Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region
Identifieur interne : 001012 ( Istex/Corpus ); précédent : 001011; suivant : 001013Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region
Auteurs : C. Derognat ; M. Beekmann ; M. Baeumle ; D. Martin ; H. SchmidtSource :
- Journal of Geophysical Research: Atmospheres [ 0148-0227 ] ; 2003-09-16.
Abstract
This paper investigates the impact of biogenic isoprene and terpene emissions on photochemical species levels in the French Ile‐de‐France region during several photooxidant pollution episodes in summer 1998 and 1999 during the Atmospheric Pollution Over the Paris Area (ESQUIF) project. The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by Simpson et al. [1999] and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias <10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NOx‐limited”). However, generally, either with or without biogenic emissions, a “VOC‐limited” regime is simulated over the Ile‐de‐France region.
Url:
DOI: 10.1029/2001JD001421
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Beekmann</name><affiliation><mods:affiliation>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</mods:affiliation></affiliation></author><author><name sortKey="Baeumle, M" sort="Baeumle, M" uniqKey="Baeumle M" first="M." last="Baeumle">M. Baeumle</name><affiliation><mods:affiliation>MetAir AG, Illnau, Switzerland</mods:affiliation></affiliation></author><author><name sortKey="Martin, D" sort="Martin, D" uniqKey="Martin D" first="D." last="Martin">D. Martin</name><affiliation><mods:affiliation>Météo France, Paris, France</mods:affiliation></affiliation></author><author><name sortKey="Schmidt, H" sort="Schmidt, H" uniqKey="Schmidt H" first="H." last="Schmidt">H. 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Derognat</name><affiliation><mods:affiliation>E-mail: derognat@aero.jussieu.fr</mods:affiliation></affiliation><affiliation><mods:affiliation>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</mods:affiliation></affiliation></author><author><name sortKey="Beekmann, M" sort="Beekmann, M" uniqKey="Beekmann M" first="M." last="Beekmann">M. Beekmann</name><affiliation><mods:affiliation>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</mods:affiliation></affiliation></author><author><name sortKey="Baeumle, M" sort="Baeumle, M" uniqKey="Baeumle M" first="M." last="Baeumle">M. Baeumle</name><affiliation><mods:affiliation>MetAir AG, Illnau, Switzerland</mods:affiliation></affiliation></author><author><name sortKey="Martin, D" sort="Martin, D" uniqKey="Martin D" first="D." last="Martin">D. 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Res.</title><idno type="ISSN">0148-0227</idno><idno type="eISSN">2156-2202</idno><imprint><publisher>Blackwell Publishing Ltd</publisher><date type="published" when="2003-09-16">2003-09-16</date><biblScope unit="volume">108</biblScope><biblScope unit="issue">D17</biblScope><biblScope unit="page" from="n/a">n/a</biblScope><biblScope unit="page" to="n/a">n/a</biblScope></imprint><idno type="ISSN">0148-0227</idno></series><idno type="istex">CD7A77D5EA76A5AB2090D2E012A57A2355D0826B</idno><idno type="DOI">10.1029/2001JD001421</idno><idno type="ArticleID">2001JD001421</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0148-0227</idno></seriesStmt></fileDesc><profileDesc><textClass></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract">This paper investigates the impact of biogenic isoprene and terpene emissions on photochemical species levels in the French Ile‐de‐France region during several photooxidant pollution episodes in summer 1998 and 1999 during the Atmospheric Pollution Over the Paris Area (ESQUIF) project. The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by Simpson et al. [1999] and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias <10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NOx‐limited”). However, generally, either with or without biogenic emissions, a “VOC‐limited” regime is simulated over the Ile‐de‐France region.</div></front></TEI><istex><corpusName>wiley</corpusName><author><json:item><name>C. Derognat</name><affiliations><json:string>E-mail: derognat@aero.jussieu.fr</json:string><json:string>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</json:string></affiliations></json:item><json:item><name>M. Beekmann</name><affiliations><json:string>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</json:string></affiliations></json:item><json:item><name>M. Baeumle</name><affiliations><json:string>MetAir AG, Illnau, Switzerland</json:string></affiliations></json:item><json:item><name>D. Martin</name><affiliations><json:string>Météo France, Paris, France</json:string></affiliations></json:item><json:item><name>H. Schmidt</name><affiliations><json:string>Laboratoire de Météorologie Dynamique, Centre National de la Recherche Scientifique, Paris, France</json:string><json:string>Now at Max‐Planck‐Institute for Meteorology, Hamburg, Germany.</json:string></affiliations></json:item></author><language><json:string>eng</json:string></language><abstract>This paper investigates the impact of biogenic isoprene and terpene emissions on photochemical species levels in the French Ile‐de‐France region during several photooxidant pollution episodes in summer 1998 and 1999 during the Atmospheric Pollution Over the Paris Area (ESQUIF) project. The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by Simpson et al. [1999] and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias >10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NOx‐limited”). 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The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by Simpson et al. [1999] and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias <10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NOx‐limited”). However, generally, either with or without biogenic emissions, a “VOC‐limited” regime is simulated over the Ile‐de‐France region.</p></abstract><textClass><keywords scheme="Journal Subject"><list><head>Index Terms</head><item><term>Project: Atmospheric Pollution Over the Paris Area (ESQUIF)</term></item><item><term>Project: Atmospheric Pollution Over the Paris Area</term></item><item><term>Composition and Chemistry</term></item><item><term>ATMOSPHERIC COMPOSITION AND STRUCTURE</term></item><item><term>Pollution: urban and regional</term></item><item><term>Troposphere: composition and chemistry</term></item><item><term>Troposphere: constituent transport and chemistry</term></item><item><term>Constituent sources and sinks</term></item><item><term>Aerosols and particles</term></item><item><term>BIOGEOSCIENCES</term></item><item><term>Pollution: urban, regional and global</term></item><item><term>OCEANOGRAPHY: GENERAL</term></item><item><term>Marine pollution</term></item><item><term>NATURAL HAZARDS</term></item><item><term>Megacities and urban environment</term></item></list></keywords></textClass><textClass><keywords scheme="Journal Subject"><list><head>article category</head><item><term>Composition and Chemistry</term></item></list></keywords></textClass></profileDesc><revisionDesc><change when="2001-10-24">Received</change><change when="2002-08-01">Registration</change><change when="2003-09-16">Published</change></revisionDesc></teiHeader></istex:fulltextTEI><json:item><original>false</original><mimetype>text/plain</mimetype><extension>txt</extension><uri>https://api.istex.fr/document/CD7A77D5EA76A5AB2090D2E012A57A2355D0826B/fulltext/txt</uri></json:item></fulltext><metadata><istex:metadataXml wicri:clean="Wiley, elements deleted: body"><istex:xmlDeclaration>version="1.0" encoding="UTF-8" standalone="yes"</istex:xmlDeclaration><istex:document><component type="serialArticle" version="2.0" xml:lang="en" xml:id="jgrd9446"><header><publicationMeta level="product"><doi>10.1002/(ISSN)2156-2202d</doi><issn type="print">0148-0227</issn><issn type="electronic">2156-2202</issn><idGroup><id type="product" value="JGRD"></id><id type="coden" value="JGREA2"></id></idGroup><titleGroup><title type="main" xml:lang="en" sort="JOURNAL OF GEOPHYSICAL RESEARCH: ATMOSPHERES">Journal of Geophysical Research: Atmospheres</title><title type="short">J. 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Res.</title></titleGroup></publicationMeta><publicationMeta level="part" position="170"><doi>10.1002/jgrd.v108.D17</doi><idGroup><id type="focusSection" value="4"></id></idGroup><titleGroup><title type="focusSection" xml:lang="en">Journal of Geophysical Research: Atmospheres</title></titleGroup><numberingGroup><numbering type="journalVolume" number="108">108</numbering><numbering type="journalIssue">D17</numbering></numberingGroup><coverDate startDate="2003-09-16">16 September 2003</coverDate></publicationMeta><publicationMeta level="unit" position="370" type="article" status="forIssue"><doi>10.1029/2001JD001421</doi><idGroup><id type="editorialOffice" value="2001JD001421"></id><id type="society" value="8560"></id><id type="unit" value="JGRD9446"></id></idGroup><countGroup><count type="pageTotal" number="15"></count></countGroup><titleGroup><title type="articleCategory">Composition and Chemistry</title><title type="tocHeading1">Composition and Chemistry</title></titleGroup><copyright ownership="thirdParty">Copyright 2003 by the American Geophysical Union.</copyright><eventGroup><event type="manuscriptReceived" date="2001-10-24"></event><event type="manuscriptRevised" date="2002-06-17"></event><event type="manuscriptAccepted" date="2002-08-01"></event><event type="firstOnline" date="2003-07-17"></event><event type="publishedOnlineFinalForm" date="2003-07-17"></event><event type="xmlConverted" agent="SPi Global Converter:AGUv3.42_TO_WileyML3Gv1.0.3 version:1.2; WileyML 3G Packaging Tool v1.0; AGU2WileyML3G Final Clean Up v1.0" date="2012-12-17"></event><event type="xmlConverted" agent="Converter:WILEY_ML3G_TO_WILEY_ML3GV2 version:3.8.8" date="2014-01-30"></event><event type="xmlConverted" agent="Converter:WML3G_To_WML3G version:4.1.7 mode:FullText,remove_FC" date="2014-10-30"></event></eventGroup><numberingGroup><numbering type="pageFirst">n/a</numbering><numbering type="pageLast">n/a</numbering></numberingGroup><subjectInfo><subject href="http://psi.agu.org/specialSection/ESQUIF1">Project: Atmospheric Pollution Over the Paris Area (ESQUIF)</subject><subject href="http://psi.agu.org/specialSection/ESQUIF1">Project: Atmospheric Pollution Over the Paris Area</subject><subject href="http://psi.agu.org/subset/ACH">Composition and Chemistry</subject><subject href="http://psi.agu.org/taxonomy5/0300">ATMOSPHERIC COMPOSITION AND STRUCTURE</subject><subjectInfo><subject href="http://psi.agu.org/taxonomy5/0345">Pollution: urban and regional</subject><subject href="http://psi.agu.org/taxonomy5/0365">Troposphere: composition and chemistry</subject><subject href="http://psi.agu.org/taxonomy5/0368">Troposphere: constituent transport and chemistry</subject><subject href="http://psi.agu.org/taxonomy5/0322">Constituent sources and sinks</subject><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/0305">Aerosols and particles</subject></subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/0400">BIOGEOSCIENCES</subject><subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/0478">Pollution: urban, regional and global</subject></subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/4200">OCEANOGRAPHY: GENERAL</subject><subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/4251">Marine pollution</subject></subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/4300">NATURAL HAZARDS</subject><subjectInfo><subject role="crossTerm" href="http://psi.agu.org/taxonomy5/4325">Megacities and urban environment</subject></subjectInfo></subjectInfo><selfCitationGroup><citation xml:id="jgrd9446-cit-0000" type="self"><author><familyName>Derognat</familyName>, <givenNames>C.</givenNames></author>, <author><givenNames>M.</givenNames> <familyName>Beekmann</familyName></author>, <author><givenNames>M.</givenNames> <familyName>Baeumle</familyName></author>, <author><givenNames>D.</givenNames> <familyName>Martin</familyName></author>, and <author><givenNames>H.</givenNames> <familyName>Schmidt</familyName></author> (<pubYear year="2003">2003</pubYear>), <articleTitle>Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region</articleTitle>, <journalTitle>J. Geophys. Res.</journalTitle>, <vol>108</vol>, 8560, doi:<accessionId ref="info:doi/10.1029/2001JD001421">10.1029/2001JD001421</accessionId>, <issue>D17</issue>.</citation></selfCitationGroup><linkGroup><link type="toTypesetVersion" href="file:JGRD.JGRD9446.pdf"></link></linkGroup></publicationMeta><contentMeta><countGroup><count type="figureTotal" number="7"></count><count type="tableTotal" number="5"></count></countGroup><titleGroup><title type="main">Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region</title><title type="short">VOC EMISSIONS IN THE ILE‐DE‐FRANCE REGION</title><title type="shortAuthors">Derognat <i>et al</i>.</title></titleGroup><creators><creator creatorRole="author" xml:id="jgrd9446-cr-0001" affiliationRef="#jgrd9446-aff-0001"><personName><givenNames>C.</givenNames> <familyName>Derognat</familyName></personName><contactDetails><email normalForm="derognat@aero.jussieu.fr">derognat@aero.jussieu.fr</email></contactDetails></creator><creator creatorRole="author" xml:id="jgrd9446-cr-0002" affiliationRef="#jgrd9446-aff-0001"><personName><givenNames>M.</givenNames> <familyName>Beekmann</familyName></personName></creator><creator creatorRole="author" xml:id="jgrd9446-cr-0003" affiliationRef="#jgrd9446-aff-0002"><personName><givenNames>M.</givenNames> <familyName>Baeumle</familyName></personName></creator><creator creatorRole="author" xml:id="jgrd9446-cr-0004" affiliationRef="#jgrd9446-aff-0003"><personName><givenNames>D.</givenNames> <familyName>Martin</familyName></personName></creator><creator creatorRole="author" xml:id="jgrd9446-cr-0005" affiliationRef="#jgrd9446-aff-0004 #jgrd9446-aff-0005"><personName><givenNames>H.</givenNames> <familyName>Schmidt</familyName></personName></creator></creators><affiliationGroup><affiliation countryCode="FR" type="organization" xml:id="jgrd9446-aff-0001"><orgName>Service d'Aeronomie, Centre National de la Recherche Scientifique</orgName><address><city>Paris</city><country>France</country></address></affiliation><affiliation countryCode="CH" type="organization" xml:id="jgrd9446-aff-0002"><orgName>MetAir AG</orgName><address><city>Illnau</city><country>Switzerland</country></address></affiliation><affiliation countryCode="FR" type="organization" xml:id="jgrd9446-aff-0003"><orgName>Météo France</orgName><address><city>Paris</city><country>France</country></address></affiliation><affiliation countryCode="FR" type="organization" xml:id="jgrd9446-aff-0004"><orgDiv>Laboratoire de Météorologie Dynamique</orgDiv><orgName>Centre National de la Recherche Scientifique</orgName><address><city>Paris</city><country>France</country></address></affiliation><affiliation type="organization" xml:id="jgrd9446-aff-0005"><unparsedAffiliation>Now at Max‐Planck‐Institute for Meteorology, Hamburg, Germany.</unparsedAffiliation></affiliation></affiliationGroup><supportingInformation></supportingInformation><abstractGroup><abstract type="main"><p xml:id="jgrd9446-para-0001" label="1">This paper investigates the impact of biogenic isoprene and terpene emissions on photochemical species levels in the French Ile‐de‐France region during several photooxidant pollution episodes in summer 1998 and 1999 during the Atmospheric Pollution Over the Paris Area (ESQUIF) project. The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by <link href="#jgrd9446-bib-0038"><i>Simpson et al.</i> [1999]</link> and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias <10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NO<sub><i>x</i></sub>‐limited”). However, generally, either with or without biogenic emissions, a “VOC‐limited” regime is simulated over the Ile‐de‐France region.</p></abstract></abstractGroup></contentMeta></header></component></istex:document></istex:metadataXml><mods version="3.6"><titleInfo lang="en"><title>Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region</title></titleInfo><titleInfo type="abbreviated"><title>VOC EMISSIONS IN THE ILE‐DE‐FRANCE REGION</title></titleInfo><titleInfo type="alternative" contentType="CDATA" lang="en"><title>Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region</title></titleInfo><name type="personal"><namePart type="given">C.</namePart><namePart type="family">Derognat</namePart><affiliation>E-mail: derognat@aero.jussieu.fr</affiliation><affiliation>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">M.</namePart><namePart type="family">Beekmann</namePart><affiliation>Service d'Aeronomie, Centre National de la Recherche Scientifique, Paris, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">M.</namePart><namePart type="family">Baeumle</namePart><affiliation>MetAir AG, Illnau, Switzerland</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">D.</namePart><namePart type="family">Martin</namePart><affiliation>Météo France, Paris, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">H.</namePart><namePart type="family">Schmidt</namePart><affiliation>Laboratoire de Météorologie Dynamique, Centre National de la Recherche Scientifique, Paris, France</affiliation><affiliation>Now at Max‐Planck‐Institute for Meteorology, Hamburg, Germany.</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="article">article</genre><originInfo><publisher>Blackwell Publishing Ltd</publisher><dateIssued encoding="w3cdtf">2003-09-16</dateIssued><dateCaptured encoding="w3cdtf">2001-10-24</dateCaptured><dateValid encoding="w3cdtf">2002-08-01</dateValid><edition>Derognat, C., M. Beekmann, M. Baeumle, D. Martin, and H. Schmidt (2003), Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area (ESQUIF) campaign in the Ile‐de‐France region, J. Geophys. Res., 108, 8560, doi:10.1029/2001JD001421, D17.</edition><copyrightDate encoding="w3cdtf">2003</copyrightDate></originInfo><language><languageTerm type="code" authority="rfc3066">en</languageTerm><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType><extent unit="figures">7</extent><extent unit="tables">5</extent></physicalDescription><abstract>This paper investigates the impact of biogenic isoprene and terpene emissions on photochemical species levels in the French Ile‐de‐France region during several photooxidant pollution episodes in summer 1998 and 1999 during the Atmospheric Pollution Over the Paris Area (ESQUIF) project. The effect of biogenic emissions on both ozone produced on a continental scale and advected in Ile‐de‐France and on ozone locally formed are assessed. For this purpose, simulations with and without biogenic emissions are performed with a nested version of the CHIMERE model. This chemistry transport model includes both a continental (western European) domain with 0.5° horizontal resolution and a regional domain (Ile‐de‐France) of 150 × 150 km extension with a horizontal resolution of 6 km. An emissions database for biogenic isoprene and terpene emissions from forests has been set up. These emissions are estimated using emission factors for different tree species recently revised by Simpson et al. [1999] and for different land use data sets, including highly resolved (1 km) satellite measurements for Ile‐de‐France. Good agreement has been found between modeled and measured (by aircraft) isoprene levels (overall bias <10%), which lends confidence to the use of the emissions database for subsequent simulations. The comparison between runs with and without biogenic volatile organic compound (VOC) emissions indicates a significant difference in ozone in Ile‐de‐France, up to 40 ppb for one extreme day. Biogenic VOC emissions from Ile‐de‐France along with those from outside the Ile‐de‐France region have an approximately equal responsibility for the additional ozone buildup. The main reason for this increased ozone formation is the enhancement of radicals due to larger concentrations of carbonyl species and ozone and their subsequent photolysis. Biogenic emissions lead to a shift in the sensitivity to emissions (toward more “NOx‐limited”). However, generally, either with or without biogenic emissions, a “VOC‐limited” regime is simulated over the Ile‐de‐France region.</abstract><relatedItem type="host"><titleInfo><title>Journal of Geophysical Research: Atmospheres</title></titleInfo><titleInfo type="abbreviated"><title>J. Geophys. Res.</title></titleInfo><subject><genre>Index Terms</genre><topic authorityURI="http://psi.agu.org/specialSection/ESQUIF1">Project: Atmospheric Pollution Over the Paris Area (ESQUIF)</topic><topic authorityURI="http://psi.agu.org/specialSection/ESQUIF1">Project: Atmospheric Pollution Over the Paris Area</topic><topic authorityURI="http://psi.agu.org/subset/ACH">Composition and Chemistry</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0300">ATMOSPHERIC COMPOSITION AND STRUCTURE</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0345">Pollution: urban and regional</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0365">Troposphere: composition and chemistry</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0368">Troposphere: constituent transport and chemistry</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0322">Constituent sources and sinks</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0305">Aerosols and particles</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0400">BIOGEOSCIENCES</topic><topic authorityURI="http://psi.agu.org/taxonomy5/0478">Pollution: urban, regional and global</topic><topic authorityURI="http://psi.agu.org/taxonomy5/4200">OCEANOGRAPHY: GENERAL</topic><topic authorityURI="http://psi.agu.org/taxonomy5/4251">Marine pollution</topic><topic authorityURI="http://psi.agu.org/taxonomy5/4300">NATURAL HAZARDS</topic><topic authorityURI="http://psi.agu.org/taxonomy5/4325">Megacities and urban environment</topic></subject><subject><genre>article category</genre><topic>Composition and Chemistry</topic></subject><identifier type="ISSN">0148-0227</identifier><identifier type="eISSN">2156-2202</identifier><identifier type="DOI">10.1002/(ISSN)2156-2202d</identifier><identifier type="CODEN">JGREA2</identifier><identifier type="PublisherID">JGRD</identifier><part><date>2003</date><detail type="volume"><caption>vol.</caption><number>108</number></detail><detail type="issue"><caption>no.</caption><number>D17</number></detail><extent unit="pages"><start>n/a</start><end>n/a</end><total>15</total></extent></part></relatedItem><identifier type="istex">CD7A77D5EA76A5AB2090D2E012A57A2355D0826B</identifier><identifier type="DOI">10.1029/2001JD001421</identifier><identifier type="ArticleID">2001JD001421</identifier><accessCondition type="use and reproduction" contentType="copyright">Copyright 2003 by the American Geophysical Union.</accessCondition><recordInfo><recordContentSource>WILEY</recordContentSource></recordInfo></mods></metadata><serie></serie></istex></record>Pour manipuler ce document sous Unix (Dilib)
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