η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes
Identifieur interne : 001B81 ( Istex/Corpus ); précédent : 001B80; suivant : 001B82η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes
Auteurs : Kristopher Kolpin ; David EmslieSource :
- Angewandte Chemie International Edition [ 1433-7851 ] ; 2010-04-01.
English descriptors
Abstract
Anyone for pi? The vinylborane PhHCCH‐B(C6F5)2 reacts with zero‐valent Group 10 transition‐metal precursors to form η3‐vinylborane complexes. The platinum tri‐tert‐butylphosphine complex exhibits an η3‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.
Url:
DOI: 10.1002/anie.200906931
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ISTEX:4599F0E6116509F77B6D1AA52B258FEA7380BE25Le document en format XML
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The vinylborane PhHCCH‐B(C6F5)2 reacts with zero‐valent Group 10 transition‐metal precursors to form η3‐vinylborane complexes. The platinum tri‐tert‐butylphosphine complex exhibits an η3‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.</div></front></TEI><istex><corpusName>wiley</corpusName><author><json:item><name>Kristopher B. Kolpin</name><affiliations><json:string>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</json:string></affiliations></json:item><json:item><name>David J. H. Emslie Prof.</name><affiliations><json:string>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</json:string><json:string>E-mail: emslied@mcmaster.ca</json:string></affiliations></json:item></author><subject><json:item><lang><json:string>eng</json:string></lang><value>boranes</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>isoelectronic analogues</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>Lewis acids</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>π interactions</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>transition metals</value></json:item></subject><articleId><json:string>ANIE200906931</json:string></articleId><language><json:string>eng</json:string></language><abstract>Anyone for pi? The vinylborane PhHCCH‐B(C6F5)2 reacts with zero‐valent Group 10 transition‐metal precursors to form η3‐vinylborane complexes. The platinum tri‐tert‐butylphosphine complex exhibits an η3‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.</abstract><qualityIndicators><score>3.434</score><pdfVersion>1.3</pdfVersion><pdfPageSize>595.276 x 841.89 pts (A4)</pdfPageSize><refBibsNative>true</refBibsNative><keywordCount>5</keywordCount><abstractCharCount>335</abstractCharCount><pdfWordCount>3026</pdfWordCount><pdfCharCount>17182</pdfCharCount><pdfPageCount>4</pdfPageCount><abstractWordCount>34</abstractWordCount></qualityIndicators><title>η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes</title><genre.original><json:string>shortCommunication</json:string></genre.original><genre><json:string>brief-communication</json:string></genre><host><volume>49</volume><publisherId><json:string>ANIE</json:string></publisherId><pages><total>4</total><last>2719</last><first>2716</first></pages><issn><json:string>1433-7851</json:string></issn><issue>15</issue><subject><json:item><value>Communication</value></json:item></subject><genre><json:string>journal</json:string></genre><language><json:string>unknown</json:string></language><eissn><json:string>1521-3773</json:string></eissn><title>Angewandte Chemie International Edition</title><doi><json:string>10.1002/(ISSN)1521-3773</json:string></doi></host><publicationDate>2010</publicationDate><copyrightDate>2010</copyrightDate><doi><json:string>10.1002/anie.200906931</json:string></doi><id>4599F0E6116509F77B6D1AA52B258FEA7380BE25</id><score>1</score><fulltext><json:item><original>true</original><mimetype>application/pdf</mimetype><extension>pdf</extension><uri>https://api.istex.fr/document/4599F0E6116509F77B6D1AA52B258FEA7380BE25/fulltext/pdf</uri></json:item><json:item><original>false</original><mimetype>application/zip</mimetype><extension>zip</extension><uri>https://api.istex.fr/document/4599F0E6116509F77B6D1AA52B258FEA7380BE25/fulltext/zip</uri></json:item><istex:fulltextTEI uri="https://api.istex.fr/document/4599F0E6116509F77B6D1AA52B258FEA7380BE25/fulltext/tei"><teiHeader><fileDesc><titleStmt><title level="a" type="main" xml:lang="en">η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes</title></titleStmt><publicationStmt><authority>ISTEX</authority><publisher>WILEY‐VCH Verlag</publisher><pubPlace>Weinheim</pubPlace><availability><p>WILEY</p></availability><date>2010</date></publicationStmt><notesStmt><note type="content">*D.J.H.E. thanks the NSERC of Canada for a Discovery Grant, the Ontario Ministry of Resarch and Innovation for an Early Researcher Award, and the CFI and OIT for New Opportunities Grants. We are also very grateful to I. Vargas‐Baca for help with DFT calculations, and J. F. Britten and H. A. Jenkins for help with X‐ray crystallography.</note><note>NSERC of Canada</note><note>Ontario Ministry of Resarch and Innovation</note><note>CFI</note><note>OIT</note></notesStmt><sourceDesc><biblStruct type="inbook"><analytic><title level="a" type="main" xml:lang="en">η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes</title><author><persName><forename type="first">Kristopher B.</forename><surname>Kolpin</surname></persName><affiliation>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</affiliation></author><author><persName><forename type="first">David J. H.</forename><surname>Emslie</surname></persName><roleName type="degree">Prof.</roleName><email>emslied@mcmaster.ca</email><affiliation>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</affiliation></author></analytic><monogr><title level="j">Angewandte Chemie International Edition</title><title level="j" type="abbrev">Angewandte Chemie International Edition</title><idno type="pISSN">1433-7851</idno><idno type="eISSN">1521-3773</idno><idno type="DOI">10.1002/(ISSN)1521-3773</idno><imprint><publisher>WILEY‐VCH Verlag</publisher><pubPlace>Weinheim</pubPlace><date type="published" when="2010-04-01"></date><biblScope unit="volume">49</biblScope><biblScope unit="issue">15</biblScope><biblScope unit="page" from="2716">2716</biblScope><biblScope unit="page" to="2719">2719</biblScope></imprint></monogr><idno type="istex">4599F0E6116509F77B6D1AA52B258FEA7380BE25</idno><idno type="DOI">10.1002/anie.200906931</idno><idno type="ArticleID">ANIE200906931</idno></biblStruct></sourceDesc></fileDesc><profileDesc><creation><date>2010</date></creation><langUsage><language ident="en">en</language></langUsage><abstract xml:lang="en" style="graphical"><p>Anyone for pi? The vinylborane PhHCCH‐B(C6F5)2 reacts with zero‐valent Group 10 transition‐metal precursors to form η3‐vinylborane complexes. The platinum tri‐tert‐butylphosphine complex exhibits an η3‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.</p></abstract><textClass xml:lang="en"><keywords scheme="keyword"><list><head>keywords</head><item><term>boranes</term></item><item><term>isoelectronic analogues</term></item><item><term>Lewis acids</term></item><item><term>π interactions</term></item><item><term>transition metals</term></item></list></keywords></textClass><textClass><keywords scheme="Journal Subject"><list><head>article-category</head><item><term>Communication</term></item></list></keywords></textClass></profileDesc><revisionDesc><change when="2009-12-09">Received</change><change when="2010-04-01">Published</change></revisionDesc></teiHeader></istex:fulltextTEI><json:item><original>false</original><mimetype>text/plain</mimetype><extension>txt</extension><uri>https://api.istex.fr/document/4599F0E6116509F77B6D1AA52B258FEA7380BE25/fulltext/txt</uri></json:item></fulltext><metadata><istex:metadataXml wicri:clean="Wiley, elements deleted: body"><istex:xmlDeclaration>version="1.0" encoding="UTF-8" standalone="yes"</istex:xmlDeclaration><istex:document><component version="2.0" type="serialArticle" xml:lang="en"><header><publicationMeta level="product"><publisherInfo><publisherName>WILEY‐VCH Verlag</publisherName><publisherLoc>Weinheim</publisherLoc></publisherInfo><doi registered="yes">10.1002/(ISSN)1521-3773</doi><issn type="print">1433-7851</issn><issn type="electronic">1521-3773</issn><idGroup><id type="product" value="ANIE"></id></idGroup><titleGroup><title type="main" xml:lang="en" sort="ANGEWANDTE CHEMIE INTERNATIONAL EDITION">Angewandte Chemie International Edition</title><title type="short">Angewandte Chemie International Edition</title></titleGroup></publicationMeta><publicationMeta level="part" position="150"><doi origin="wiley" registered="yes">10.1002/anie.v49:15</doi><numberingGroup><numbering type="journalVolume" number="49">49</numbering><numbering type="journalIssue">15</numbering></numberingGroup><coverDate startDate="2010-04-01">April 1, 2010</coverDate></publicationMeta><publicationMeta level="unit" type="shortCommunication" position="15" status="forIssue"><doi origin="wiley" registered="yes">10.1002/anie.200906931</doi><idGroup><id type="unit" value="ANIE200906931"></id></idGroup><countGroup><count type="pageTotal" number="4"></count></countGroup><titleGroup><title type="articleCategory">Communication</title><title type="tocHeading1">Communications</title><title type="tocHeading2">Vinylborane Complexes</title></titleGroup><copyright ownership="publisher">Copyright © 2010 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</copyright><eventGroup><event type="manuscriptReceived" date="2009-12-09"></event><event type="manuscriptRevised" date="2010-01-20"></event><event type="firstOnline" date="2010-03-15"></event><event type="publishedOnlineFinalForm" date="2010-03-26"></event><event type="xmlConverted" agent="Converter:JWSART34_TO_WML3G version:2.3.6 mode:FullText source:FullText result:FullText mathml2tex" date="2010-04-30"></event><event type="xmlConverted" agent="Converter:WILEY_ML3G_TO_WILEY_ML3GV2 version:3.8.8" date="2014-01-03"></event><event type="xmlConverted" agent="Converter:WML3G_To_WML3G version:4.1.7 mode:FullText,remove_FC" date="2014-10-14"></event></eventGroup><numberingGroup><numbering type="pageFirst">2716</numbering><numbering type="pageLast">2719</numbering></numberingGroup><objectNameGroup><objectName elementName="figure">Scheme</objectName></objectNameGroup><linkGroup><link type="toTypesetVersion" href="file:ANIE.ANIE200906931.pdf"></link></linkGroup></publicationMeta><contentMeta><countGroup><count type="figureTotal" number="7"></count><count type="tableTotal" number="0"></count><count type="referenceTotal" number="55"></count></countGroup><titleGroup><title type="main" xml:lang="en">η<sup>3</sup>‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes<link href="#nss"></link></title></titleGroup><creators><creator xml:id="au1" creatorRole="author" affiliationRef="#aa"><personName><givenNames>Kristopher B.</givenNames><familyName>Kolpin</familyName></personName></creator><creator xml:id="au2" creatorRole="author" affiliationRef="#aa"><personName><givenNames>David J. H.</givenNames><familyName>Emslie</familyName><degrees>Prof.</degrees></personName><contactDetails><email>emslied@mcmaster.ca</email></contactDetails></creator></creators><affiliationGroup><affiliation xml:id="aa" countryCode="CA" type="organization"><unparsedAffiliation>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 <url href="http://www.chemistry.mcmaster.ca/faculty/emslie/">http://www.chemistry.mcmaster.ca/faculty/emslie/</url></unparsedAffiliation></affiliation></affiliationGroup><keywordGroup xml:lang="en" type="author"><keyword xml:id="kwd1">boranes</keyword><keyword xml:id="kwd2">isoelectronic analogues</keyword><keyword xml:id="kwd3">Lewis acids</keyword><keyword xml:id="kwd4">π interactions</keyword><keyword xml:id="kwd5">transition metals</keyword></keywordGroup><fundingInfo><fundingAgency>NSERC of Canada</fundingAgency></fundingInfo><fundingInfo><fundingAgency>Ontario Ministry of Resarch and Innovation</fundingAgency></fundingInfo><fundingInfo><fundingAgency>CFI</fundingAgency></fundingInfo><fundingInfo><fundingAgency>OIT</fundingAgency></fundingInfo><supportingInformation><p>Detailed facts of importance to specialist readers are published as ”Supporting Information”. Such documents are peer‐reviewed, but not copy‐edited or typeset. They are made available as submitted by the authors. </p><supportingInfoItem><mediaResource alt="supporting information" href="urn-x:wiley:14337851:media:anie200906931:anie_200906931_sm_miscellaneous_information"></mediaResource><caption>miscellaneous_information</caption></supportingInfoItem></supportingInformation><abstractGroup><abstract type="graphical" xml:lang="en"><p><b>Anyone for pi?</b> The vinylborane PhHCCH‐B(C<sub>6</sub>F<sub>5</sub>)<sub>2</sub> reacts with zero‐valent Group 10 transition‐metal precursors to form η<sup>3</sup>‐vinylborane complexes. The platinum tri‐<i>tert</i>‐butylphosphine complex exhibits an η<sup>3</sup>‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.<blockFixed type="graphic"><mediaResourceGroup><mediaResource alt="image" eRights="yes" copyright="WILEY-VCH" href="urn:x-wiley:14337851:media:ANIE200906931:content"></mediaResource><mediaResource alt="thumbnail image" rendition="webLoRes" mimeType="image/gif" href=""></mediaResource><mediaResource alt="original image" rendition="webOriginal" mimeType="image/gif" href=""></mediaResource><mediaResource alt="magnified image" rendition="webHiRes" mimeType="image/gif" href=""></mediaResource></mediaResourceGroup></blockFixed></p></abstract></abstractGroup></contentMeta><noteGroup><note xml:id="nss"><p>D.J.H.E. thanks the NSERC of Canada for a Discovery Grant, the Ontario Ministry of Resarch and Innovation for an Early Researcher Award, and the CFI and OIT for New Opportunities Grants. We are also very grateful to I. Vargas‐Baca for help with DFT calculations, and J. F. Britten and H. A. Jenkins for help with X‐ray crystallography.</p></note></noteGroup></header></component></istex:document></istex:metadataXml><mods version="3.6"><titleInfo lang="en"><title>η3‐Vinylborane Complexes of Platinum and Nickel: Borataallyl‐ and Alkyl/Borataalkene‐Like Coordination Modes</title></titleInfo><titleInfo type="alternative" contentType="CDATA" lang="en"><title>η</title></titleInfo><name type="personal"><namePart type="given">Kristopher B.</namePart><namePart type="family">Kolpin</namePart><affiliation>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">David J. H.</namePart><namePart type="family">Emslie</namePart><namePart type="termsOfAddress">Prof.</namePart><affiliation>Department of Chemistry and Chemical Biology, McMaster University, 1280 Main Street West, Hamilton, Ontario, L8S 4M1 (Canada), Fax: (+1) 905‐522‐2509 http://www.chemistry.mcmaster.ca/faculty/emslie/</affiliation><affiliation>E-mail: emslied@mcmaster.ca</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="brief-communication" displayLabel="shortCommunication"></genre><originInfo><publisher>WILEY‐VCH Verlag</publisher><place><placeTerm type="text">Weinheim</placeTerm></place><dateIssued encoding="w3cdtf">2010-04-01</dateIssued><dateCaptured encoding="w3cdtf">2009-12-09</dateCaptured><copyrightDate encoding="w3cdtf">2010</copyrightDate></originInfo><language><languageTerm type="code" authority="rfc3066">en</languageTerm><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType><extent unit="figures">7</extent><extent unit="references">55</extent></physicalDescription><abstract type="graphical" lang="en">Anyone for pi? The vinylborane PhHCCH‐B(C6F5)2 reacts with zero‐valent Group 10 transition‐metal precursors to form η3‐vinylborane complexes. The platinum tri‐tert‐butylphosphine complex exhibits an η3‐borataallyl‐like coordination mode whereas the nickel bis(triphenylphosphine) complex tends towards alkyl/borataalkene coordination.</abstract><note type="content">*D.J.H.E. thanks the NSERC of Canada for a Discovery Grant, the Ontario Ministry of Resarch and Innovation for an Early Researcher Award, and the CFI and OIT for New Opportunities Grants. We are also very grateful to I. Vargas‐Baca for help with DFT calculations, and J. F. Britten and H. A. Jenkins for help with X‐ray crystallography.</note><note type="funding">NSERC of Canada</note><note type="funding">Ontario Ministry of Resarch and Innovation</note><note type="funding">CFI</note><note type="funding">OIT</note><subject lang="en"><genre>keywords</genre><topic>boranes</topic><topic>isoelectronic analogues</topic><topic>Lewis acids</topic><topic>π interactions</topic><topic>transition metals</topic></subject><relatedItem type="host"><titleInfo><title>Angewandte Chemie International Edition</title></titleInfo><titleInfo type="abbreviated"><title>Angewandte Chemie International Edition</title></titleInfo><genre type="journal">journal</genre><note type="content"> Detailed facts of importance to specialist readers are published as ”Supporting Information”. Such documents are peer‐reviewed, but not copy‐edited or typeset. They are made available as submitted by the authors.Supporting Info Item: miscellaneous_information - </note><subject><genre>article-category</genre><topic>Communication</topic></subject><identifier type="ISSN">1433-7851</identifier><identifier type="eISSN">1521-3773</identifier><identifier type="DOI">10.1002/(ISSN)1521-3773</identifier><identifier type="PublisherID">ANIE</identifier><part><date>2010</date><detail type="volume"><caption>vol.</caption><number>49</number></detail><detail type="issue"><caption>no.</caption><number>15</number></detail><extent unit="pages"><start>2716</start><end>2719</end><total>4</total></extent></part></relatedItem><identifier type="istex">4599F0E6116509F77B6D1AA52B258FEA7380BE25</identifier><identifier type="DOI">10.1002/anie.200906931</identifier><identifier type="ArticleID">ANIE200906931</identifier><accessCondition type="use and reproduction" contentType="copyright">Copyright © 2010 WILEY‐VCH Verlag GmbH & Co. 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