Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France) : Transport and fate of PAHs from the atmosphere to the outlet
Identifieur interne : 000200 ( PascalFrancis/Checkpoint ); précédent : 000199; suivant : 000201Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France) : Transport and fate of PAHs from the atmosphere to the outlet
Auteurs : A. Motelay-Massei [France] ; B. Garban [France] ; K. Tiphagne-Larcher [France] ; M. Chevreuil [France] ; D. Ollivon [France]Source :
- Water research : (Oxford) [ 0043-1354 ] ; 2006.
Descripteurs français
- Pascal (Inist)
- Wicri :
- geographic : France.
- topic : Hydrocarbure, Zone urbaine.
English descriptors
- KwdEn :
Abstract
Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kg km-2yr-1 while PAH atmospheric deposition was 0.21 kg km-2yr-1. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air-water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).
Affiliations:
- France
- Haute-Normandie, Région Normandie, Île-de-France
- Mont-Saint-Aignan, Paris
- Université de Rouen
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Motelay-Massei</name><affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Département de Géologie, UMR CNRS 6143, Faculté des Sciences et Techniques, Université de Rouen, 10 Boulevard de Broglie</s1><s2>76821 Mont-Saint-Aignan</s2><s3>FRA</s3><sZ>1 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Région Normandie</region><region type="old region" nuts="2">Haute-Normandie</region><settlement type="city">Mont-Saint-Aignan</settlement></placeName><orgName type="university">Université de Rouen</orgName></affiliation></author><author><name sortKey="Garban, B" sort="Garban, B" uniqKey="Garban B" first="B." last="Garban">B. Garban</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Laboratoire Hydrologie et Environnement, Ecole Pratique des Hautes Etudes, UMR Sisyphe 7619,Uniuersité Pierre et Marie Curie, 4 place Jussieu, case 105</s1><s2>75252 Paris</s2><s3>FRA</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Île-de-France</region><settlement type="city">Paris</settlement></placeName></affiliation></author><author><name sortKey="Tiphagne Larcher, K" sort="Tiphagne Larcher, K" uniqKey="Tiphagne Larcher K" first="K." last="Tiphagne-Larcher">K. Tiphagne-Larcher</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Laboratoire Hydrologie et Environnement, Ecole Pratique des Hautes Etudes, UMR Sisyphe 7619,Uniuersité Pierre et Marie Curie, 4 place Jussieu, case 105</s1><s2>75252 Paris</s2><s3>FRA</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Île-de-France</region><settlement type="city">Paris</settlement></placeName></affiliation></author><author><name sortKey="Chevreuil, M" sort="Chevreuil, M" uniqKey="Chevreuil M" first="M." last="Chevreuil">M. Chevreuil</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Laboratoire Hydrologie et Environnement, Ecole Pratique des Hautes Etudes, UMR Sisyphe 7619,Uniuersité Pierre et Marie Curie, 4 place Jussieu, case 105</s1><s2>75252 Paris</s2><s3>FRA</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Île-de-France</region><settlement type="city">Paris</settlement></placeName></affiliation></author><author><name sortKey="Ollivon, D" sort="Ollivon, D" uniqKey="Ollivon D" first="D." last="Ollivon">D. Ollivon</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Laboratoire Hydrologie et Environnement, Ecole Pratique des Hautes Etudes, UMR Sisyphe 7619,Uniuersité Pierre et Marie Curie, 4 place Jussieu, case 105</s1><s2>75252 Paris</s2><s3>FRA</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Île-de-France</region><settlement type="city">Paris</settlement></placeName></affiliation></author></analytic><series><title level="j" type="main">Water research : (Oxford)</title><title level="j" type="abbreviated">Water res. : (Oxf.)</title><idno type="ISSN">0043-1354</idno><imprint><date when="2006">2006</date></imprint></series></biblStruct></sourceDesc><seriesStmt><title level="j" type="main">Water research : (Oxford)</title><title level="j" type="abbreviated">Water res. : (Oxf.)</title><idno type="ISSN">0043-1354</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Air pollution</term><term>Atmospheric fallout</term><term>France</term><term>Hydrocarbon</term><term>Material balance</term><term>Pollutant behavior</term><term>Polycyclic aromatic compound</term><term>Runoff water</term><term>Stream</term><term>Street</term><term>Surface water</term><term>Surveillance</term><term>Transport process</term><term>Urban area</term><term>Watershed</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Bilan matière</term><term>Composé aromatique polycyclique</term><term>Hydrocarbure</term><term>Zone urbaine</term><term>Bassin versant</term><term>Phénomène transport</term><term>Surveillance</term><term>Pollution air</term><term>Retombée atmosphérique</term><term>Eau ruissellement</term><term>Cours eau</term><term>Rue</term><term>Eau surface</term><term>France</term><term>Devenir polluant</term></keywords><keywords scheme="Wicri" type="geographic" xml:lang="fr"><term>France</term></keywords><keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Hydrocarbure</term><term>Zone urbaine</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kg km<sup>-2</sup>yr<sup>-1</sup> while PAH atmospheric deposition was 0.21 kg km<sup>-2</sup>yr<sup>-1</sup>. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air-water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0043-1354</s0></fA01><fA02 i1="01"><s0>WATRAG</s0></fA02><fA03 i2="1"><s0>Water res. : (Oxf.)</s0></fA03><fA05><s2>40</s2></fA05><fA06><s2>10</s2></fA06><fA08 i1="01" i2="1" l="ENG"><s1>Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France) : Transport and fate of PAHs from the atmosphere to the outlet</s1></fA08><fA11 i1="01" i2="1"><s1>MOTELAY-MASSEI (A.)</s1></fA11><fA11 i1="02" i2="1"><s1>GARBAN (B.)</s1></fA11><fA11 i1="03" i2="1"><s1>TIPHAGNE-LARCHER (K.)</s1></fA11><fA11 i1="04" i2="1"><s1>CHEVREUIL (M.)</s1></fA11><fA11 i1="05" i2="1"><s1>OLLIVON (D.)</s1></fA11><fA14 i1="01"><s1>Département de Géologie, UMR CNRS 6143, Faculté des Sciences et Techniques, Université de Rouen, 10 Boulevard de Broglie</s1><s2>76821 Mont-Saint-Aignan</s2><s3>FRA</s3><sZ>1 aut.</sZ></fA14><fA14 i1="02"><s1>Laboratoire Hydrologie et Environnement, Ecole Pratique des Hautes Etudes, UMR Sisyphe 7619,Uniuersité Pierre et Marie Curie, 4 place Jussieu, case 105</s1><s2>75252 Paris</s2><s3>FRA</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ></fA14><fA20><s1>1995-2006</s1></fA20><fA21><s1>2006</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>8940A</s2><s5>354000142583300080</s5></fA43><fA44><s0>0000</s0><s1>© 2006 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>1 p.1/4</s0></fA45><fA47 i1="01" i2="1"><s0>06-0325876</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Water research : (Oxford)</s0></fA64><fA66 i1="01"><s0>GBR</s0></fA66><fC01 i1="01" l="ENG"><s0>Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kg km<sup>-2</sup>yr<sup>-1</sup> while PAH atmospheric deposition was 0.21 kg km<sup>-2</sup>yr<sup>-1</sup>. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. 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Motelay-Massei</name></region><name sortKey="Chevreuil, M" sort="Chevreuil, M" uniqKey="Chevreuil M" first="M." last="Chevreuil">M. Chevreuil</name><name sortKey="Garban, B" sort="Garban, B" uniqKey="Garban B" first="B." last="Garban">B. Garban</name><name sortKey="Ollivon, D" sort="Ollivon, D" uniqKey="Ollivon D" first="D." last="Ollivon">D. Ollivon</name><name sortKey="Tiphagne Larcher, K" sort="Tiphagne Larcher, K" uniqKey="Tiphagne Larcher K" first="K." last="Tiphagne-Larcher">K. Tiphagne-Larcher</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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