s2>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE"><s0>Cobalt Oxyde</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Cobalt Oxides</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Cobalto Óxido</s0>
<s1>ACT</s1>
<s2>NC</s2>
<s2>NA</s2>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE"><s0>Composé quaternaire</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG"><s0>Quaternary compound</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA"><s0>Compuesto cuaternario</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Réaction électrochimique</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Electrochemical reaction</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA"><s0>Reacción electroquímica</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Composé insertion</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Intercalation compound</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Compuesto inserción</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Désinsertion</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Desinsertion</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Desinserción</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Iode</s0>
<s1>ENT</s1>
<s2>NC</s2>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Iodine</s0>
<s1>ENT</s1>
<s2>NC</s2>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="GER"><s0>Iod</s0>
<s1>ENT</s1>
<s2>NC</s2>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Iodo</s0>
<s1>ENT</s1>
<s2>NC</s2>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Matériau électrode</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Electrode material</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Material electrodo</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Accumulateur électrochimique</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Secondary cell</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="GER"><s0>Elektrische Batterie</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Acumulador electroquímico</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Coefficient diffusion</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Diffusion coefficient</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="GER"><s0>Diffusionskoeffizient</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Coeficiente difusión</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Cinétique</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Kinetics</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="GER"><s0>Kinetik</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Cinética</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Solution électrolyte</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Electrolyte solution</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Solución electrólito</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Solution non aqueuse</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Non aqueous solution</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Solución no acuosa</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>XRD</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>XRD</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Paramètre cristallin</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Lattice parameters</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="X" l="GER"><s0>Gitterparameter</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Parámetro cristalino</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Propriété magnétique</s0>
<s5>18</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Magnetic properties</s0>
<s5>18</s5>
</fC03>
<fC03 i1="17" i2="X" l="GER"><s0>Magnetische Eigenschaft</s0>
<s5>18</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Propiedad magnética</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>NaxNi0,6Co0,4O2</s0>
<s4>INC</s4>
<s5>52</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Co Na Ni O</s0>
<s4>INC</s4>
<s5>53</s5>
</fC03>
<fC07 i1="01" i2="X" l="FRE"><s0>Métal transition Composé</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>16</s5>
</fC07>
<fC07 i1="01" i2="X" l="ENG"><s0>Transition metal Compounds</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>16</s5>
</fC07>
<fC07 i1="01" i2="X" l="SPA"><s0>Metal transición Compuesto</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>16</s5>
</fC07>
<fN21><s1>119</s1>
</fN21>
</pA>
</standard>
</inist>
<affiliations><list><country><li>France</li>
<li>Maroc</li>
</country>
<region><li>Aquitaine</li>
<li>Nouvelle-Aquitaine</li>
</region>
<settlement><li>Pessac</li>
</settlement>
</list>
<tree><country name="Maroc"><noRegion><name sortKey="Saadoune, I" sort="Saadoune, I" uniqKey="Saadoune I" first="I." last="Saadoune">I. Saadoune</name>
</noRegion>
<name sortKey="Maazaz, A" sort="Maazaz, A" uniqKey="Maazaz A" first="A." last="Maazaz">A. Maazaz</name>
</country>
<country name="France"><region name="Nouvelle-Aquitaine"><name sortKey="Menetrier, M" sort="Menetrier, M" uniqKey="Menetrier M" first="M." last="Menetrier">M. Menetrier</name>
</region>
<name sortKey="Delmas, C" sort="Delmas, C" uniqKey="Delmas C" first="C." last="Delmas">C. Delmas</name>
</country>
</tree>
</affiliations>
</record>

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On the NaxNi0.6Co0.4O2 system : Physical and electrochemical studies

On the NaxNi0.6Co0.4O2 system : Physical and electrochemical studies

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