Two Non‐covalent Methods to Decorate Nanoparticles with Block Copolymers
Identifieur interne : 001B75 ( Istex/Corpus ); précédent : 001B74; suivant : 001B76Two Non‐covalent Methods to Decorate Nanoparticles with Block Copolymers
Auteurs : Christophe SchatzSource :
- Macromolecular Chemistry and Physics [ 1022-1352 ] ; 2014-05.
Abstract
The physical adsorption of block copolymers is a simple and reliable approach to functionalize the surface of organic or inorganic nanoparticles. This article presents two novel methods of particle coating with block copolymers that may apply to various aqueous colloidal dispersions. The first method relies on the use of charged block copolymers having two adsorbing blocks, which can adopt a typical anchor‐buoy conformation at the particle surface when proper conditions are used. The second approach consists of self‐assembling a bilayer of amphiphilic block copolymers around charged nanoparticles. In both cases, a special emphasis is placed on the process used to control and orient the molecular interactions between the copolymer and the particles.
Two novel approaches of particle functionalization with block copolymers are introduced. The first method is based on the physical adsorption of a charged block copolymer with two adsorbing blocks. The second method consists of self‐assembling a bilayer of amphiphilic block copolymer at the particle surface through a change of solvent polarity.
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DOI: 10.1002/macp.201300756
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KGaA, Weinheim</licence></availability><date type="published" when="2014-05"></date></publicationStmt><notesStmt><note type="content-type" subtype="article" source="article" scheme="https://content-type.data.istex.fr/ark:/67375/XTP-6N5SZHKN-D">article</note><note type="publication-type" subtype="journal" scheme="https://publication-type.data.istex.fr/ark:/67375/JMC-0GLKJH51-B">journal</note></notesStmt><sourceDesc><biblStruct type="article"><analytic><title level="a" type="main">Two Non‐covalent Methods to Decorate Nanoparticles with Block Copolymers</title><author xml:id="author-0000" role="corresp"><persName><forename type="first">Christophe</forename><surname>Schatz</surname></persName><state type="biography"><desc><hi rend="bold">Christophe Schatz</hi> has been assistant professor since 2006 at “Ecole Nationale Supérieure de Chimie, Physique et Biologie” (ENSCBP) in Bordeaux and researcher at “Laboratoire de Chimie des Polymères Organiques” (LCPO). In December 2003, he defended his Ph.D. thesis on the solution behavior of polysaccharides and the formation of polyelectrolyte complexes at the University of Lyon. In 2004–2005, he went to the University of Newcastle (Australia) as a postdoctoral fellow to study the behavior of polymer stimuli–responsive micelles at the solid–liquid interface. He is currently working on macromolecular assemblies in solution and at interfaces, with a special focus on polysaccharide‐based systems.
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In December 2003, he defended his Ph.D. thesis on the solution behavior of polysaccharides and the formation of polyelectrolyte complexes at the University of Lyon. In 2004–2005, he went to the University of Newcastle (Australia) as a postdoctoral fellow to study the behavior of polymer stimuli–responsive micelles at the solid–liquid interface. 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This article presents two novel methods of particle coating with block copolymers that may apply to various aqueous colloidal dispersions. The first method relies on the use of charged block copolymers having two adsorbing blocks, which can adopt a typical anchor‐buoy conformation at the particle surface when proper conditions are used. The second approach consists of self‐assembling a bilayer of amphiphilic block copolymers around charged nanoparticles. In both cases, a special emphasis is placed on the process used to control and orient the molecular interactions between the copolymer and the particles.</abstract><abstract type="graphical" lang="en">Two novel approaches of particle functionalization with block copolymers are introduced. The first method is based on the physical adsorption of a charged block copolymer with two adsorbing blocks. The second method consists of self‐assembling a bilayer of amphiphilic block copolymer at the particle surface through a change of solvent polarity.</abstract><subject lang="en"><genre>keywords</genre><topic>block copolymers</topic><topic>nanoparticles</topic><topic>polymer adsorption</topic><topic>polymer brushes</topic><topic>self‐assembly</topic></subject><relatedItem type="host"><titleInfo><title>Macromolecular Chemistry and Physics</title></titleInfo><titleInfo type="abbreviated"><title>Macromol. Chem. Phys.</title></titleInfo><genre type="journal" authority="ISTEX" authorityURI="https://publication-type.data.istex.fr" valueURI="https://publication-type.data.istex.fr/ark:/67375/JMC-0GLKJH51-B">journal</genre><subject><genre>article-category</genre><topic>Talents and Trends</topic><topic>Talents and Trends</topic></subject><identifier type="ISSN">1022-1352</identifier><identifier type="eISSN">1521-3935</identifier><identifier type="DOI">10.1002/(ISSN)1521-3935</identifier><identifier type="PublisherID">MACP</identifier><part><date>2014</date><detail type="volume"><caption>vol.</caption><number>215</number></detail><detail type="issue"><caption>no.</caption><number>10</number></detail><extent unit="pages"><start>945</start><end>957</end><total>13</total></extent></part></relatedItem><relatedItem type="references" displayLabel="macp201300756-cit-0001"><titleInfo><title>Nanomedicine</title></titleInfo><genre>journal-article</genre><note type="citation/reference">a) H. Jia, S. 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