LrgpV1, PascalFrancis, Curation, bibRecord, 000998

Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading

Identifieur interne : 000998 ( PascalFrancis/Curation ); précédent : 000997; suivant : 000999

Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading

Auteurs : Adele Brunetti [Italie] ; Alessio Caravella [Italie, Japon] ; Enrico Drioli [Italie] ; Giuseppe Barbieri [Italie]

Source :

Chemical engineering & technology [ 0930-7516 ] ; 2012.

RBID : Pascal:12-0330320

Descripteurs français

Pascal (Inist)
- Réacteur membrane, Gaz à l'eau, Gaz synthèse, Valorisation, Extrait, Echangeur chaleur, Opération unitaire.

English descriptors

KwdEn :
- Extract, Heat exchanger, Membrane reactor, Synthesis gas, Unit operation, Upgrading, Water gas.

Abstract

Pd-based membrane reactors (MRs) selectively removing hydrogen shift the equilibrium conversion of this new reactor type to values higher than those imposed by thermodynamics to traditional reactors. Thus, the equilibrium conversion of CO is significantly increased and can be very strongly depending on the hydrogen extracted also at a higher temperature. This property of the MRs offers important benefits also in terms of process intensification. In the typical high-temperature range for this reaction, i.e., 300-450 °C, the performance of an MR turned out to be so effective that the two reactors of a traditional process can be replaced by one MR of lower volume, too. The conversion of the MR is higher than the one of the whole traditional process which includes a heat exchanger in addition to two reactors. Consequently, less and smaller unit operations are required when an MR operates the water gas shift reaction pursuing the process intensification philosophy.

A01	`01`	`1`		`@0 0930-7516`
A02	`01`			`@0 CETEER`
A03		`1`		`@0 Chem. eng. technol.`
A05				`@2 35`
A06				`@2 7`
A08	`01`	`1`	`ENG`	`@1 Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading`
A09	`01`	`1`	`ENG`	`@1 Reactor Design & Process Intensification`
A11	`01`	`1`		`@1 BRUNETTI (Adele)`
A11	`02`	`1`		`@1 CARAVELLA (Alessio)`
A11	`03`	`1`		`@1 DRIOLI (Enrico)`
A11	`04`	`1`		`@1 BARBIERI (Giuseppe)`
A12	`01`	`1`		`@1 CHARPENTIER (Jean-Claude) @9 ed.`
A14	`01`			`@1 National Research Council, Institute for Membrane Technology (ITM-CNR) @2 Rende @3 ITA @Z 1 aut. @Z 2 aut. @Z 3 aut. @Z 4 aut.`
A14	`02`			`@1 The University of Calabria, Department of Chemical Engineering and Materials @2 Rende @3 ITA @Z 3 aut.`
A14	`03`			`@1 Present address: National Institute of Advanced Industrial Science and Technology (AIST), Research Institute for Innovation in Sustainable Chemistry @2 Tsukuba (Ibaraki) @3 JPN @Z 2 aut.`
A15	`01`			`@1 Laboratoire Réactions et Génie des Procédés, CNRS/ENSIC Université de Lorraine @2 Nancy @3 FRA @Z 1 aut.`
A20				`@1 1238-1248`
A21				`@1 2012`
A23	`01`			`@0 ENG`
A43	`01`			`@1 INIST @2 20728 @5 354000500864540110`
A44				`@0 0000 @1 © 2012 INIST-CNRS. All rights reserved.`
A45				`@0 39 ref.`
A47	`01`	`1`		`@0 12-0330320`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Chemical engineering & technology`
A66	`01`			`@0 DEU`
C01	`01`		`ENG`	@0 Pd-based membrane reactors (MRs) selectively removing hydrogen shift the equilibrium conversion of this new reactor type to values higher than those imposed by thermodynamics to traditional reactors. Thus, the equilibrium conversion of CO is significantly increased and can be very strongly depending on the hydrogen extracted also at a higher temperature. This property of the MRs offers important benefits also in terms of process intensification. In the typical high-temperature range for this reaction, i.e., 300-450 °C, the performance of an MR turned out to be so effective that the two reactors of a traditional process can be replaced by one MR of lower volume, too. The conversion of the MR is higher than the one of the whole traditional process which includes a heat exchanger in addition to two reactors. Consequently, less and smaller unit operations are required when an MR operates the water gas shift reaction pursuing the process intensification philosophy.
C02	`01`	`X`		`@0 001D07H`
C02	`02`	`X`		`@0 001D07S`
C03	`01`	`X`	`FRE`	`@0 Réacteur membrane @5 01`
C03	`01`	`X`	`ENG`	`@0 Membrane reactor @5 01`
C03	`01`	`X`	`SPA`	`@0 Reactor membrana @5 01`
C03	`02`	`X`	`FRE`	`@0 Gaz à l'eau @5 02`
C03	`02`	`X`	`ENG`	`@0 Water gas @5 02`
C03	`02`	`X`	`SPA`	`@0 Gas con agua @5 02`
C03	`03`	`X`	`FRE`	`@0 Gaz synthèse @5 03`
C03	`03`	`X`	`ENG`	`@0 Synthesis gas @5 03`
C03	`03`	`X`	`SPA`	`@0 Gas síntesis @5 03`
C03	`04`	`X`	`FRE`	`@0 Valorisation @5 04`
C03	`04`	`X`	`ENG`	`@0 Upgrading @5 04`
C03	`04`	`X`	`SPA`	`@0 Valorización @5 04`
C03	`05`	`X`	`FRE`	`@0 Extrait @5 05`
C03	`05`	`X`	`ENG`	`@0 Extract @5 05`
C03	`05`	`X`	`SPA`	`@0 Extracto @5 05`
C03	`06`	`X`	`FRE`	`@0 Echangeur chaleur @5 06`
C03	`06`	`X`	`ENG`	`@0 Heat exchanger @5 06`
C03	`06`	`X`	`SPA`	`@0 Intercambiador calor @5 06`
C03	`07`	`X`	`FRE`	`@0 Opération unitaire @5 07`
C03	`07`	`X`	`ENG`	`@0 Unit operation @5 07`
C03	`07`	`X`	`SPA`	`@0 Operación unitaria @5 07`
N21				`@1 254`
N44	`01`			`@1 OTO`
N82				`@1 OTO`

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Pascal:12-0330320

Le document en format XML

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<author><name sortKey="Caravella, Alessio" sort="Caravella, Alessio" uniqKey="Caravella A" first="Alessio" last="Caravella">Alessio Caravella</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>National Research Council, Institute for Membrane Technology (ITM-CNR)</s1>
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<s3>ITA</s3>
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<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Present address: National Institute of Advanced Industrial Science and Technology (AIST), Research Institute for Innovation in Sustainable Chemistry</s1>
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<series><title level="j" type="main">Chemical engineering & technology</title>
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<front><div type="abstract" xml:lang="en">Pd-based membrane reactors (MRs) selectively removing hydrogen shift the equilibrium conversion of this new reactor type to values higher than those imposed by thermodynamics to traditional reactors. Thus, the equilibrium conversion of CO is significantly increased and can be very strongly depending on the hydrogen extracted also at a higher temperature. This property of the MRs offers important benefits also in terms of process intensification. In the typical high-temperature range for this reaction, i.e., 300-450 °C, the performance of an MR turned out to be so effective that the two reactors of a traditional process can be replaced by one MR of lower volume, too. The conversion of the MR is higher than the one of the whole traditional process which includes a heat exchanger in addition to two reactors. Consequently, less and smaller unit operations are required when an MR operates the water gas shift reaction pursuing the process intensification philosophy.</div>
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<fC01 i1="01" l="ENG"><s0>Pd-based membrane reactors (MRs) selectively removing hydrogen shift the equilibrium conversion of this new reactor type to values higher than those imposed by thermodynamics to traditional reactors. Thus, the equilibrium conversion of CO is significantly increased and can be very strongly depending on the hydrogen extracted also at a higher temperature. This property of the MRs offers important benefits also in terms of process intensification. In the typical high-temperature range for this reaction, i.e., 300-450 °C, the performance of an MR turned out to be so effective that the two reactors of a traditional process can be replaced by one MR of lower volume, too. The conversion of the MR is higher than the one of the whole traditional process which includes a heat exchanger in addition to two reactors. Consequently, less and smaller unit operations are required when an MR operates the water gas shift reaction pursuing the process intensification philosophy.</s0>
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Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading

Process Intensification by Membrane Reactors: High-Temperature Water Gas Shift Reaction as Single Stage for Syngas Upgrading

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Descripteurs français

English descriptors

Abstract

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Le document en format XML

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