N‐Acyliminium Ion Chemistry: Highly Efficient and Versatile Carbon–Carbon Bond Formation by Nucleophilic Substitution of Hydroxy Groups Catalyzed by Sn(NTf2)4
Identifieur interne : 000479 ( Istex/Curation ); précédent : 000478; suivant : 000480N‐Acyliminium Ion Chemistry: Highly Efficient and Versatile Carbon–Carbon Bond Formation by Nucleophilic Substitution of Hydroxy Groups Catalyzed by Sn(NTf2)4
Auteurs : Raja Ben Thman [Tunisie] ; Radouane Affani ; Marie-José Tranchant ; Sylvain Antoniotti ; Vincent Dalla [France] ; Elisabet Du Ach [France]Source :
- Angewandte Chemie [ 0044-8249 ] ; 2010-01-18.
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Abstract
Atomökonomisch: Nichtmodifizierte N,O‐Halbacetale wurden in einer katalytischen, hocheffizienten α‐Amidoalkylierung kohlenstoffzentrierter Nucleophile eingesetzt, darunter Siliciumverbindungen, aktive Methylenderivate, elektronenreiche Arene und selbst einfache Ketone (siehe Schema). In der Regel genügt 1 Mol‐% des supersauren Lewis‐Reagens Sn(NTf2)4 als Katalysator.
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DOI: 10.1002/ange.200906036
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Radouane Affani<affiliation><mods:affiliation>URCOM, EA 3221, FR 3038, Faculté des Sciences et Techniques de l'Université du Havre, 25, Rue Philippe Lebon, BP 540, 76058 Le Havre (France), Fax: (+33) 2‐3274‐4391</mods:affiliation>
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<affiliation><mods:affiliation>URCOM, EA 3221, FR 3038, Faculté des Sciences et Techniques de l'Université du Havre, 25, Rue Philippe Lebon, BP 540, 76058 Le Havre (France), Fax: (+33) 2‐3274‐4391</mods:affiliation>
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<affiliation><mods:affiliation>LCMBA. UMR 6001, Université de Nice‐Sophia Antipolis, C.N.R.S. Institut de Chimie de Nice, 28, avenue de Valrose, 06108 Nice (France), Fax: (+33) 4‐9207‐6125</mods:affiliation>
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Le document en format XML
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<front><div type="abstract">Atomökonomisch: Nichtmodifizierte N,O‐Halbacetale wurden in einer katalytischen, hocheffizienten α‐Amidoalkylierung kohlenstoffzentrierter Nucleophile eingesetzt, darunter Siliciumverbindungen, aktive Methylenderivate, elektronenreiche Arene und selbst einfache Ketone (siehe Schema). In der Regel genügt 1 Mol‐% des supersauren Lewis‐Reagens Sn(NTf2)4 als Katalysator.</div>
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