Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar
Identifieur interne : 000C07 ( PascalFrancis/Curation ); précédent : 000C06; suivant : 000C08Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar
Auteurs : Meththika Vithanage [Corée du Sud, Sri Lanka] ; ANUSHKA UPAMALI RAJAPAKSHA [Corée du Sud, Sri Lanka] ; XIANGYU TANG [République populaire de Chine] ; Sören Thiele-Bruhn [Allemagne] ; KYE HOON KIM [Corée du Sud] ; Sung-Eun Lee [Corée du Sud] ; YONG SIK OK [Corée du Sud, Canada]Source :
- Journal of environmental management [ 0301-4797 ] ; 2014.
Descripteurs français
- Pascal (Inist)
- Wicri :
- topic : Médicament.
English descriptors
- KwdEn :
Abstract
Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (KD,eff) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.
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<term>Environmental management</term>
<term>Environmental monitoring</term>
<term>Environmental protection</term>
<term>Invasive species</term>
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<term>Plant</term>
<term>Soot</term>
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<term>Transport</term>
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<term>Sol agricole</term>
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<term>Espèce envahissante</term>
<term>Charbon bois</term>
<term>Suie</term>
<term>Médicament</term>
<term>Biosorption</term>
<term>Matière organique</term>
<term>Gestion environnement</term>
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<front><div type="abstract" xml:lang="en">Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (K<sub>D,eff</sub>
) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.</div>
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<fA08 i1="01" i2="1" l="ENG"><s1>Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar</s1>
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<fA11 i1="01" i2="1"><s1>VITHANAGE (Meththika)</s1>
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<fA11 i1="02" i2="1"><s1>ANUSHKA UPAMALI RAJAPAKSHA</s1>
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<fA14 i1="07"><s1>Department of Renewable Resources, University of Alberta</s1>
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<fC01 i1="01" l="ENG"><s0>Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (K<sub>D,eff</sub>
) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.</s0>
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<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Biosorption</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Biosorción</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Matière organique</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Organic matter</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Materia orgánica</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Gestion environnement</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Environmental management</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Gestiòn medio ambiente</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Surveillance écologique</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Environmental monitoring</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Vigilancia ecológica</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Protection environnement</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Environmental protection</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Protección medio ambiente</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Polluant émergent</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Emerging contaminant</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fN21><s1>209</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
</pA>
</standard>
</inist>
</record>
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