Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): Transport and fate of PAHs from the atmosphere to the outlet
Identifieur interne : 000214 ( Hal/Curation ); précédent : 000213; suivant : 000215Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): Transport and fate of PAHs from the atmosphere to the outlet
Auteurs : A. Motelay-Massei [France] ; Brigitte Garban [France] ; Karen Tiphagne-Larcher [France] ; Marc Chevreuil [France] ; Donatienne Ollivon [France]Source :
English descriptors
Abstract
Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kgkm-2 yr-1 while PAH atmospheric deposition was 0.21 kgkm-2 yr-1. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air–water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).
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DOI: 10.1016/j.watres.2006.03.015
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PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kgkm-2 yr-1 while PAH atmospheric deposition was 0.21 kgkm-2 yr-1. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air–water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).</div></front></TEI><hal api="V3"><titleStmt><title xml:lang="en">Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): Transport and fate of PAHs from the atmosphere to the outlet</title><author role="aut"><persName><forename type="first">A.</forename><surname>Motelay-Massei</surname></persName><email>anne.motelay-massei@univ-rouen.fr</email><idno type="halauthor">357505</idno><affiliation ref="#struct-847"></affiliation></author><author role="aut"><persName><forename type="first">Brigitte</forename><surname>Garban</surname></persName><email></email><idno type="halauthor">240319</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Karen</forename><surname>Tiphagne-Larcher</surname></persName><email></email><idno type="halauthor">240320</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Marc</forename><surname>Chevreuil</surname></persName><email></email><idno type="halauthor">240322</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Donatienne</forename><surname>Ollivon</surname></persName><email></email><idno type="halauthor">240318</idno><affiliation ref="#struct-142101"></affiliation></author><editor role="depositor"><persName><forename>Valérie</forename><surname>Casado-Malaizé</surname></persName><email>valerie.casado-malaize@unicaen.fr</email></editor></titleStmt><editionStmt><edition n="v1" type="current"><date type="whenSubmitted">2008-10-07 14:56:05</date><date type="whenModified">2016-09-29 01:21:20</date><date type="whenReleased">2008-10-07 14:56:05</date><date type="whenProduced">2006-03-21</date></edition><respStmt><resp>contributor</resp><name key="113231"><persName><forename>Valérie</forename><surname>Casado-Malaizé</surname></persName><email>valerie.casado-malaize@unicaen.fr</email></name></respStmt></editionStmt><publicationStmt><distributor>CCSD</distributor><idno type="halId">hal-00327144</idno><idno type="halUri">https://hal.archives-ouvertes.fr/hal-00327144</idno><idno type="halBibtex">motelaymassei:hal-00327144</idno><idno type="halRefHtml">WATER RESE ARCH, 2006, 40, pp.1995 - 2006. <10.1016/j.watres.2006.03.015></idno><idno type="halRef">WATER RESE ARCH, 2006, 40, pp.1995 - 2006. <10.1016/j.watres.2006.03.015></idno></publicationStmt><seriesStmt><idno type="stamp" n="CNRS">CNRS - Centre national de la recherche scientifique</idno><idno type="stamp" n="UNIV-ROUEN">Université de Rouen</idno><idno type="stamp" n="UNIV-CAEN">Université de Caen</idno><idno type="stamp" n="INSU">INSU - Institut National des Sciences de l'Univers</idno><idno type="stamp" n="ENSMP" p="PARISTECH">MINES ParisTech</idno><idno type="stamp" n="PARISTECH">ParisTech</idno><idno type="stamp" n="GIP-BE">GIP Bretagne Environnement</idno><idno type="stamp" n="INSTITUT-TELECOM">Institut Télécom</idno><idno type="stamp" n="METIS_UMR7619" p="UPMC">Milieux Environnementaux, Transferts et Interactions dans les hydrosystèmes et les Sols</idno><idno type="stamp" n="UPMC">Université Pierre et Marie Curie</idno><idno type="stamp" n="UMR6143M2C">productions UMR 6143</idno><idno type="stamp" n="EPHE">Ecole Pratique des Hautes Etudes</idno><idno type="stamp" n="PSL">Paris Sciences et Lettres (PSL) Research University</idno><idno type="stamp" n="COMUE-NORMANDIE">Normandie Université</idno></seriesStmt><notesStmt><note type="audience" n="2">International</note><note type="popular" n="0">No</note><note type="peer" n="1">Yes</note></notesStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): Transport and fate of PAHs from the atmosphere to the outlet</title><author role="aut"><persName><forename type="first">A.</forename><surname>Motelay-Massei</surname></persName><email>anne.motelay-massei@univ-rouen.fr</email><idno type="halAuthorId">357505</idno><affiliation ref="#struct-847"></affiliation></author><author role="aut"><persName><forename type="first">Brigitte</forename><surname>Garban</surname></persName><idno type="halAuthorId">240319</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Karen</forename><surname>Tiphagne-Larcher</surname></persName><idno type="halAuthorId">240320</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Marc</forename><surname>Chevreuil</surname></persName><idno type="halAuthorId">240322</idno><affiliation ref="#struct-142101"></affiliation></author><author role="aut"><persName><forename type="first">Donatienne</forename><surname>Ollivon</surname></persName><idno type="halAuthorId">240318</idno><affiliation ref="#struct-142101"></affiliation></author></analytic><monogr><idno type="halJournalId" status="INCOMING">51210</idno><title level="j">WATER RESE ARCH</title><imprint><biblScope unit="volume">40</biblScope><biblScope unit="pp">1995 – 2006</biblScope><date type="datePub">2006-03-21</date></imprint></monogr><idno type="doi">10.1016/j.watres.2006.03.015</idno></biblStruct></sourceDesc><profileDesc><langUsage><language ident="en">English</language></langUsage><textClass><keywords scheme="author"><term xml:lang="en">PAHs Urban watershed Atmospheric deposition Runoff Mass balance</term></keywords><classCode scheme="halDomain" n="sdu.envi">Sciences of the Universe [physics]/Continental interfaces, environment</classCode><classCode scheme="halTypology" n="ART">Journal articles</classCode></textClass><abstract xml:lang="en">Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kgkm-2 yr-1 while PAH atmospheric deposition was 0.21 kgkm-2 yr-1. The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air–water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).</abstract></profileDesc></hal></record>Pour manipuler ce document sous Unix (Dilib)
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