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Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar

Identifieur interne : 000C07 ( PascalFrancis/Curation ); précédent : 000C06; suivant : 000C08

Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar

Auteurs : Meththika Vithanage [Corée du Sud, Sri Lanka] ; ANUSHKA UPAMALI RAJAPAKSHA [Corée du Sud, Sri Lanka] ; XIANGYU TANG [République populaire de Chine] ; Sören Thiele-Bruhn [Allemagne] ; KYE HOON KIM [Corée du Sud] ; Sung-Eun Lee [Corée du Sud] ; YONG SIK OK [Corée du Sud, Canada]

Source :

RBID : Pascal:14-0170411

Descripteurs français

English descriptors

Abstract

Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (KD,eff) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.
pA  
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A02 01      @0 JEVMAW
A03   1    @0 J. environ. manage.
A05       @2 141
A08 01  1  ENG  @1 Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar
A11 01  1    @1 VITHANAGE (Meththika)
A11 02  1    @1 ANUSHKA UPAMALI RAJAPAKSHA
A11 03  1    @1 XIANGYU TANG
A11 04  1    @1 THIELE-BRUHN (Sören)
A11 05  1    @1 KYE HOON KIM
A11 06  1    @1 LEE (Sung-Eun)
A11 07  1    @1 YONG SIK OK
A14 01      @1 Korea Biochar Research Center and Department of Biological Environment, Kangwon National University @2 Chuncheon @3 KOR @Z 1 aut. @Z 2 aut. @Z 7 aut.
A14 02      @1 Chemical and Environmental Systems Modeling Research Group, Institute of Fundamental Studies @2 Kandy @3 LKA @Z 1 aut. @Z 2 aut.
A14 03      @1 Institute of Mountain Hazards and Environment, Chinese Academy of Sciences @2 Chengdu @3 CHN @Z 3 aut.
A14 04      @1 Department of Soil Science, University of Trier @2 Trier @3 DEU @Z 4 aut.
A14 05      @1 Department of Environmental Horticulture, The University of Seoul @2 Seoul @3 KOR @Z 5 aut.
A14 06      @1 School of Applied Biosciences, Kyungpook National University @2 Daegu @3 KOR @Z 6 aut.
A14 07      @1 Department of Renewable Resources, University of Alberta @2 Edmonton @3 CAN @Z 7 aut.
A20       @1 95-103
A21       @1 2014
A23 01      @0 ENG
A43 01      @1 INIST @2 16218 @5 354000502757270110
A44       @0 0000 @1 © 2014 INIST-CNRS. All rights reserved.
A45       @0 3/4 p.
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C01 01    ENG  @0 Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (KD,eff) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.
C02 01  X    @0 002A14D02A
C02 02  X    @0 002A14D02B
C03 01  X  FRE  @0 Sorption @5 01
C03 01  X  ENG  @0 Sorption @5 01
C03 01  X  SPA  @0 Sorción @5 01
C03 02  X  FRE  @0 Transport @5 02
C03 02  X  ENG  @0 Transport @5 02
C03 02  X  SPA  @0 Transporte @5 02
C03 03  X  FRE  @0 Sol agricole @2 NT @5 03
C03 03  X  ENG  @0 Agricultural soil @2 NT @5 03
C03 03  X  SPA  @0 Suelo agrícola @2 NT @5 03
C03 04  X  FRE  @0 Plante @5 04
C03 04  X  ENG  @0 Plant @5 04
C03 04  X  SPA  @0 Planta @5 04
C03 05  X  FRE  @0 Espèce envahissante @5 05
C03 05  X  ENG  @0 Invasive species @5 05
C03 05  X  SPA  @0 Especie invasora @5 05
C03 06  X  FRE  @0 Charbon bois @5 06
C03 06  X  ENG  @0 Charcoal @5 06
C03 06  X  SPA  @0 Carbón madera @5 06
C03 07  X  FRE  @0 Suie @5 07
C03 07  X  ENG  @0 Soot @5 07
C03 07  X  SPA  @0 Hollín @5 07
C03 08  X  FRE  @0 Médicament @5 08
C03 08  X  ENG  @0 Drug @5 08
C03 08  X  SPA  @0 Medicamento @5 08
C03 09  X  FRE  @0 Biosorption @5 09
C03 09  X  ENG  @0 Biosorption @5 09
C03 09  X  SPA  @0 Biosorción @5 09
C03 10  X  FRE  @0 Matière organique @5 10
C03 10  X  ENG  @0 Organic matter @5 10
C03 10  X  SPA  @0 Materia orgánica @5 10
C03 11  X  FRE  @0 Gestion environnement @5 11
C03 11  X  ENG  @0 Environmental management @5 11
C03 11  X  SPA  @0 Gestiòn medio ambiente @5 11
C03 12  X  FRE  @0 Surveillance écologique @5 12
C03 12  X  ENG  @0 Environmental monitoring @5 12
C03 12  X  SPA  @0 Vigilancia ecológica @5 12
C03 13  X  FRE  @0 Protection environnement @5 13
C03 13  X  ENG  @0 Environmental protection @5 13
C03 13  X  SPA  @0 Protección medio ambiente @5 13
C03 14  X  FRE  @0 Polluant émergent @4 CD @5 96
C03 14  X  ENG  @0 Emerging contaminant @4 CD @5 96
N21       @1 209
N44 01      @1 OTO
N82       @1 OTO

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Pascal:14-0170411

Le document en format XML

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<term>Agricultural soil</term>
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<term>Drug</term>
<term>Emerging contaminant</term>
<term>Environmental management</term>
<term>Environmental monitoring</term>
<term>Environmental protection</term>
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<term>Sorption</term>
<term>Transport</term>
<term>Sol agricole</term>
<term>Plante</term>
<term>Espèce envahissante</term>
<term>Charbon bois</term>
<term>Suie</term>
<term>Médicament</term>
<term>Biosorption</term>
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<term>Protection environnement</term>
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<div type="abstract" xml:lang="en">Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (K
<sub>D,eff</sub>
) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.</div>
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<s2>Trier</s2>
<s3>DEU</s3>
<sZ>4 aut.</sZ>
</fA14>
<fA14 i1="05">
<s1>Department of Environmental Horticulture, The University of Seoul</s1>
<s2>Seoul</s2>
<s3>KOR</s3>
<sZ>5 aut.</sZ>
</fA14>
<fA14 i1="06">
<s1>School of Applied Biosciences, Kyungpook National University</s1>
<s2>Daegu</s2>
<s3>KOR</s3>
<sZ>6 aut.</sZ>
</fA14>
<fA14 i1="07">
<s1>Department of Renewable Resources, University of Alberta</s1>
<s2>Edmonton</s2>
<s3>CAN</s3>
<sZ>7 aut.</sZ>
</fA14>
<fA20>
<s1>95-103</s1>
</fA20>
<fA21>
<s1>2014</s1>
</fA21>
<fA23 i1="01">
<s0>ENG</s0>
</fA23>
<fA43 i1="01">
<s1>INIST</s1>
<s2>16218</s2>
<s5>354000502757270110</s5>
</fA43>
<fA44>
<s0>0000</s0>
<s1>© 2014 INIST-CNRS. All rights reserved.</s1>
</fA44>
<fA45>
<s0>3/4 p.</s0>
</fA45>
<fA47 i1="01" i2="1">
<s0>14-0170411</s0>
</fA47>
<fA60>
<s1>P</s1>
</fA60>
<fA61>
<s0>A</s0>
</fA61>
<fA64 i1="01" i2="1">
<s0>Journal of environmental management</s0>
</fA64>
<fA66 i1="01">
<s0>GBR</s0>
</fA66>
<fC01 i1="01" l="ENG">
<s0>Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (K
<sub>D,eff</sub>
) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.</s0>
</fC01>
<fC02 i1="01" i2="X">
<s0>002A14D02A</s0>
</fC02>
<fC02 i1="02" i2="X">
<s0>002A14D02B</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE">
<s0>Sorption</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG">
<s0>Sorption</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA">
<s0>Sorción</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE">
<s0>Transport</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG">
<s0>Transport</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA">
<s0>Transporte</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE">
<s0>Sol agricole</s0>
<s2>NT</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG">
<s0>Agricultural soil</s0>
<s2>NT</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA">
<s0>Suelo agrícola</s0>
<s2>NT</s2>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE">
<s0>Plante</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG">
<s0>Plant</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA">
<s0>Planta</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE">
<s0>Espèce envahissante</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG">
<s0>Invasive species</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA">
<s0>Especie invasora</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE">
<s0>Charbon bois</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG">
<s0>Charcoal</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA">
<s0>Carbón madera</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE">
<s0>Suie</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG">
<s0>Soot</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA">
<s0>Hollín</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE">
<s0>Médicament</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG">
<s0>Drug</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA">
<s0>Medicamento</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE">
<s0>Biosorption</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG">
<s0>Biosorption</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA">
<s0>Biosorción</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE">
<s0>Matière organique</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG">
<s0>Organic matter</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA">
<s0>Materia orgánica</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE">
<s0>Gestion environnement</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG">
<s0>Environmental management</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA">
<s0>Gestiòn medio ambiente</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE">
<s0>Surveillance écologique</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG">
<s0>Environmental monitoring</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA">
<s0>Vigilancia ecológica</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE">
<s0>Protection environnement</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG">
<s0>Environmental protection</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA">
<s0>Protección medio ambiente</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE">
<s0>Polluant émergent</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG">
<s0>Emerging contaminant</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fN21>
<s1>209</s1>
</fN21>
<fN44 i1="01">
<s1>OTO</s1>
</fN44>
<fN82>
<s1>OTO</s1>
</fN82>
</pA>
</standard>
</inist>
</record>

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