Pyrolysis and gasification of typical components in wastes with macro-TGA.
Identifieur interne : 001B70 ( Main/Exploration ); précédent : 001B69; suivant : 001B71Pyrolysis and gasification of typical components in wastes with macro-TGA.
Auteurs : Aihong Meng [République populaire de Chine] ; Shen Chen [République populaire de Chine] ; Yanqiu Long [République populaire de Chine] ; Hui Zhou [République populaire de Chine] ; Yanguo Zhang [République populaire de Chine] ; Qinghai Li [République populaire de Chine]Source :
- Waste management (New York, N.Y.) [ 1879-2456 ] ; 2015.
Descripteurs français
- KwdFr :
- MESH :
English descriptors
- KwdEn :
- MESH :
- chemical , analysis : Air Pollutants, Carbon Dioxide, Solid Waste.
- Incineration, Kinetics, Models, Theoretical, Refuse Disposal, Thermogravimetry.
Abstract
The pyrolysis and gasification of typical components of solid waste, cellulose, hemicellulose, lignin, pectin, starch, polyethylene (PE), polystyrene (PS), polyvinyl chloride (PVC) and poly(ethylene terephthalate) (PET) were performed and compared in a macro thermogravimetric analyzer (macro-TGA). Three model biomasses, poplar stem, orange peel and Chinese cabbage, were applied to pyrolysis and gasification simulation by their components based on TG curves. Compared to those from TGA, peaks temperature of the differential thermogravimetric (DTG) curves of each samples pyrolysis on macro-TGA delayed 30-55°C due to heat transferring effect. CO2 promoted the thermal decomposition of hemicellulose, lignin, starch, pectin and model biomasses significantly by Boudouard reaction, and enhanced slightly the decomposition of PET. The activation energy (AE) of biomass components pyrolysis on macro-TGA was 167-197 kJ/mol, while that of plastic samples was 185-235 kJ/mol. The activation energy of 351-377 kJ/mol was corresponding to the Boudouard reaction in CO2 gasification. All overlap ratios in pseudo-components simulation were higher than 0.98 to indicate that pseudo-components model could be applied to both pyrolysis and CO2 gasification, and the mass fractions of components derived from pyrolysis and gasification were slightly different but not brought in obvious difference in simulating curves when they were applied across.
DOI: 10.1016/j.wasman.2015.08.025
PubMed: 26318422
Affiliations:
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Electronic address: zhangyg@tsinghua.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author><author><name sortKey="Li, Qinghai" sort="Li, Qinghai" uniqKey="Li Q" first="Qinghai" last="Li">Qinghai Li</name><affiliation wicri:level="1"><nlm:affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author></analytic><series><title level="j">Waste management (New York, N.Y.)</title><idno type="eISSN">1879-2456</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Air Pollutants (analysis)</term><term>Carbon Dioxide (analysis)</term><term>Incineration (MeSH)</term><term>Kinetics (MeSH)</term><term>Models, Theoretical (MeSH)</term><term>Refuse Disposal (MeSH)</term><term>Solid Waste (analysis)</term><term>Thermogravimetry (MeSH)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Cinétique (MeSH)</term><term>Dioxyde de carbone (analyse)</term><term>Déchets solides (analyse)</term><term>Incinération (MeSH)</term><term>Modèles théoriques (MeSH)</term><term>Polluants atmosphériques (analyse)</term><term>Thermogravimétrie (MeSH)</term><term>Élimination des déchets (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Air Pollutants</term><term>Carbon Dioxide</term><term>Solid Waste</term></keywords><keywords scheme="MESH" qualifier="analyse" xml:lang="fr"><term>Dioxyde de carbone</term><term>Déchets solides</term><term>Polluants atmosphériques</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Incineration</term><term>Kinetics</term><term>Models, Theoretical</term><term>Refuse Disposal</term><term>Thermogravimetry</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Cinétique</term><term>Incinération</term><term>Modèles théoriques</term><term>Thermogravimétrie</term><term>Élimination des déchets</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The pyrolysis and gasification of typical components of solid waste, cellulose, hemicellulose, lignin, pectin, starch, polyethylene (PE), polystyrene (PS), polyvinyl chloride (PVC) and poly(ethylene terephthalate) (PET) were performed and compared in a macro thermogravimetric analyzer (macro-TGA). Three model biomasses, poplar stem, orange peel and Chinese cabbage, were applied to pyrolysis and gasification simulation by their components based on TG curves. Compared to those from TGA, peaks temperature of the differential thermogravimetric (DTG) curves of each samples pyrolysis on macro-TGA delayed 30-55°C due to heat transferring effect. CO2 promoted the thermal decomposition of hemicellulose, lignin, starch, pectin and model biomasses significantly by Boudouard reaction, and enhanced slightly the decomposition of PET. The activation energy (AE) of biomass components pyrolysis on macro-TGA was 167-197 kJ/mol, while that of plastic samples was 185-235 kJ/mol. The activation energy of 351-377 kJ/mol was corresponding to the Boudouard reaction in CO2 gasification. All overlap ratios in pseudo-components simulation were higher than 0.98 to indicate that pseudo-components model could be applied to both pyrolysis and CO2 gasification, and the mass fractions of components derived from pyrolysis and gasification were slightly different but not brought in obvious difference in simulating curves when they were applied across.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">26318422</PMID><DateCompleted><Year>2016</Year><Month>08</Month><Day>16</Day></DateCompleted><DateRevised><Year>2015</Year><Month>11</Month><Day>10</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1879-2456</ISSN><JournalIssue CitedMedium="Internet"><Volume>46</Volume><PubDate><Year>2015</Year><Month>Dec</Month></PubDate></JournalIssue><Title>Waste management (New York, N.Y.)</Title><ISOAbbreviation>Waste Manag</ISOAbbreviation></Journal><ArticleTitle>Pyrolysis and gasification of typical components in wastes with macro-TGA.</ArticleTitle><Pagination><MedlinePgn>247-56</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.wasman.2015.08.025</ELocationID><ELocationID EIdType="pii" ValidYN="Y">S0956-053X(15)30093-3</ELocationID><Abstract><AbstractText>The pyrolysis and gasification of typical components of solid waste, cellulose, hemicellulose, lignin, pectin, starch, polyethylene (PE), polystyrene (PS), polyvinyl chloride (PVC) and poly(ethylene terephthalate) (PET) were performed and compared in a macro thermogravimetric analyzer (macro-TGA). Three model biomasses, poplar stem, orange peel and Chinese cabbage, were applied to pyrolysis and gasification simulation by their components based on TG curves. Compared to those from TGA, peaks temperature of the differential thermogravimetric (DTG) curves of each samples pyrolysis on macro-TGA delayed 30-55°C due to heat transferring effect. CO2 promoted the thermal decomposition of hemicellulose, lignin, starch, pectin and model biomasses significantly by Boudouard reaction, and enhanced slightly the decomposition of PET. The activation energy (AE) of biomass components pyrolysis on macro-TGA was 167-197 kJ/mol, while that of plastic samples was 185-235 kJ/mol. The activation energy of 351-377 kJ/mol was corresponding to the Boudouard reaction in CO2 gasification. All overlap ratios in pseudo-components simulation were higher than 0.98 to indicate that pseudo-components model could be applied to both pyrolysis and CO2 gasification, and the mass fractions of components derived from pyrolysis and gasification were slightly different but not brought in obvious difference in simulating curves when they were applied across.</AbstractText><CopyrightInformation>Copyright © 2015 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Meng</LastName><ForeName>Aihong</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Chen</LastName><ForeName>Shen</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Long</LastName><ForeName>Yanqiu</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhou</LastName><ForeName>Hui</ForeName><Initials>H</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Yanguo</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China. Electronic address: zhangyg@tsinghua.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Li</LastName><ForeName>Qinghai</ForeName><Initials>Q</Initials><AffiliationInfo><Affiliation>Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Thermal Engineering, Tsinghua University, Beijing 100084, PR China.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2015</Year><Month>08</Month><Day>28</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>Waste Manag</MedlineTA><NlmUniqueID>9884362</NlmUniqueID><ISSNLinking>0956-053X</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D000393">Air Pollutants</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D062611">Solid Waste</NameOfSubstance></Chemical><Chemical><RegistryNumber>142M471B3J</RegistryNumber><NameOfSubstance UI="D002245">Carbon Dioxide</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000393" MajorTopicYN="N">Air Pollutants</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="Y">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002245" MajorTopicYN="N">Carbon Dioxide</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="Y">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D017745" MajorTopicYN="Y">Incineration</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D007700" MajorTopicYN="N">Kinetics</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008962" MajorTopicYN="N">Models, Theoretical</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D012037" MajorTopicYN="Y">Refuse Disposal</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D062611" MajorTopicYN="N">Solid Waste</DescriptorName><QualifierName UI="Q000032" MajorTopicYN="Y">analysis</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D013818" MajorTopicYN="N">Thermogravimetry</DescriptorName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Distribution activation energy model (DAEM)</Keyword><Keyword MajorTopicYN="N">Gasification</Keyword><Keyword MajorTopicYN="N">Macro-TGA</Keyword><Keyword MajorTopicYN="N">Pseudo-components model</Keyword><Keyword MajorTopicYN="N">Pyrolysis</Keyword><Keyword MajorTopicYN="N">Simulation</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2015</Year><Month>04</Month><Day>18</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2015</Year><Month>08</Month><Day>04</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2015</Year><Month>08</Month><Day>18</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2015</Year><Month>8</Month><Day>31</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2015</Year><Month>9</Month><Day>1</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2016</Year><Month>8</Month><Day>17</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">26318422</ArticleId><ArticleId IdType="pii">S0956-053X(15)30093-3</ArticleId><ArticleId IdType="doi">10.1016/j.wasman.2015.08.025</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>République populaire de Chine</li></country><settlement><li>Pékin</li></settlement></list><tree><country name="République populaire de Chine"><noRegion><name sortKey="Meng, Aihong" sort="Meng, Aihong" uniqKey="Meng A" first="Aihong" last="Meng">Aihong Meng</name></noRegion><name sortKey="Chen, Shen" sort="Chen, Shen" uniqKey="Chen S" first="Shen" last="Chen">Shen Chen</name><name sortKey="Li, Qinghai" sort="Li, Qinghai" uniqKey="Li Q" first="Qinghai" last="Li">Qinghai Li</name><name sortKey="Long, Yanqiu" sort="Long, Yanqiu" uniqKey="Long Y" first="Yanqiu" last="Long">Yanqiu Long</name><name sortKey="Zhang, Yanguo" sort="Zhang, Yanguo" uniqKey="Zhang Y" first="Yanguo" last="Zhang">Yanguo Zhang</name><name sortKey="Zhou, Hui" sort="Zhou, Hui" uniqKey="Zhou H" first="Hui" last="Zhou">Hui Zhou</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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