System-forming functions of bound water in the mechanism of topochemical reactions of formation of ultrathin layers on water surface
Identifieur interne : 002295 ( Istex/Corpus ); précédent : 002294; suivant : 002296System-forming functions of bound water in the mechanism of topochemical reactions of formation of ultrathin layers on water surface
Auteurs : N. A. Bulienkov ; E. A. ZheligovskayaSource :
- Biophysics [ 0006-3509 ] ; 2013-01-01.
English descriptors
Abstract
Abstract: The system-forming role of the surface layer of water in the process of formation of ultrathin layers from the epoxide oligomer and triethylenetetramine or phosphotungstic acid on the surface of the aqueous phase is shown. Previously, this process was studied experimentally. The surface layer of the aqueous phase plays the role of a matrix, on which an epoxide oligomer monolayer and triethylenetetramine or phosphotungstic acid molecules are immobilized by hydrogen-bonding with water molecules from above or from below this matrix, respectively. Thus, topochemical reactions between the epoxide oligomer and triethylenetetramine or between the epoxide oligomer molecules in the presence of phosphotungstic acid become possible, so that ultrathin network epoxide-triethylenetetramine or epoxide layers are formed on the surface of water.
Url:
DOI: 10.1134/S0006350913010041
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DisplayOrder="Western"><GivenName>N.</GivenName><GivenName>A.</GivenName><FamilyName>Bulienkov</FamilyName></AuthorName><Contact><Email>lmm@phyche.ac.ru</Email></Contact></Author><Author AffiliationIDS="Aff17621"><AuthorName DisplayOrder="Western"><GivenName>E.</GivenName><GivenName>A.</GivenName><FamilyName>Zheligovskaya</FamilyName></AuthorName></Author><Affiliation ID="Aff17621"><OrgDivision>Frumkin Institute of Physical Chemistry and Electrochemistry</OrgDivision><OrgName>Russian Academy of Sciences</OrgName><OrgAddress><City>Moscow</City><Postcode>119071</Postcode><Country Code="RU">Russia</Country></OrgAddress></Affiliation></AuthorGroup><Abstract ID="Abs1" Language="En"><Heading>Abstract</Heading><Para>The system-forming role of the surface layer of water in the process of formation of ultrathin layers from the epoxide oligomer and triethylenetetramine or phosphotungstic acid on the surface of the aqueous phase is shown. Previously, this process was studied experimentally. The surface layer of the aqueous phase plays the role of a matrix, on which an epoxide oligomer monolayer and triethylenetetramine or phosphotungstic acid molecules are immobilized by hydrogen-bonding with water molecules from above or from below this matrix, respectively. Thus, topochemical reactions between the epoxide oligomer and triethylenetetramine or between the epoxide oligomer molecules in the presence of phosphotungstic acid become possible, so that ultrathin network epoxide-triethylenetetramine or epoxide layers are formed on the surface of water.</Para></Abstract><KeywordGroup Language="En"><Heading>Keywords</Heading><Keyword>bound water</Keyword><Keyword>self-organization</Keyword><Keyword>surface layer</Keyword><Keyword>structural mechanism</Keyword></KeywordGroup><ArticleNote Type="Misc"><SimplePara>Original Russian Text © N.A. Bulienkov, E.A. Zheligovskaya, 2013, published in Biofizika, 2013, Vol. 58, No. 1, pp. 8–26.</SimplePara></ArticleNote></ArticleHeader><NoBody></NoBody></Article></Issue></Volume></Journal></Publisher></istex:document></istex:metadataXml><mods version="3.6"><titleInfo lang="en"><title>System-forming functions of bound water in the mechanism of topochemical reactions of formation of ultrathin layers on water surface</title></titleInfo><titleInfo type="alternative" contentType="CDATA"><title>System-forming functions of bound water in the mechanism of topochemical reactions of formation of ultrathin layers on water surface</title></titleInfo><name type="personal" displayLabel="corresp"><namePart type="given">N.</namePart><namePart type="given">A.</namePart><namePart type="family">Bulienkov</namePart><affiliation>Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, 119071, Moscow, Russia</affiliation><affiliation>E-mail: lmm@phyche.ac.ru</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">E.</namePart><namePart type="given">A.</namePart><namePart type="family">Zheligovskaya</namePart><affiliation>Frumkin Institute of Physical Chemistry and Electrochemistry, Russian Academy of Sciences, 119071, Moscow, Russia</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="research-article" displayLabel="OriginalPaper" authority="ISTEX" authorityURI="https://content-type.data.istex.fr" valueURI="https://content-type.data.istex.fr/ark:/67375/XTP-1JC4F85T-7">research-article</genre><originInfo><publisher>SP MAIK Nauka/Interperiodica</publisher><place><placeTerm type="text">Dordrecht</placeTerm></place><dateCreated encoding="w3cdtf">2012-10-01</dateCreated><dateIssued encoding="w3cdtf">2013-01-01</dateIssued><copyrightDate encoding="w3cdtf">2013</copyrightDate></originInfo><language><languageTerm type="code" authority="rfc3066">en</languageTerm><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><abstract lang="en">Abstract: The system-forming role of the surface layer of water in the process of formation of ultrathin layers from the epoxide oligomer and triethylenetetramine or phosphotungstic acid on the surface of the aqueous phase is shown. Previously, this process was studied experimentally. The surface layer of the aqueous phase plays the role of a matrix, on which an epoxide oligomer monolayer and triethylenetetramine or phosphotungstic acid molecules are immobilized by hydrogen-bonding with water molecules from above or from below this matrix, respectively. 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