Rational Design of Conjugated Polymer Supramolecules with Tunable Colorimetric Responses
Identifieur interne : 001486 ( Istex/Corpus ); précédent : 001485; suivant : 001487Rational Design of Conjugated Polymer Supramolecules with Tunable Colorimetric Responses
Auteurs : Dong June Ahn ; Sumi Lee ; Jong-Man KimSource :
- Advanced Functional Materials [ 1616-301X ] ; 2009-05-22.
English descriptors
- Teeft :
- Absorption maxima, Alkyl, American chemical society, Amide, Aqueous solution, Aromatic, Aromatic interactions, Carboxylic, Carboxylic groups, Charych, Chem, Chromism, Color change, Color transition, Color transitions, Colorimetric, Colorimetric reversibility, Colorimetric stabilities, Colorimetric stability, Colorimetrically, Complete colorimetric reversibility, Diacetylene, Diacetylene monomer, Diacetylene monomers, Diagnostic method, Ethylene, Ethylene glycol, Feature article, Funct, Glycol, Gmbh, Hanyang university, Headgroup, Headgroup interactions, Heat treatment, High temperature, High temperatures, Inclusion complexes, Intermediate states, Internal amide groups, Irreversible, Isosbestic, Isosbestic point, Isosbestic points, Kgaa, Lipid, Macromolecule, Mater, Mechanical strain, Monomer, Naphthyl, Naphthyl groups, Organic solvents, Original intensity, Pcda, Pda, Phenyl, Polymer, Polymer vesicles, Polymerized, Polymerized vesicles, Reversibility, Reversible, Reversible color transition, Reversible pdas, Reversible thermochromism, Room temperature, Schematic representation, Sensor, Sensor systems, Spectroscopic, Strong headgroup interaction, Strong headgroup interactions, Supramolecules, Thermal cycle, Thermal cycles, Thermal stimulation, Thermochromism, Verlag, Verlag gmbh, Vesicle, Visible spectroscopic monitoring, Weinheim.
Abstract
Polydiacetylenes (PDAs), a family of highly π‐conjugated polymers, have unique characteristics associated with their ability to self‐assemble. Disruption of the extensively delocalized enyne backbones of molecularly ordered PDA sidechains induces a blue‐to‐red color change, which has been elegantly applied in the design of chemosensors. Recently, colorimetrically reversible PDAs have received significant attention, not only to gain a better understanding of the fundamentals of PDA chromism, but also to develop methodologies to overcome limitations associated with their colorimetrically irreversible counterparts. In this article, recent progress made in the field of colorimetrically tunable (reversible, stable, or sensitive) PDAs is described. Major emphasis is given to rational design strategies developed in our group. Relevant mechanistic investigations, a diagnostic method to test colorimetric reversibility, as well as future challenges in this area will be also discussed.
The rational design of thermochromic polydiacetylenes (PDAs) by manipulating strong headgroup interactions, which leads to colorimetrically tunable systems, within the authors' groups is described. In addition, a diagnostic method for assigning colorimetric reversibility to PDAs as well as an analysis of future challenges in this area is also presented.
Url:
DOI: 10.1002/adfm.200801074
Links to Exploration step
ISTEX:92AA1CC74CBB4856292C19A7EF4E3EC5FA055170Le document en format XML
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groups</term><term>Irreversible</term><term>Isosbestic</term><term>Isosbestic point</term><term>Isosbestic points</term><term>Kgaa</term><term>Lipid</term><term>Macromolecule</term><term>Mater</term><term>Mechanical strain</term><term>Monomer</term><term>Naphthyl</term><term>Naphthyl groups</term><term>Organic solvents</term><term>Original intensity</term><term>Pcda</term><term>Pda</term><term>Phenyl</term><term>Polymer</term><term>Polymer vesicles</term><term>Polymerized</term><term>Polymerized vesicles</term><term>Reversibility</term><term>Reversible</term><term>Reversible color transition</term><term>Reversible pdas</term><term>Reversible thermochromism</term><term>Room temperature</term><term>Schematic representation</term><term>Sensor</term><term>Sensor systems</term><term>Spectroscopic</term><term>Strong headgroup interaction</term><term>Strong headgroup interactions</term><term>Supramolecules</term><term>Thermal cycle</term><term>Thermal cycles</term><term>Thermal 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Disruption of the extensively delocalized enyne backbones of molecularly ordered PDA sidechains induces a blue‐to‐red color change, which has been elegantly applied in the design of chemosensors. Recently, colorimetrically reversible PDAs have received significant attention, not only to gain a better understanding of the fundamentals of PDA chromism, but also to develop methodologies to overcome limitations associated with their colorimetrically irreversible counterparts. In this article, recent progress made in the field of colorimetrically tunable (reversible, stable, or sensitive) PDAs is described. Major emphasis is given to rational design strategies developed in our group. Relevant mechanistic investigations, a diagnostic method to test colorimetric reversibility, as well as future challenges in this area will be also discussed.</div><div type="abstract" xml:lang="en">The rational design of thermochromic polydiacetylenes (PDAs) by manipulating strong headgroup interactions, which leads to colorimetrically tunable systems, within the authors' groups is described. In addition, a diagnostic method for assigning colorimetric reversibility to PDAs as well as an analysis of future challenges in this area is also presented.</div></front></TEI><istex><corpusName>wiley</corpusName><keywords><teeft><json:string>pda</json:string><json:string>colorimetric</json:string><json:string>chem</json:string><json:string>colorimetrically</json:string><json:string>vesicle</json:string><json:string>headgroup</json:string><json:string>colorimetric reversibility</json:string><json:string>thermochromism</json:string><json:string>supramolecules</json:string><json:string>reversibility</json:string><json:string>polymer</json:string><json:string>color change</json:string><json:string>funct</json:string><json:string>diacetylene</json:string><json:string>carboxylic</json:string><json:string>weinheim</json:string><json:string>kgaa</json:string><json:string>polymerized</json:string><json:string>verlag 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KGaA, Weinheim</licence></availability><date type="published" when="2009-05-22"></date></publicationStmt><notesStmt><note type="content-type" subtype="article" source="article" scheme="https://content-type.data.istex.fr/ark:/67375/XTP-6N5SZHKN-D">article</note><note type="publication-type" subtype="journal" scheme="https://publication-type.data.istex.fr/ark:/67375/JMC-0GLKJH51-B">journal</note></notesStmt><sourceDesc><biblStruct type="article"><analytic><title level="a" type="main">Rational Design of Conjugated Polymer Supramolecules with Tunable Colorimetric Responses</title><author xml:id="author-0000"><persName><forename type="first">Dong June</forename><surname>Ahn</surname></persName><affiliation><orgName type="laboratory">Department of Chemical and Biological Engineering</orgName><orgName type="institution">Korea University Seoul 136‐701 (Korea)</orgName></affiliation></author><author xml:id="author-0001"><persName><forename type="first">Sumi</forename><surname>Lee</surname></persName><affiliation><orgName type="division">Department of Chemical Engineering</orgName><orgName type="institution">Hanyang University Seoul 133‐791 (Korea)</orgName></affiliation></author><author xml:id="author-0002" role="corresp"><persName><forename type="first">Jong‐Man</forename><surname>Kim</surname></persName><email>jmk@hanyang.ac.kr</email><affiliation><orgName type="division">Department of Chemical Engineering</orgName><orgName type="institution">Hanyang University Seoul 133‐791 (Korea)</orgName></affiliation></author><idno type="istex">92AA1CC74CBB4856292C19A7EF4E3EC5FA055170</idno><idno type="ark">ark:/67375/WNG-849J28X3-5</idno><idno type="DOI">10.1002/adfm.200801074</idno><idno type="unit">ADFM200801074</idno><idno type="toTypesetVersion">file:ADFM.ADFM200801074.pdf</idno></analytic><monogr><title level="j" type="main">Advanced Functional Materials</title><title level="j" type="alt">ADVANCED FUNCTIONAL MATERIALS</title><idno type="pISSN">1616-301X</idno><idno type="eISSN">1616-3028</idno><idno type="book-DOI">10.1002/(ISSN)1616-3028</idno><idno type="book-part-DOI">10.1002/adfm.v19:10</idno><idno type="product">ADFM</idno><imprint><biblScope unit="vol">19</biblScope><biblScope unit="issue">10</biblScope><biblScope unit="page" from="1483">1483</biblScope><biblScope unit="page" to="1496">1496</biblScope><biblScope unit="page-count">14</biblScope><publisher>WILEY‐VCH Verlag</publisher><pubPlace>Weinheim</pubPlace><date type="published" when="2009-05-22"></date></imprint></monogr></biblStruct></sourceDesc></fileDesc><encodingDesc><schemaRef type="ODD" url="https://xml-schema.delivery.istex.fr/tei-istex.odd"></schemaRef><appInfo><application ident="pub2tei" version="1.0.10" when="2019-12-20"><label>pub2TEI-ISTEX</label><desc>A set of style sheets for converting XML documents encoded in various scientific publisher formats into a common TEI format.
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KGaA, Weinheim</copyright><eventGroup><event type="manuscriptReceived" date="2008-07-26"></event><event type="manuscriptRevised" date="2008-09-01"></event><event type="firstOnline" date="2008-12-30"></event><event type="publishedOnlineFinalForm" date="2009-05-18"></event><event type="xmlConverted" agent="Converter:JWSART34_TO_WML3G version:2.3.6 mode:FullText source:HeaderRef result:HeaderRef" date="2010-04-14"></event><event type="xmlConverted" agent="Converter:WILEY_ML3G_TO_WILEY_ML3GV2 version:3.8.8" date="2013-12-31"></event><event type="xmlConverted" agent="Converter:WML3G_To_WML3G version:4.1.7 mode:FullText,remove_FC" date="2014-10-14"></event></eventGroup><numberingGroup><numbering type="pageFirst">1483</numbering><numbering type="pageLast">1496</numbering></numberingGroup><correspondenceTo>Department of Chemical Engineering, Hanyang University Seoul 133‐791 (Korea).</correspondenceTo><linkGroup><link type="toTypesetVersion" href="file:ADFM.ADFM200801074.pdf"></link></linkGroup></publicationMeta><contentMeta><countGroup><count type="figureTotal" number="9"></count><count type="tableTotal" number="0"></count><count type="referenceTotal" number="102"></count></countGroup><titleGroup><title type="main" xml:lang="en">Rational Design of Conjugated Polymer Supramolecules with Tunable Colorimetric Responses</title></titleGroup><creators><creator xml:id="au1" creatorRole="author" affiliationRef="#af2"><personName><givenNames>Dong June</givenNames><familyName>Ahn</familyName></personName></creator><creator xml:id="au2" creatorRole="author" affiliationRef="#af1"><personName><givenNames>Sumi</givenNames><familyName>Lee</familyName></personName></creator><creator xml:id="au3" creatorRole="author" affiliationRef="#af1" corresponding="yes"><personName><givenNames>Jong‐Man</givenNames><familyName>Kim</familyName></personName><contactDetails><email>jmk@hanyang.ac.kr</email></contactDetails></creator></creators><affiliationGroup><affiliation xml:id="af1" countryCode="KR" type="organization"><unparsedAffiliation>Department of Chemical Engineering, Hanyang University Seoul 133‐791 (Korea)</unparsedAffiliation></affiliation><affiliation xml:id="af2" countryCode="KR" type="organization"><unparsedAffiliation>Department of Chemical and Biological Engineering, Korea University Seoul 136‐701 (Korea)</unparsedAffiliation></affiliation></affiliationGroup><keywordGroup xml:lang="en" type="author"><keyword xml:id="kwd1">conjugated polymers</keyword><keyword xml:id="kwd2">cyclodextrins</keyword><keyword xml:id="kwd3">Poly(acetylenes)</keyword><keyword xml:id="kwd4">thermochromism</keyword></keywordGroup><abstractGroup><abstract type="main" xml:lang="en"><title type="main">Abstract</title><p>Polydiacetylenes (PDAs), a family of highly π‐conjugated polymers, have unique characteristics associated with their ability to self‐assemble. Disruption of the extensively delocalized enyne backbones of molecularly ordered PDA sidechains induces a blue‐to‐red color change, which has been elegantly applied in the design of chemosensors. Recently, colorimetrically reversible PDAs have received significant attention, not only to gain a better understanding of the fundamentals of PDA chromism, but also to develop methodologies to overcome limitations associated with their colorimetrically irreversible counterparts. In this article, recent progress made in the field of colorimetrically tunable (reversible, stable, or sensitive) PDAs is described. Major emphasis is given to rational design strategies developed in our group. 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Disruption of the extensively delocalized enyne backbones of molecularly ordered PDA sidechains induces a blue‐to‐red color change, which has been elegantly applied in the design of chemosensors. Recently, colorimetrically reversible PDAs have received significant attention, not only to gain a better understanding of the fundamentals of PDA chromism, but also to develop methodologies to overcome limitations associated with their colorimetrically irreversible counterparts. In this article, recent progress made in the field of colorimetrically tunable (reversible, stable, or sensitive) PDAs is described. Major emphasis is given to rational design strategies developed in our group. Relevant mechanistic investigations, a diagnostic method to test colorimetric reversibility, as well as future challenges in this area will be also discussed.</abstract><abstract type="graphical" lang="en">The rational design of thermochromic polydiacetylenes (PDAs) by manipulating strong headgroup interactions, which leads to colorimetrically tunable systems, within the authors' groups is described. In addition, a diagnostic method for assigning colorimetric reversibility to PDAs as well as an analysis of future challenges in this area is also presented.</abstract><subject lang="en"><genre>keywords</genre><topic>conjugated polymers</topic><topic>cyclodextrins</topic><topic>Poly(acetylenes)</topic><topic>thermochromism</topic></subject><relatedItem type="host"><titleInfo><title>Advanced Functional Materials</title></titleInfo><titleInfo type="abbreviated"><title>Adv. Funct. 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