A Convergent Approach for a Deep Converting Lignin-First Biorefinery Rendering High-Energy-Density Drop-in Fuels.
Identifieur interne : 001091 ( Main/Exploration ); précédent : 001090; suivant : 001092A Convergent Approach for a Deep Converting Lignin-First Biorefinery Rendering High-Energy-Density Drop-in Fuels.
Auteurs : Zhengwen Cao [Allemagne] ; Michael Dierks [Allemagne] ; Matthew Thomas Clough [Allemagne] ; Ilton Barros Daltro De Castro [Allemagne] ; Roberto Rinaldi [Royaume-Uni]Source :
- Joule [ 2542-4351 ] ; 2018.
Abstract
Herein, a lignin-centered convergent approach to produce either aliphatic or aromatic bio-hydrocarbons is introduced. First, poplar or spruce wood was deconstructed by a lignin-first biorefining process, a technique based on the early-stage catalytic conversion of lignin, yielding lignin oils along with cellulosic pulps. Next, the lignin oils were catalytically upgraded in the presence of a phosphidated Ni/SiO2 catalyst under H2 pressure. Notably, selectivity toward aliphatics or aromatics can simply be adjusted by changes in H2 pressure and temperature. The process renders two distinct main cuts of branched hydrocarbons (gasoline: C6-C10, and kerosene/diesel: C14-C20). As the approach is H2-intensive, we examined the utilization of pulp as an H2 source via gasification. For several biomass sources, the H2 obtainable by gasification stoichiometrically meets the H2 demand of the deep converting lignin-first biorefinery, making this concept plausible for the production of high-energy-density drop-in biofuels.
DOI: 10.1016/j.joule.2018.03.012
PubMed: 29955733
PubMed Central: PMC6015120
Affiliations:
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<front><div type="abstract" xml:lang="en">Herein, a lignin-centered convergent approach to produce either aliphatic or aromatic bio-hydrocarbons is introduced. First, poplar or spruce wood was deconstructed by a lignin-first biorefining process, a technique based on the early-stage catalytic conversion of lignin, yielding lignin oils along with cellulosic pulps. Next, the lignin oils were catalytically upgraded in the presence of a phosphidated Ni/SiO<sub>2</sub>
catalyst under H<sub>2</sub>
pressure. Notably, selectivity toward aliphatics or aromatics can simply be adjusted by changes in H<sub>2</sub>
pressure and temperature. The process renders two distinct main cuts of branched hydrocarbons (gasoline: C<sub>6</sub>
-C<sub>10</sub>
, and kerosene/diesel: C<sub>14</sub>
-C<sub>20</sub>
). As the approach is H<sub>2</sub>
-intensive, we examined the utilization of pulp as an H<sub>2</sub>
source via gasification. For several biomass sources, the H<sub>2</sub>
obtainable by gasification stoichiometrically meets the H<sub>2</sub>
demand of the deep converting lignin-first biorefinery, making this concept plausible for the production of high-energy-density drop-in biofuels.</div>
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<Abstract><AbstractText>Herein, a lignin-centered convergent approach to produce either aliphatic or aromatic bio-hydrocarbons is introduced. First, poplar or spruce wood was deconstructed by a lignin-first biorefining process, a technique based on the early-stage catalytic conversion of lignin, yielding lignin oils along with cellulosic pulps. Next, the lignin oils were catalytically upgraded in the presence of a phosphidated Ni/SiO<sub>2</sub>
catalyst under H<sub>2</sub>
pressure. Notably, selectivity toward aliphatics or aromatics can simply be adjusted by changes in H<sub>2</sub>
pressure and temperature. The process renders two distinct main cuts of branched hydrocarbons (gasoline: C<sub>6</sub>
-C<sub>10</sub>
, and kerosene/diesel: C<sub>14</sub>
-C<sub>20</sub>
). As the approach is H<sub>2</sub>
-intensive, we examined the utilization of pulp as an H<sub>2</sub>
source via gasification. For several biomass sources, the H<sub>2</sub>
obtainable by gasification stoichiometrically meets the H<sub>2</sub>
demand of the deep converting lignin-first biorefinery, making this concept plausible for the production of high-energy-density drop-in biofuels.</AbstractText>
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