Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): transport and fate of PAHs from the atmosphere to the outlet.
Identifieur interne : 000151 ( Ncbi/Checkpoint ); précédent : 000150; suivant : 000152Mass balance for polycyclic aromatic hydrocarbons in the urban watershed of Le Havre (France): transport and fate of PAHs from the atmosphere to the outlet.
Auteurs : A. Motelay-Massei [France] ; B. Garban ; K. Tiphagne-Larcher ; M. Chevreuil ; D. OllivonSource :
- Water research [ 0043-1354 ] ; 2006.
Descripteurs français
- Wicri :
- geographic : France.
English descriptors
- KwdEn :
- MESH :
- chemical , analysis : Air Pollutants, Polycyclic Hydrocarbons, Aromatic, Water Pollutants, Chemical.
- geographic : France.
- chemistry : Rivers.
- Air Movements, Environmental Monitoring, Urbanization, Water Movements.
Abstract
Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kg km(-2) yr(-1) while PAH atmospheric deposition was 0.21 kg km(-2) yr(-1). The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air-water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).
DOI: 10.1016/j.watres.2006.03.015
PubMed: 16697025
Affiliations:
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pubmed:16697025Le document en format XML
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<author><name sortKey="Garban, B" sort="Garban, B" uniqKey="Garban B" first="B" last="Garban">B. Garban</name>
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<author><name sortKey="Tiphagne Larcher, K" sort="Tiphagne Larcher, K" uniqKey="Tiphagne Larcher K" first="K" last="Tiphagne-Larcher">K. Tiphagne-Larcher</name>
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<series><title level="j">Water research</title>
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<front><div type="abstract" xml:lang="en">Polycyclic aromatic hydrocarbon (PAH) concentrations have been monitored simultaneously in ambient air, bulk atmospheric deposition and runoff waters during one year in a small urban watershed of the Seine river basin (France). PAH fluxes from the atmosphere to the outlet of the urban watershed have been calculated to establish a mass balance for PAHs. PAH flux in runoff waters was 5.2 kg km(-2) yr(-1) while PAH atmospheric deposition was 0.21 kg km(-2) yr(-1). The comparison between atmospheric input and output by runoff has shown the importance of street deposits that appeared to be the most important source of PAHs for surface waters in urban areas. PAH profiles in the various compartments showed the fate of PAHs in the air-water system: proportion of carcinogenic PAHs was more important in runoff waters (35%) than in bulk atmospheric deposition (22%) and air (6%).</div>
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<name sortKey="Ollivon, D" sort="Ollivon, D" uniqKey="Ollivon D" first="D" last="Ollivon">D. Ollivon</name>
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