Hydrogen storage properties of B‐ and N‐doped microporous carbon
Identifieur interne : 000275 ( Istex/Corpus ); précédent : 000274; suivant : 000276Hydrogen storage properties of B‐ and N‐doped microporous carbon
Auteurs : Lifeng Wang ; Frances H. Yang ; Ralph T. YangSource :
- AIChE Journal [ 0001-1541 ] ; 2009-07.
English descriptors
- KwdEn :
Abstract
A B‐ and N‐doped microporous carbon has been synthesized via a substitution reaction. The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. Ab initio molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. The theoretical calculations can explain the experimental results well, which also shed light on the most favorable and possible sites with which the spiltover hydrogen atoms bind. © 2009 American Institute of Chemical Engineers AIChE J, 2009
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DOI: 10.1002/aic.11851
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Yang</name><affiliation><mods:affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</mods:affiliation></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">ISTEX</idno><idno type="RBID">ISTEX:321DF89F4A4AFDBEC7E09E63766755A9A44A23F8</idno><date when="2009" year="2009">2009</date><idno type="doi">10.1002/aic.11851</idno><idno type="url">https://api.istex.fr/document/321DF89F4A4AFDBEC7E09E63766755A9A44A23F8/fulltext/pdf</idno><idno type="wicri:Area/Istex/Corpus">000275</idno></publicationStmt><sourceDesc><biblStruct><analytic><title level="a" type="main" xml:lang="en">Hydrogen storage properties of B‐ and N‐doped microporous carbon</title><author><name sortKey="Wang, Lifeng" sort="Wang, Lifeng" uniqKey="Wang L" first="Lifeng" last="Wang">Lifeng Wang</name><affiliation><mods:affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</mods:affiliation></affiliation></author><author><name sortKey="Yang, Frances H" sort="Yang, Frances H" uniqKey="Yang F" first="Frances H." last="Yang">Frances H. Yang</name><affiliation><mods:affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</mods:affiliation></affiliation></author><author><name sortKey="Yang, Ralph T" sort="Yang, Ralph T" uniqKey="Yang R" first="Ralph T." last="Yang">Ralph T. Yang</name><affiliation><mods:affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</mods:affiliation></affiliation></author></analytic><monogr></monogr><series><title level="j">AIChE Journal</title><title level="j" type="abbrev">AIChE J.</title><idno type="ISSN">0001-1541</idno><idno type="eISSN">1547-5905</idno><imprint><publisher>Wiley Subscription Services, Inc., A Wiley Company</publisher><pubPlace>Hoboken</pubPlace><date type="published" when="2009-07">2009-07</date><biblScope unit="volume">55</biblScope><biblScope unit="issue">7</biblScope><biblScope unit="page" from="1823">1823</biblScope><biblScope unit="page" to="1833">1833</biblScope></imprint><idno type="ISSN">0001-1541</idno></series><idno type="istex">321DF89F4A4AFDBEC7E09E63766755A9A44A23F8</idno><idno type="DOI">10.1002/aic.11851</idno><idno type="ArticleID">AIC11851</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0001-1541</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>boron‐ and nitrogen‐doped carbon</term><term>hydrogen binding on carbon</term><term>hydrogen spillover</term><term>hydrogen storage</term><term>microporous carbon</term></keywords></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">A B‐ and N‐doped microporous carbon has been synthesized via a substitution reaction. The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. Ab initio molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. The theoretical calculations can explain the experimental results well, which also shed light on the most favorable and possible sites with which the spiltover hydrogen atoms bind. © 2009 American Institute of Chemical Engineers AIChE J, 2009</div></front></TEI><istex><corpusName>wiley</corpusName><author><json:item><name>Lifeng Wang</name><affiliations><json:string>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</json:string></affiliations></json:item><json:item><name>Frances H. Yang</name><affiliations><json:string>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</json:string></affiliations></json:item><json:item><name>Ralph T. Yang</name><affiliations><json:string>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</json:string></affiliations></json:item></author><subject><json:item><lang><json:string>eng</json:string></lang><value>microporous carbon</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>boron‐ and nitrogen‐doped carbon</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>hydrogen storage</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>hydrogen spillover</value></json:item><json:item><lang><json:string>eng</json:string></lang><value>hydrogen binding on carbon</value></json:item></subject><language><json:string>eng</json:string></language><abstract>A B‐ and N‐doped microporous carbon has been synthesized via a substitution reaction. The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. Ab initio molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. 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The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. Ab initio molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. 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T.</givenNames><familyName>Yang</familyName></personName><contactDetails><email>yang@umich.edu</email></contactDetails></creator></creators><affiliationGroup><affiliation xml:id="af1" countryCode="US" type="organization"><unparsedAffiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</unparsedAffiliation></affiliation></affiliationGroup><keywordGroup xml:lang="en" type="author"><keyword xml:id="kwd1">microporous carbon</keyword><keyword xml:id="kwd2">boron‐ and nitrogen‐doped carbon</keyword><keyword xml:id="kwd3">hydrogen storage</keyword><keyword xml:id="kwd4">hydrogen spillover</keyword><keyword xml:id="kwd5">hydrogen binding on carbon</keyword></keywordGroup><fundingInfo><fundingAgency>US Department of Energy's Office of Energy Efficiency and Renewable Energy</fundingAgency></fundingInfo><fundingInfo><fundingAgency>Hydrogen Sorption Center of Excellence (HS CoE)</fundingAgency></fundingInfo><fundingInfo><fundingAgency>NSF</fundingAgency></fundingInfo><supportingInformation><p> Additional Supporting Information may be found in the online version of this article. </p><supportingInfoItem><mediaResource alt="supporting information" href="urn-x:wiley:00011541:media:aic11851:aic_11851_sm_Suppinfo"></mediaResource><caption>Supplementary Material</caption></supportingInfoItem></supportingInformation><abstractGroup><abstract type="main" xml:lang="en"><title type="main">Abstract</title><p>A B‐ and N‐doped microporous carbon has been synthesized via a substitution reaction. The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. <i>Ab initio</i> molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. The theoretical calculations can explain the experimental results well, which also shed light on the most favorable and possible sites with which the spiltover hydrogen atoms bind. © 2009 American Institute of Chemical Engineers AIChE J, 2009</p></abstract></abstractGroup></contentMeta></header></component></istex:document></istex:metadataXml><mods version="3.6"><titleInfo lang="en"><title>Hydrogen storage properties of B‐ and N‐doped microporous carbon</title></titleInfo><titleInfo type="alternative" contentType="CDATA" lang="en"><title>Hydrogen storage properties of B‐ and N‐doped microporous carbon</title></titleInfo><name type="personal"><namePart type="given">Lifeng</namePart><namePart type="family">Wang</namePart><affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Frances H.</namePart><namePart type="family">Yang</namePart><affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">Ralph T.</namePart><namePart type="family">Yang</namePart><affiliation>Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</affiliation><description>Correspondence: Dept. of Chemical Engineering, University of Michigan, Ann Arbor, MI 48109</description><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="article" displayLabel="article"></genre><originInfo><publisher>Wiley Subscription Services, Inc., A Wiley Company</publisher><place><placeTerm type="text">Hoboken</placeTerm></place><dateIssued encoding="w3cdtf">2009-07</dateIssued><dateCaptured encoding="w3cdtf">2008-08-04</dateCaptured><copyrightDate encoding="w3cdtf">2009</copyrightDate></originInfo><language><languageTerm type="code" authority="rfc3066">en</languageTerm><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType><extent unit="figures">16</extent><extent unit="tables">5</extent><extent unit="references">72</extent><extent unit="words">7727</extent></physicalDescription><abstract lang="en">A B‐ and N‐doped microporous carbon has been synthesized via a substitution reaction. The obtained carbon exhibited much higher surface area than the previously reported B‐ and N‐doped carbon. The hydrogen storage measurements indicated that the B‐ and N‐doped microporous carbon had a 53% higher storage capacity than the carbon materials with similar surface areas. Furthermore, hydrogen storage via spillover was studied on Ru‐supported B‐ and N‐doped microporous carbon and a storage capacity of 1.2 wt % at 298 K and 10 MPa was obtained, showing an enhancement factor of 2.2. Ab initio molecular orbital calculations were also performed for the binding energies between the spiltover hydrogen atom and various sites on the doped carbon. The theoretical calculations can explain the experimental results well, which also shed light on the most favorable and possible sites with which the spiltover hydrogen atoms bind. © 2009 American Institute of Chemical Engineers AIChE J, 2009</abstract><note type="funding">US Department of Energy's Office of Energy Efficiency and Renewable Energy</note><note type="funding">Hydrogen Sorption Center of Excellence (HS CoE)</note><note type="funding">NSF</note><subject lang="en"><genre>Keywords</genre><topic>microporous carbon</topic><topic>boron‐ and nitrogen‐doped carbon</topic><topic>hydrogen storage</topic><topic>hydrogen spillover</topic><topic>hydrogen binding on carbon</topic></subject><relatedItem type="host"><titleInfo><title>AIChE Journal</title></titleInfo><titleInfo type="abbreviated"><title>AIChE J.</title></titleInfo><genre type="Journal">journal</genre><note type="content"> Additional Supporting Information may be found in the online version of this article.Supporting Info Item: Supplementary Material - </note><subject><genre>article category</genre><topic>Materials, Interfaces, and Electrochemical Phenomena</topic></subject><identifier type="ISSN">0001-1541</identifier><identifier type="eISSN">1547-5905</identifier><identifier type="DOI">10.1002/(ISSN)1547-5905</identifier><identifier type="PublisherID">AIC</identifier><part><date>2009</date><detail type="volume"><caption>vol.</caption><number>55</number></detail><detail type="issue"><caption>no.</caption><number>7</number></detail><extent unit="pages"><start>1823</start><end>1833</end><total>11</total></extent></part></relatedItem><identifier type="istex">321DF89F4A4AFDBEC7E09E63766755A9A44A23F8</identifier><identifier type="DOI">10.1002/aic.11851</identifier><identifier type="ArticleID">AIC11851</identifier><accessCondition type="use and reproduction" contentType="copyright">Copyright © 2009 American Institute of Chemical Engineers (AIChE)</accessCondition><recordInfo><recordContentSource>WILEY</recordContentSource><recordOrigin>Wiley Subscription Services, Inc., A Wiley Company</recordOrigin></recordInfo></mods></metadata><serie></serie></istex></record>Pour manipuler ce document sous Unix (Dilib)
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