LrgpV1, Main, Exploration, bibRecord, 000752

Steam methane reforming reaction process intensification by using a millistructured reactor: Experimental setup and model validation for global kinetic reaction rate estimation

Identifieur interne : 000752 ( Main/Exploration ); précédent : 000751; suivant : 000753

Steam methane reforming reaction process intensification by using a millistructured reactor: Experimental setup and model validation for global kinetic reaction rate estimation

Auteurs : Mamadou Mbodji [France] ; Jean-Marc Commenge [France] ; Laurent Falk [France] ; Damien Di Marco [France] ; Fabrice Rossignol [France] ; L. Prost [France] ; S. Valentin [France] ; R. Joly [France] ; P. Del-Gallo [France]

Source :

Chemical Engineering Journal [ 1385-8947 ] ; 2012-10-01.

RBID : Hal:hal-00777216

Descripteurs français

Wicri :
- topic : Hydrogène.

English descriptors

mix :
- Hydrogen, Kinetic data acquisition, Methane reforming, Microreactor modeling, Microstructured reactor, Process intensification, Syngas.

Abstract

In the frame of steam methane reforming process intensification, a highly active and stable catalyst based on rhodium with catalyst formulation and structure adapted to millistructured reactors has been formulated. This catalyst has been tested in industrial conditions (800, 850 or 900 degrees C and 20 bars) on a single channel which is representative of one channel of a more complex millistructured SMR reactor. Then, a detailed mathematical model for acquisition of the global reaction kinetics with this new catalyst has been developed and validated from experimental catalytic tests. The developed kinetics is dependent of the catalyst microstructure. This study presents the set-up, the model, the experimental catalytic runs and the global kinetics estimation protocol. It demonstrates, on one hand, that millistructured reactor is suitable for kinetic data acquisition and, on the other hand, the possibility of SMR process intensification, for improved energy efficiency and process size reduction.

Url:

https://hal.archives-ouvertes.fr/hal-00777216

DOI: 10.1016/j.cej.2012.07.117

Affiliations:

Links toward previous steps (curation, corpus...)

to stream Hal, to step Corpus: 000A68
to stream Hal, to step Curation: 000A68
to stream Hal, to step Checkpoint: 000696
to stream Main, to step Merge: 000809
to stream Main, to step Curation: 000752

Le document en format XML

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<idno type="DOI">10.1016/j.cej.2012.07.117</idno>
<series><title level="j">Chemical Engineering Journal</title>
<idno type="ISSN">1385-8947</idno>
<imprint><date type="datePub">2012-10-01</date>
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<profileDesc><textClass><keywords scheme="mix" xml:lang="en"><term>Hydrogen</term>
<term>Kinetic data acquisition</term>
<term>Methane reforming</term>
<term>Microreactor modeling</term>
<term>Microstructured reactor</term>
<term>Process intensification</term>
<term>Syngas</term>
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<front><div type="abstract" xml:lang="en">In the frame of steam methane reforming process intensification, a highly active and stable catalyst based on rhodium with catalyst formulation and structure adapted to millistructured reactors has been formulated. This catalyst has been tested in industrial conditions (800, 850 or 900 degrees C and 20 bars) on a single channel which is representative of one channel of a more complex millistructured SMR reactor. Then, a detailed mathematical model for acquisition of the global reaction kinetics with this new catalyst has been developed and validated from experimental catalytic tests. The developed kinetics is dependent of the catalyst microstructure. This study presents the set-up, the model, the experimental catalytic runs and the global kinetics estimation protocol. It demonstrates, on one hand, that millistructured reactor is suitable for kinetic data acquisition and, on the other hand, the possibility of SMR process intensification, for improved energy efficiency and process size reduction.</div>
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<name sortKey="Prost, L" sort="Prost, L" uniqKey="Prost L" first="L." last="Prost">L. Prost</name>
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   |texte=   Steam methane reforming reaction process intensification by using a millistructured reactor: Experimental setup and model validation for global kinetic reaction rate estimation
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Steam methane reforming reaction process intensification by using a millistructured reactor: Experimental setup and model validation for global kinetic reaction rate estimation

Steam methane reforming reaction process intensification by using a millistructured reactor: Experimental setup and model validation for global kinetic reaction rate estimation

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