Characterization of ionic liquid pretreated aspen wood using semi-quantitative methods for ethanol production.
Identifieur interne : 002764 ( Main/Exploration ); précédent : 002763; suivant : 002765Characterization of ionic liquid pretreated aspen wood using semi-quantitative methods for ethanol production.
Auteurs : Amir Goshadrou [Canada] ; Keikhosro Karimi ; Mark LefsrudSource :
- Carbohydrate polymers [ 1879-1344 ] ; 2013.
Descripteurs français
- KwdFr :
- MESH :
- composition chimique : Bois, Imidazoles, Lignine, Liquides ioniques, Populus, Éthanol.
- Fermentation, Hydrolyse.
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Ethanol, Imidazoles, Ionic Liquids, Lignin.
- chemistry : Populus, Wood.
- Fermentation, Hydrolysis.
Abstract
Aspen wood (Populus tremula) was pretreated with ionic liquid 1-ethyl-3-methylimidazolium acetate ([EMIM]OAc) and dilute sulfuric acid for improvement of ethanol production. The ionic liquid pretreatment included wood dissolution at 120°C and 5% solid loading for 1, 3, and 5h followed by regeneration using water as an anti-solvent. More than 95% enzymatic digestibility was achieved for the ionic liquid treated wood, while the yield from the untreated wood was only 5.3%. Furthermore, over 81% of the maximum theoretical ethanol yield was attained after 24h fermentation of the ionic liquid treated wood, whereas the yields were only 5.3% and 42.1% for the untreated and dilute acid treated materials, respectively. A side-by-side comparative analysis of the pretreated materials using semi-quantitative techniques (e.g., Simons' staining and enzyme adsorption) revealed that the ionic liquid treatment was much more successful in increasing the cellulose accessibility to cellulases and decreasing the lignin content.
DOI: 10.1016/j.carbpol.2013.04.017
PubMed: 23768585
Affiliations:
Links toward previous steps (curation, corpus...)
Le document en format XML
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<author><name sortKey="Goshadrou, Amir" sort="Goshadrou, Amir" uniqKey="Goshadrou A" first="Amir" last="Goshadrou">Amir Goshadrou</name>
<affiliation wicri:level="4"><nlm:affiliation>Department of Bioresource Engineering, McGill University, 21111 Lakeshore Road, Ste. Anne de Bellevue, Montreal, Quebec H9X 3V9, Canada.</nlm:affiliation>
<country xml:lang="fr">Canada</country>
<wicri:regionArea>Department of Bioresource Engineering, McGill University, 21111 Lakeshore Road, Ste. Anne de Bellevue, Montreal, Quebec H9X 3V9</wicri:regionArea>
<orgName type="university">Université McGill</orgName>
<placeName><settlement type="city">Montréal</settlement>
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<author><name sortKey="Karimi, Keikhosro" sort="Karimi, Keikhosro" uniqKey="Karimi K" first="Keikhosro" last="Karimi">Keikhosro Karimi</name>
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<author><name sortKey="Lefsrud, Mark" sort="Lefsrud, Mark" uniqKey="Lefsrud M" first="Mark" last="Lefsrud">Mark Lefsrud</name>
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<affiliation wicri:level="4"><nlm:affiliation>Department of Bioresource Engineering, McGill University, 21111 Lakeshore Road, Ste. Anne de Bellevue, Montreal, Quebec H9X 3V9, Canada.</nlm:affiliation>
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<series><title level="j">Carbohydrate polymers</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Ethanol (chemistry)</term>
<term>Fermentation (MeSH)</term>
<term>Hydrolysis (MeSH)</term>
<term>Imidazoles (chemistry)</term>
<term>Ionic Liquids (chemistry)</term>
<term>Lignin (chemistry)</term>
<term>Populus (chemistry)</term>
<term>Wood (chemistry)</term>
</keywords>
<keywords scheme="KwdFr" xml:lang="fr"><term>Bois (composition chimique)</term>
<term>Fermentation (MeSH)</term>
<term>Hydrolyse (MeSH)</term>
<term>Imidazoles (composition chimique)</term>
<term>Lignine (composition chimique)</term>
<term>Liquides ioniques (composition chimique)</term>
<term>Populus (composition chimique)</term>
<term>Éthanol (composition chimique)</term>
</keywords>
<keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Ethanol</term>
<term>Imidazoles</term>
<term>Ionic Liquids</term>
<term>Lignin</term>
</keywords>
<keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Populus</term>
<term>Wood</term>
</keywords>
<keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Bois</term>
<term>Imidazoles</term>
<term>Lignine</term>
<term>Liquides ioniques</term>
<term>Populus</term>
<term>Éthanol</term>
</keywords>
<keywords scheme="MESH" xml:lang="en"><term>Fermentation</term>
<term>Hydrolysis</term>
</keywords>
<keywords scheme="MESH" xml:lang="fr"><term>Fermentation</term>
<term>Hydrolyse</term>
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<front><div type="abstract" xml:lang="en">Aspen wood (Populus tremula) was pretreated with ionic liquid 1-ethyl-3-methylimidazolium acetate ([EMIM]OAc) and dilute sulfuric acid for improvement of ethanol production. The ionic liquid pretreatment included wood dissolution at 120°C and 5% solid loading for 1, 3, and 5h followed by regeneration using water as an anti-solvent. More than 95% enzymatic digestibility was achieved for the ionic liquid treated wood, while the yield from the untreated wood was only 5.3%. Furthermore, over 81% of the maximum theoretical ethanol yield was attained after 24h fermentation of the ionic liquid treated wood, whereas the yields were only 5.3% and 42.1% for the untreated and dilute acid treated materials, respectively. A side-by-side comparative analysis of the pretreated materials using semi-quantitative techniques (e.g., Simons' staining and enzyme adsorption) revealed that the ionic liquid treatment was much more successful in increasing the cellulose accessibility to cellulases and decreasing the lignin content.</div>
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<Issue>2</Issue>
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<Title>Carbohydrate polymers</Title>
<ISOAbbreviation>Carbohydr Polym</ISOAbbreviation>
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<ArticleTitle>Characterization of ionic liquid pretreated aspen wood using semi-quantitative methods for ethanol production.</ArticleTitle>
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<Abstract><AbstractText>Aspen wood (Populus tremula) was pretreated with ionic liquid 1-ethyl-3-methylimidazolium acetate ([EMIM]OAc) and dilute sulfuric acid for improvement of ethanol production. The ionic liquid pretreatment included wood dissolution at 120°C and 5% solid loading for 1, 3, and 5h followed by regeneration using water as an anti-solvent. More than 95% enzymatic digestibility was achieved for the ionic liquid treated wood, while the yield from the untreated wood was only 5.3%. Furthermore, over 81% of the maximum theoretical ethanol yield was attained after 24h fermentation of the ionic liquid treated wood, whereas the yields were only 5.3% and 42.1% for the untreated and dilute acid treated materials, respectively. A side-by-side comparative analysis of the pretreated materials using semi-quantitative techniques (e.g., Simons' staining and enzyme adsorption) revealed that the ionic liquid treatment was much more successful in increasing the cellulose accessibility to cellulases and decreasing the lignin content.</AbstractText>
<CopyrightInformation>Copyright © 2013 Elsevier Ltd. All rights reserved.</CopyrightInformation>
</Abstract>
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<ForeName>Amir</ForeName>
<Initials>A</Initials>
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<Author ValidYN="Y"><LastName>Lefsrud</LastName>
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