Terpenic olefin epoxidation using metals acetylacetonates as catalysts
Identifieur interne : 000998 ( Istex/Corpus ); précédent : 000997; suivant : 000999Terpenic olefin epoxidation using metals acetylacetonates as catalysts
Auteurs : Naima Fdil ; Abderrahmane Romane ; Smail Allaoud ; Abdallah Karim ; Yves Castanet ; André MortreuxSource :
- Journal of Molecular Catalysis A: Chemical [ 1381-1169 ] ; 1996.
Abstract
Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (Mn(acac)n) have been used, some of which also gave satisfactory results.
Url:
DOI: 10.1016/1381-1169(95)00284-7
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de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Karim, Abdallah" sort="Karim, Abdallah" uniqKey="Karim A" first="Abdallah" last="Karim">Abdallah Karim</name><affiliation><mods:affiliation>Corresponding author.</mods:affiliation></affiliation><affiliation><mods:affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Castanet, Yves" sort="Castanet, Yves" uniqKey="Castanet Y" first="Yves" last="Castanet">Yves Castanet</name><affiliation><mods:affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</mods:affiliation></affiliation></author><author><name sortKey="Mortreux, Andre" sort="Mortreux, Andre" uniqKey="Mortreux A" first="André" last="Mortreux">André Mortreux</name><affiliation><mods:affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</mods:affiliation></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">ISTEX</idno><idno type="RBID">ISTEX:2CCC00693B144E4B2A3B4295A723045BBB2711C1</idno><date when="1996" year="1996">1996</date><idno type="doi">10.1016/1381-1169(95)00284-7</idno><idno type="url">https://api.istex.fr/document/2CCC00693B144E4B2A3B4295A723045BBB2711C1/fulltext/pdf</idno><idno type="wicri:Area/Istex/Corpus">000998</idno><idno type="wicri:explorRef" wicri:stream="Istex" wicri:step="Corpus" wicri:corpus="ISTEX">000998</idno></publicationStmt><sourceDesc><biblStruct><analytic><title level="a">Terpenic olefin epoxidation using metals acetylacetonates as catalysts</title><author><name sortKey="Fdil, Naima" sort="Fdil, Naima" uniqKey="Fdil N" first="Naima" last="Fdil">Naima Fdil</name><affiliation><mods:affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Romane, Abderrahmane" sort="Romane, Abderrahmane" uniqKey="Romane A" first="Abderrahmane" last="Romane">Abderrahmane Romane</name><affiliation><mods:affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Allaoud, Smail" sort="Allaoud, Smail" uniqKey="Allaoud S" first="Smail" last="Allaoud">Smail Allaoud</name><affiliation><mods:affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Karim, Abdallah" sort="Karim, Abdallah" uniqKey="Karim A" first="Abdallah" last="Karim">Abdallah Karim</name><affiliation><mods:affiliation>Corresponding author.</mods:affiliation></affiliation><affiliation><mods:affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</mods:affiliation></affiliation></author><author><name sortKey="Castanet, Yves" sort="Castanet, Yves" uniqKey="Castanet Y" first="Yves" last="Castanet">Yves Castanet</name><affiliation><mods:affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</mods:affiliation></affiliation></author><author><name sortKey="Mortreux, Andre" sort="Mortreux, Andre" uniqKey="Mortreux A" first="André" last="Mortreux">André Mortreux</name><affiliation><mods:affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</mods:affiliation></affiliation></author></analytic><monogr></monogr><series><title level="j">Journal of Molecular Catalysis A: Chemical</title><title level="j" type="abbrev">MOLCAA</title><idno type="ISSN">1381-1169</idno><imprint><publisher>ELSEVIER</publisher><date type="published" when="1996">1996</date><biblScope unit="volume">108</biblScope><biblScope unit="issue">1</biblScope><biblScope unit="page" from="15">15</biblScope><biblScope unit="page" to="21">21</biblScope></imprint><idno type="ISSN">1381-1169</idno></series><idno type="istex">2CCC00693B144E4B2A3B4295A723045BBB2711C1</idno><idno type="DOI">10.1016/1381-1169(95)00284-7</idno><idno type="PII">1381-1169(95)00284-7</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">1381-1169</idno></seriesStmt></fileDesc><profileDesc><textClass></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (Mn(acac)n) have been used, some of which also gave satisfactory results.</div></front></TEI><istex><corpusName>elsevier</corpusName><author><json:item><name>Naima Fdil</name><affiliations><json:string>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</json:string></affiliations></json:item><json:item><name>Abderrahmane Romane</name><affiliations><json:string>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</json:string></affiliations></json:item><json:item><name>Smail Allaoud</name><affiliations><json:string>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</json:string></affiliations></json:item><json:item><name>Abdallah Karim</name><affiliations><json:string>Corresponding author.</json:string><json:string>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</json:string></affiliations></json:item><json:item><name>Yves Castanet</name><affiliations><json:string>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</json:string></affiliations></json:item><json:item><name>André Mortreux</name><affiliations><json:string>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</json:string></affiliations></json:item></author><subject><json:item><lang><json:string>eng</json:string></lang><value>Chemical and metal catalysis</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Epoxidation</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Nickel</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Acetylacetonate</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Transition metals</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Terpenic olefins</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Oxygen</value></json:item></subject><language><json:string>eng</json:string></language><originalGenre><json:string>Full-length article</json:string></originalGenre><abstract>Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (Mn(acac)n) have been used, some of which also gave satisfactory results.</abstract><qualityIndicators><score>2.136</score><pdfVersion>1.2</pdfVersion><pdfPageSize>648 x 864 pts</pdfPageSize><refBibsNative>true</refBibsNative><keywordCount>7</keywordCount><abstractCharCount>385</abstractCharCount><pdfWordCount>1512</pdfWordCount><pdfCharCount>11002</pdfCharCount><pdfPageCount>7</pdfPageCount><abstractWordCount>52</abstractWordCount></qualityIndicators><title>Terpenic olefin epoxidation using metals acetylacetonates as 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catalysts</title></titleStmt><publicationStmt><authority>ISTEX</authority><publisher>ELSEVIER</publisher><availability><p>ELSEVIER</p></availability><date>1996</date></publicationStmt><notesStmt><note type="content">Section title: Article</note></notesStmt><sourceDesc><biblStruct type="inbook"><analytic><title level="a">Terpenic olefin epoxidation using metals acetylacetonates as catalysts</title><author xml:id="author-1"><persName><forename type="first">Naima</forename><surname>Fdil</surname></persName><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation></author><author xml:id="author-2"><persName><forename type="first">Abderrahmane</forename><surname>Romane</surname></persName><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation></author><author xml:id="author-3"><persName><forename type="first">Smail</forename><surname>Allaoud</surname></persName><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation></author><author xml:id="author-4"><persName><forename type="first">Abdallah</forename><surname>Karim</surname></persName><affiliation>Corresponding author.</affiliation><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation></author><author xml:id="author-5"><persName><forename type="first">Yves</forename><surname>Castanet</surname></persName><affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</affiliation></author><author xml:id="author-6"><persName><forename type="first">André</forename><surname>Mortreux</surname></persName><affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</affiliation></author></analytic><monogr><title level="j">Journal of Molecular Catalysis A: Chemical</title><title level="j" type="abbrev">MOLCAA</title><idno type="pISSN">1381-1169</idno><idno type="PII">S1381-1169(00)X0008-8</idno><imprint><publisher>ELSEVIER</publisher><date type="published" when="1996"></date><biblScope unit="volume">108</biblScope><biblScope unit="issue">1</biblScope><biblScope unit="page" from="15">15</biblScope><biblScope unit="page" to="21">21</biblScope></imprint></monogr><idno type="istex">2CCC00693B144E4B2A3B4295A723045BBB2711C1</idno><idno type="DOI">10.1016/1381-1169(95)00284-7</idno><idno type="PII">1381-1169(95)00284-7</idno></biblStruct></sourceDesc></fileDesc><profileDesc><creation><date>1996</date></creation><langUsage><language ident="en">en</language></langUsage><abstract xml:lang="en"><p>Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (Mn(acac)n) have been used, some of which also gave satisfactory results.</p></abstract><textClass><keywords scheme="keyword"><list><head>article-category</head><item><term>Chemical and metal catalysis</term></item></list></keywords></textClass><textClass><keywords scheme="keyword"><list><head>Keywords</head><item><term>Epoxidation</term></item><item><term>Nickel</term></item><item><term>Acetylacetonate</term></item><item><term>Transition metals</term></item><item><term>Terpenic olefins</term></item><item><term>Oxygen</term></item></list></keywords></textClass></profileDesc><revisionDesc><change when="1996">Published</change></revisionDesc></teiHeader></istex:fulltextTEI><json:item><original>false</original><mimetype>text/plain</mimetype><extension>txt</extension><uri>https://api.istex.fr/document/2CCC00693B144E4B2A3B4295A723045BBB2711C1/fulltext/txt</uri></json:item></fulltext><metadata><istex:metadataXml wicri:clean="Elsevier, elements deleted: tail"><istex:xmlDeclaration>version="1.0" encoding="utf-8"</istex:xmlDeclaration><istex:docType PUBLIC="-//ES//DTD journal article DTD version 4.5.2//EN//XML" URI="art452.dtd" name="istex:docType"></istex:docType><istex:document><converted-article version="4.5.2" docsubtype="fla"><item-info><jid>MOLCAA</jid><aid>95002847</aid><ce:pii>1381-1169(95)00284-7</ce:pii><ce:doi>10.1016/1381-1169(95)00284-7</ce:doi><ce:copyright type="unknown" year="1996"></ce:copyright><ce:doctopics><ce:doctopic><ce:text>Chemical and metal catalysis</ce:text></ce:doctopic></ce:doctopics></item-info><head><ce:dochead><ce:textfn>Article</ce:textfn></ce:dochead><ce:title>Terpenic olefin epoxidation using metals acetylacetonates as catalysts</ce:title><ce:author-group><ce:author><ce:given-name>Naima</ce:given-name><ce:surname>Fdil</ce:surname><ce:cross-ref refid="AFF1"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>Abderrahmane</ce:given-name><ce:surname>Romane</ce:surname><ce:cross-ref refid="AFF1"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>Smail</ce:given-name><ce:surname>Allaoud</ce:surname><ce:cross-ref refid="AFF1"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>Abdallah</ce:given-name><ce:surname>Karim</ce:surname><ce:cross-ref refid="COR1"><ce:sup>∗</ce:sup></ce:cross-ref><ce:cross-ref refid="AFF1"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>Yves</ce:given-name><ce:surname>Castanet</ce:surname><ce:cross-ref refid="AFF2"><ce:sup>b</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>André</ce:given-name><ce:surname>Mortreux</ce:surname><ce:cross-ref refid="AFF2"><ce:sup>b</ce:sup></ce:cross-ref></ce:author><ce:affiliation id="AFF1"><ce:label>a</ce:label><ce:textfn>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</ce:textfn></ce:affiliation><ce:affiliation id="AFF2"><ce:label>b</ce:label><ce:textfn>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</ce:textfn></ce:affiliation><ce:correspondence id="COR1"><ce:label>∗</ce:label><ce:text>Corresponding author.</ce:text></ce:correspondence></ce:author-group><ce:date-received day="29" month="5" year="1995"></ce:date-received><ce:date-accepted day="16" month="10" year="1995"></ce:date-accepted><ce:abstract><ce:section-title>Abstract</ce:section-title><ce:abstract-sec><ce:simple-para>Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (M<ce:sup><ce:italic>n</ce:italic></ce:sup>(acac)<ce:inf><ce:italic>n</ce:italic></ce:inf>) have been used, some of which also gave satisfactory results.</ce:simple-para></ce:abstract-sec></ce:abstract><ce:keywords><ce:section-title>Keywords</ce:section-title><ce:keyword><ce:text>Epoxidation</ce:text></ce:keyword><ce:keyword><ce:text>Nickel</ce:text></ce:keyword><ce:keyword><ce:text>Acetylacetonate</ce:text></ce:keyword><ce:keyword><ce:text>Transition metals</ce:text></ce:keyword><ce:keyword><ce:text>Terpenic olefins</ce:text></ce:keyword><ce:keyword><ce:text>Oxygen</ce:text></ce:keyword></ce:keywords></head></converted-article></istex:document></istex:metadataXml><mods version="3.6"><titleInfo><title>Terpenic olefin epoxidation using metals acetylacetonates as catalysts</title></titleInfo><titleInfo type="alternative" contentType="CDATA"><title>Terpenic olefin epoxidation using metals acetylacetonates as catalysts</title></titleInfo><name type="personal"><namePart type="given">Naima</namePart><namePart type="family">Fdil</namePart><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Abderrahmane</namePart><namePart type="family">Romane</namePart><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Smail</namePart><namePart type="family">Allaoud</namePart><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Abdallah</namePart><namePart type="family">Karim</namePart><affiliation>Corresponding author.</affiliation><affiliation>Laboratoire de Chimie de Coordination, Faculté des Sciences Semlalia, Université Cadi Ayyad, BP S15, Marrakech, Morocco</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Yves</namePart><namePart type="family">Castanet</namePart><affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">André</namePart><namePart type="family">Mortreux</namePart><affiliation>Laboratoire de Catalyse Hétérogène et Homogène, URA CNRS 402, ENSC LILLE, BP 108, 59652 Villeneuve D'Ascq cedex, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="research-article" displayLabel="Full-length article"></genre><originInfo><publisher>ELSEVIER</publisher><dateIssued encoding="w3cdtf">1996</dateIssued><copyrightDate encoding="w3cdtf">1996</copyrightDate></originInfo><language><languageTerm type="code" authority="iso639-2b">eng</languageTerm><languageTerm type="code" authority="rfc3066">en</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType></physicalDescription><abstract lang="en">Efficient epoxidation of natural terpenic olefins is performed using nickel acetylacetonate, oxygen and a branched aldehyde at ambient temperature. Total conversions are achieved with selectivities up to 90% into epoxide. Under the same conditions other catalytic systems using transition metal acetylacetonates (Mn(acac)n) have been used, some of which also gave satisfactory results.</abstract><note type="content">Section title: Article</note><subject><genre>article-category</genre><topic>Chemical and metal catalysis</topic></subject><subject><genre>Keywords</genre><topic>Epoxidation</topic><topic>Nickel</topic><topic>Acetylacetonate</topic><topic>Transition metals</topic><topic>Terpenic olefins</topic><topic>Oxygen</topic></subject><relatedItem type="host"><titleInfo><title>Journal of Molecular Catalysis A: Chemical</title></titleInfo><titleInfo type="abbreviated"><title>MOLCAA</title></titleInfo><genre type="journal">journal</genre><originInfo><dateIssued encoding="w3cdtf">19960425</dateIssued></originInfo><identifier type="ISSN">1381-1169</identifier><identifier type="PII">S1381-1169(00)X0008-8</identifier><part><date>19960425</date><detail type="volume"><number>108</number><caption>vol.</caption></detail><detail type="issue"><number>1</number><caption>no.</caption></detail><extent unit="issue pages"><start>L1</start><end>L3</end></extent><extent unit="issue pages"><start>5</start><end>50</end></extent><extent unit="pages"><start>15</start><end>21</end></extent></part></relatedItem><identifier type="istex">2CCC00693B144E4B2A3B4295A723045BBB2711C1</identifier><identifier type="DOI">10.1016/1381-1169(95)00284-7</identifier><identifier type="PII">1381-1169(95)00284-7</identifier><recordInfo><recordContentSource>ELSEVIER</recordContentSource></recordInfo></mods></metadata><serie></serie></istex></record>Pour manipuler ce document sous Unix (Dilib)
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