Activation of Molecular Nitrogen: Coordination, Cleavage and Functionalization of N2 Mediated By Metal Complexes
Identifieur interne : 001157 ( Istex/Corpus ); précédent : 001156; suivant : 001158Activation of Molecular Nitrogen: Coordination, Cleavage and Functionalization of N2 Mediated By Metal Complexes
Auteurs : Michael Shaver ; Michael FryzukSource :
- Advanced Synthesis & Catalysis [ 1615-4150 ] ; 2003-09.
Abstract
Recent developments in the activation and reactivity of coordinated dinitrogen are reviewed. Examples of weakly activated dinitrogen metal complexes, strongly reduced nitrogen‐nitrogen bonds and N2 cleavage reactions are discussed. Protonation reactions to form ammonia or hydrazido derivatives are covered along with processes in which nitrogen‐boron, nitrogen‐silicon or nitrogen‐carbon bonds can form. Although this review builds on previous publications, a general introduction to this field is included.
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DOI: 10.1002/adsc.200303081
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ISTEX:4693C79E56DAB165A9EB8ACF29CC541CB5078669Le document en format XML
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Although this review builds on previous publications, a general introduction to this field is included.</p></abstract></abstractGroup></contentMeta></header></component></istex:document></istex:metadataXml><mods version="3.6"><titleInfo lang="en"><title>Activation of Molecular Nitrogen: Coordination, Cleavage and Functionalization of N2 Mediated By Metal Complexes</title></titleInfo><titleInfo type="alternative" contentType="CDATA" lang="en"><title>Activation of Molecular Nitrogen: Coordination, Cleavage and Functionalization of N2 Mediated By Metal Complexes</title></titleInfo><name type="personal"><namePart type="given">Michael P.</namePart><namePart type="family">Shaver</namePart><affiliation>University of British Columbia, 2036 Main Mall, Vancouver, British Columbia, Canada, V6T 1Z1, Fax: (+1)‐604‐822‐2847.</affiliation><affiliation>E-mail: mshaver@chem.ubc.ca</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Michael D.</namePart><namePart type="family">Fryzuk</namePart><affiliation>University of British Columbia, 2036 Main Mall, Vancouver, British Columbia, Canada, V6T 1Z1, Fax: (+1)‐604‐822‐2847.</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="review-article" displayLabel="reviewArticle" authority="ISTEX" authorityURI="https://content-type.data.istex.fr" valueURI="https://content-type.data.istex.fr/ark:/67375/XTP-L5L7X3NF-P">review-article</genre><originInfo><publisher>WILEY‐VCH Verlag</publisher><place><placeTerm type="text">Weinheim</placeTerm></place><dateIssued encoding="w3cdtf">2003-09</dateIssued><dateCaptured encoding="w3cdtf">2003-04-25</dateCaptured><copyrightDate encoding="w3cdtf">2003</copyrightDate></originInfo><language><languageTerm type="code" authority="rfc3066">en</languageTerm><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><physicalDescription><extent unit="figures">0</extent><extent unit="tables">0</extent><extent unit="references">125</extent></physicalDescription><abstract lang="en">Recent developments in the activation and reactivity of coordinated dinitrogen are reviewed. Examples of weakly activated dinitrogen metal complexes, strongly reduced nitrogen‐nitrogen bonds and N2 cleavage reactions are discussed. Protonation reactions to form ammonia or hydrazido derivatives are covered along with processes in which nitrogen‐boron, nitrogen‐silicon or nitrogen‐carbon bonds can form. Although this review builds on previous publications, a general introduction to this field is included.</abstract><subject lang="en"><genre>keywords</genre><topic>activation</topic><topic>coordination modes</topic><topic>dinitrogen</topic><topic>metal complexes</topic><topic>nitrogen fixation</topic><topic>reactivity</topic></subject><relatedItem type="host"><titleInfo><title>Advanced Synthesis & Catalysis</title></titleInfo><titleInfo type="abbreviated"><title>Adv. Synth. 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