Remediation of Soil Polluted with Cd in a Postmining Area Using Thiourea-Modified Biochar.
Identifieur interne : 000151 ( Main/Exploration ); précédent : 000150; suivant : 000152Remediation of Soil Polluted with Cd in a Postmining Area Using Thiourea-Modified Biochar.
Auteurs : Yanfeng Zhu [République populaire de Chine] ; Jing Ma [République populaire de Chine] ; Fu Chen [République populaire de Chine] ; Ruilian Yu [République populaire de Chine] ; Gongren Hu [République populaire de Chine] ; Shaoliang Zhang [République populaire de Chine]Source :
- International journal of environmental research and public health [ 1660-4601 ] ; 2020.
Abstract
Cadmium presence in soil is considered a significant threat to human health. Biochar is recognized as an effective method to immobilize Cd ions in different soils. However, obtaining effective and viable biochar to remove elevated Cd from postmining soil remains a challenge. More modifiers need to be explored to improve biochar remediation capacity. In this investigation, pot experiments were conducted to study the effects of poplar-bark biochar (PBC600) and thiourea-modified poplar-bark biochar (TPBC600) on Cd speciation and availability, as well as on soil properties. Our results showed that the addition of biochar had a significant influence on soil properties. In the presence of TPBC600, the acid-soluble and reducible Cd fractions were transformed into oxidizable and residual Cd fractions. This process effectively reduced Cd bioavailability in the soil system. Compared to PBC600, TPBC600 was more effective in improving soil pH, electrical conductivity (EC), organic matter (SOM), total nitrogen (TN), ammonium nitrogen (NH4+-N), nitrate nitrogen (NO3--N), available potassium (AK), available phosphorus (AP), and available sulfur (AS). However, this improvement diminished as incubation time increased. Results of Pearson correlation analysis, multivariate linear regression analysis, and principal component analysis showed that soil pH and available phosphorus played key roles in reducing the available cadmium in soil. Therefore, TPBC600 was shown to be an effective modifier that could be used in the remediation of soil polluted with Cd.
DOI: 10.3390/ijerph17207654
PubMed: 33092212
PubMed Central: PMC7589461
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Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Chemical Engineering, Huaqiao University, Xiamen 361021</wicri:regionArea><wicri:noRegion>Xiamen 361021</wicri:noRegion></affiliation></author><author><name sortKey="Ma, Jing" sort="Ma, Jing" uniqKey="Ma J" first="Jing" last="Ma">Jing Ma</name><affiliation wicri:level="1"><nlm:affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation></author><author><name sortKey="Chen, Fu" sort="Chen, Fu" uniqKey="Chen F" first="Fu" last="Chen">Fu Chen</name><affiliation wicri:level="1"><nlm:affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation></author><author><name sortKey="Yu, Ruilian" sort="Yu, Ruilian" uniqKey="Yu R" first="Ruilian" last="Yu">Ruilian Yu</name><affiliation wicri:level="1"><nlm:affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Chemical Engineering, Huaqiao University, Xiamen 361021</wicri:regionArea><wicri:noRegion>Xiamen 361021</wicri:noRegion></affiliation></author><author><name sortKey="Hu, Gongren" sort="Hu, Gongren" uniqKey="Hu G" first="Gongren" last="Hu">Gongren Hu</name><affiliation wicri:level="1"><nlm:affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Chemical Engineering, Huaqiao University, Xiamen 361021</wicri:regionArea><wicri:noRegion>Xiamen 361021</wicri:noRegion></affiliation></author><author><name sortKey="Zhang, Shaoliang" sort="Zhang, Shaoliang" uniqKey="Zhang S" first="Shaoliang" last="Zhang">Shaoliang Zhang</name><affiliation wicri:level="1"><nlm:affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu</wicri:regionArea><wicri:noRegion>Jiangsu</wicri:noRegion></affiliation></author></analytic><series><title level="j">International journal of environmental research and public health</title><idno type="eISSN">1660-4601</idno><imprint><date when="2020" type="published">2020</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Cadmium presence in soil is considered a significant threat to human health. Biochar is recognized as an effective method to immobilize Cd ions in different soils. However, obtaining effective and viable biochar to remove elevated Cd from postmining soil remains a challenge. More modifiers need to be explored to improve biochar remediation capacity. In this investigation, pot experiments were conducted to study the effects of poplar-bark biochar (PBC600) and thiourea-modified poplar-bark biochar (TPBC600) on Cd speciation and availability, as well as on soil properties. Our results showed that the addition of biochar had a significant influence on soil properties. In the presence of TPBC600, the acid-soluble and reducible Cd fractions were transformed into oxidizable and residual Cd fractions. This process effectively reduced Cd bioavailability in the soil system. Compared to PBC600, TPBC600 was more effective in improving soil pH, electrical conductivity (EC), organic matter (SOM), total nitrogen (TN), ammonium nitrogen (NH4+-N), nitrate nitrogen (NO3--N), available potassium (AK), available phosphorus (AP), and available sulfur (AS). However, this improvement diminished as incubation time increased. Results of Pearson correlation analysis, multivariate linear regression analysis, and principal component analysis showed that soil pH and available phosphorus played key roles in reducing the available cadmium in soil. Therefore, TPBC600 was shown to be an effective modifier that could be used in the remediation of soil polluted with Cd.</div></front></TEI><pubmed><MedlineCitation Status="In-Data-Review" Owner="NLM"><PMID Version="1">33092212</PMID><DateRevised><Year>2020</Year><Month>10</Month><Day>30</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">1660-4601</ISSN><JournalIssue CitedMedium="Internet"><Volume>17</Volume><Issue>20</Issue><PubDate><Year>2020</Year><Month>Oct</Month><Day>20</Day></PubDate></JournalIssue><Title>International journal of environmental research and public health</Title><ISOAbbreviation>Int J Environ Res Public Health</ISOAbbreviation></Journal><ArticleTitle>Remediation of Soil Polluted with Cd in a Postmining Area Using Thiourea-Modified Biochar.</ArticleTitle><ELocationID EIdType="pii" ValidYN="Y">E7654</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.3390/ijerph17207654</ELocationID><Abstract><AbstractText>Cadmium presence in soil is considered a significant threat to human health. Biochar is recognized as an effective method to immobilize Cd ions in different soils. However, obtaining effective and viable biochar to remove elevated Cd from postmining soil remains a challenge. More modifiers need to be explored to improve biochar remediation capacity. In this investigation, pot experiments were conducted to study the effects of poplar-bark biochar (PBC600) and thiourea-modified poplar-bark biochar (TPBC600) on Cd speciation and availability, as well as on soil properties. Our results showed that the addition of biochar had a significant influence on soil properties. In the presence of TPBC600, the acid-soluble and reducible Cd fractions were transformed into oxidizable and residual Cd fractions. This process effectively reduced Cd bioavailability in the soil system. Compared to PBC600, TPBC600 was more effective in improving soil pH, electrical conductivity (EC), organic matter (SOM), total nitrogen (TN), ammonium nitrogen (NH4+-N), nitrate nitrogen (NO3--N), available potassium (AK), available phosphorus (AP), and available sulfur (AS). However, this improvement diminished as incubation time increased. Results of Pearson correlation analysis, multivariate linear regression analysis, and principal component analysis showed that soil pH and available phosphorus played key roles in reducing the available cadmium in soil. Therefore, TPBC600 was shown to be an effective modifier that could be used in the remediation of soil polluted with Cd.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Zhu</LastName><ForeName>Yanfeng</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ma</LastName><ForeName>Jing</ForeName><Initials>J</Initials><Identifier Source="ORCID">0000-0003-1177-1305</Identifier><AffiliationInfo><Affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Chen</LastName><ForeName>Fu</ForeName><Initials>F</Initials><Identifier Source="ORCID">0000-0002-9145-6702</Identifier><AffiliationInfo><Affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Low Carbon Energy Institute, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yu</LastName><ForeName>Ruilian</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Hu</LastName><ForeName>Gongren</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>College of Chemical Engineering, Huaqiao University, Xiamen 361021, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Shaoliang</ForeName><Initials>S</Initials><Identifier Source="ORCID">0000-0002-2063-8218</Identifier><AffiliationInfo><Affiliation>Engineering Research Center of Ministry of Education for Mine Ecological Restoration, China University of Mining and Technology, Xuzhou 221008, Jiangsu, China.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><GrantList CompleteYN="Y"><Grant><GrantID>No. 2017XKZD14</GrantID><Agency>China University of Mining and Technology</Agency><Country></Country></Grant></GrantList><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2020</Year><Month>10</Month><Day>20</Day></ArticleDate></Article><MedlineJournalInfo><Country>Switzerland</Country><MedlineTA>Int J Environ Res Public Health</MedlineTA><NlmUniqueID>101238455</NlmUniqueID><ISSNLinking>1660-4601</ISSNLinking></MedlineJournalInfo><CitationSubset>IM</CitationSubset><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">biochar</Keyword><Keyword MajorTopicYN="N">cadmium</Keyword><Keyword MajorTopicYN="N">immobilization</Keyword><Keyword MajorTopicYN="N">soil</Keyword><Keyword MajorTopicYN="N">thiourea</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2020</Year><Month>09</Month><Day>28</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2020</Year><Month>10</Month><Day>15</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2020</Year><Month>10</Month><Day>18</Day></PubMedPubDate><PubMedPubDate 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IdType="pubmed">28672262</ArticleId></ArticleIdList></Reference></ReferenceList></PubmedData></pubmed><affiliations><list><country><li>République populaire de Chine</li></country></list><tree><country name="République populaire de Chine"><noRegion><name sortKey="Zhu, Yanfeng" sort="Zhu, Yanfeng" uniqKey="Zhu Y" first="Yanfeng" last="Zhu">Yanfeng Zhu</name></noRegion><name sortKey="Chen, Fu" sort="Chen, Fu" uniqKey="Chen F" first="Fu" last="Chen">Fu Chen</name><name sortKey="Chen, Fu" sort="Chen, Fu" uniqKey="Chen F" first="Fu" last="Chen">Fu Chen</name><name sortKey="Hu, Gongren" sort="Hu, Gongren" uniqKey="Hu G" first="Gongren" last="Hu">Gongren Hu</name><name sortKey="Ma, Jing" sort="Ma, Jing" uniqKey="Ma J" first="Jing" last="Ma">Jing Ma</name><name sortKey="Ma, Jing" sort="Ma, Jing" uniqKey="Ma J" first="Jing" last="Ma">Jing Ma</name><name sortKey="Yu, Ruilian" sort="Yu, Ruilian" uniqKey="Yu R" first="Ruilian" last="Yu">Ruilian Yu</name><name sortKey="Zhang, Shaoliang" sort="Zhang, Shaoliang" uniqKey="Zhang S" first="Shaoliang" last="Zhang">Shaoliang Zhang</name><name sortKey="Zhu, Yanfeng" sort="Zhu, Yanfeng" uniqKey="Zhu Y" first="Yanfeng" last="Zhu">Yanfeng Zhu</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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