State-to-State Inelastic Scattering of O2 with Helium.
Identifieur interne : 000054 ( PubMed/Corpus ); précédent : 000053; suivant : 000055State-to-State Inelastic Scattering of O2 with Helium.
Auteurs : Chandan Kumar Bishwakarma ; George Van Oevelen ; Roy Scheidsbach ; David H. Parker ; Yulia Kalugina ; François LiqueSource :
- The journal of physical chemistry. A [ 1520-5215 ] ; 2016.
Abstract
Molecular oxygen (O2) is extremely important for a wide variety of processes on and outside Earth. Indeed, O2–He collisions are crucial to model O2 abundance in space or to create ultracold O2 molecules. A crossed molecular beam experiment to probe rotational excitation of O2 due to helium collisions at energies of 660 cm–1 is reported. Velocity map imaging was combined with state-selective detection of O2(X3Σg–) by (2+1) resonance-enhanced multiphoton ionization. The obtained raw O2+ images were corrected from density to flux and the differential cross sections (DCS) were then extracted for six O2 final states. Exact quantum mechanical calculations were also performed. A very good agreement between experimental and theoretical DCSs was found by using an initial O2 beam population ratio of 80% for the first rotational state and 20% for the first excited state. The agreement demonstrates our ability to model inelastic processes between O2 molecules and rare gas both theoretically and experimentally.
DOI: 10.1021/acs.jpca.6b00817
PubMed: 26829188
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pubmed:26829188Le document en format XML
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<author><name sortKey="Lique, Francois" sort="Lique, Francois" uniqKey="Lique F" first="François" last="Lique">François Lique</name>
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<front><div type="abstract" xml:lang="en">Molecular oxygen (O2) is extremely important for a wide variety of processes on and outside Earth. Indeed, O2–He collisions are crucial to model O2 abundance in space or to create ultracold O2 molecules. A crossed molecular beam experiment to probe rotational excitation of O2 due to helium collisions at energies of 660 cm–1 is reported. Velocity map imaging was combined with state-selective detection of O2(X3Σg–) by (2+1) resonance-enhanced multiphoton ionization. The obtained raw O2+ images were corrected from density to flux and the differential cross sections (DCS) were then extracted for six O2 final states. Exact quantum mechanical calculations were also performed. A very good agreement between experimental and theoretical DCSs was found by using an initial O2 beam population ratio of 80% for the first rotational state and 20% for the first excited state. The agreement demonstrates our ability to model inelastic processes between O2 molecules and rare gas both theoretically and experimentally.</div>
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<Abstract><AbstractText>Molecular oxygen (O2) is extremely important for a wide variety of processes on and outside Earth. Indeed, O2–He collisions are crucial to model O2 abundance in space or to create ultracold O2 molecules. A crossed molecular beam experiment to probe rotational excitation of O2 due to helium collisions at energies of 660 cm–1 is reported. Velocity map imaging was combined with state-selective detection of O2(X3Σg–) by (2+1) resonance-enhanced multiphoton ionization. The obtained raw O2+ images were corrected from density to flux and the differential cross sections (DCS) were then extracted for six O2 final states. Exact quantum mechanical calculations were also performed. A very good agreement between experimental and theoretical DCSs was found by using an initial O2 beam population ratio of 80% for the first rotational state and 20% for the first excited state. The agreement demonstrates our ability to model inelastic processes between O2 molecules and rare gas both theoretically and experimentally.</AbstractText>
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