Catalytic pyrolysis of tire waste: Impacts of biochar catalyst on product evolution.
Identifieur interne : 000146 ( Main/Corpus ); précédent : 000145; suivant : 000147Catalytic pyrolysis of tire waste: Impacts of biochar catalyst on product evolution.
Auteurs : Li Chao ; Chenting Zhang ; Lijun Zhang ; Mortaza Gholizadeh ; Xun HuSource :
- Waste management (New York, N.Y.) [ 1879-2456 ] ; 2020.
English descriptors
- KwdEn :
- MESH :
Abstract
Tire scrap is a solid waste that can be potentially used as the feedstock for the production of liquid fuels via the thermochemical process such as catalytic pyrolysis. Nevertheless, it remains challenging to develop the efficient while cost-effective catalyst for the catalytic pyrolysis of tire. In this study, the pyrolysis of tire scrap at 500 °C with the biochar produced from the gasification of poplar wood at 850 °C were conducted. The biochar catalyst significantly affected the evolution of the volatiles and the char properties, while had a slight impact on the yields of the gas, tar and char products. The biochar catalyst catalyzes the cracking of limonene, a major liquid product in tar, to form significantly more propane in gases and alkanes or alkenes in the tar. In addition, the interaction between the biochar with the oxygen-containing organics promoted the re-condensation reaction, which increased the oxygen content in the char, but the biochar catalyst did not influence the evolution of the aromatics. Additionally, the catalytic pyrolysis also makes the biochar catalyst more oxygen-deficient and more resistant towards oxidation. Concluding all the results showed that biochar, which were produced from the gasification of poplar wood can be a potential catalyst for the pyrolysis of tire.
DOI: 10.1016/j.wasman.2020.07.045
PubMed: 32781409
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pubmed:32781409Le document en format XML
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<author><name sortKey="Chao, Li" sort="Chao, Li" uniqKey="Chao L" first="Li" last="Chao">Li Chao</name>
<affiliation><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation>
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<author><name sortKey="Zhang, Chenting" sort="Zhang, Chenting" uniqKey="Zhang C" first="Chenting" last="Zhang">Chenting Zhang</name>
<affiliation><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation>
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<author><name sortKey="Zhang, Lijun" sort="Zhang, Lijun" uniqKey="Zhang L" first="Lijun" last="Zhang">Lijun Zhang</name>
<affiliation><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation>
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<author><name sortKey="Gholizadeh, Mortaza" sort="Gholizadeh, Mortaza" uniqKey="Gholizadeh M" first="Mortaza" last="Gholizadeh">Mortaza Gholizadeh</name>
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<author><name sortKey="Hu, Xun" sort="Hu, Xun" uniqKey="Hu X" first="Xun" last="Hu">Xun Hu</name>
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<front><div type="abstract" xml:lang="en">Tire scrap is a solid waste that can be potentially used as the feedstock for the production of liquid fuels via the thermochemical process such as catalytic pyrolysis. Nevertheless, it remains challenging to develop the efficient while cost-effective catalyst for the catalytic pyrolysis of tire. In this study, the pyrolysis of tire scrap at 500 °C with the biochar produced from the gasification of poplar wood at 850 °C were conducted. The biochar catalyst significantly affected the evolution of the volatiles and the char properties, while had a slight impact on the yields of the gas, tar and char products. The biochar catalyst catalyzes the cracking of limonene, a major liquid product in tar, to form significantly more propane in gases and alkanes or alkenes in the tar. In addition, the interaction between the biochar with the oxygen-containing organics promoted the re-condensation reaction, which increased the oxygen content in the char, but the biochar catalyst did not influence the evolution of the aromatics. Additionally, the catalytic pyrolysis also makes the biochar catalyst more oxygen-deficient and more resistant towards oxidation. Concluding all the results showed that biochar, which were produced from the gasification of poplar wood can be a potential catalyst for the pyrolysis of tire.</div>
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<Title>Waste management (New York, N.Y.)</Title>
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<ArticleTitle>Catalytic pyrolysis of tire waste: Impacts of biochar catalyst on product evolution.</ArticleTitle>
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<Abstract><AbstractText>Tire scrap is a solid waste that can be potentially used as the feedstock for the production of liquid fuels via the thermochemical process such as catalytic pyrolysis. Nevertheless, it remains challenging to develop the efficient while cost-effective catalyst for the catalytic pyrolysis of tire. In this study, the pyrolysis of tire scrap at 500 °C with the biochar produced from the gasification of poplar wood at 850 °C were conducted. The biochar catalyst significantly affected the evolution of the volatiles and the char properties, while had a slight impact on the yields of the gas, tar and char products. The biochar catalyst catalyzes the cracking of limonene, a major liquid product in tar, to form significantly more propane in gases and alkanes or alkenes in the tar. In addition, the interaction between the biochar with the oxygen-containing organics promoted the re-condensation reaction, which increased the oxygen content in the char, but the biochar catalyst did not influence the evolution of the aromatics. Additionally, the catalytic pyrolysis also makes the biochar catalyst more oxygen-deficient and more resistant towards oxidation. Concluding all the results showed that biochar, which were produced from the gasification of poplar wood can be a potential catalyst for the pyrolysis of tire.</AbstractText>
<CopyrightInformation>Copyright © 2020 Elsevier Ltd. All rights reserved.</CopyrightInformation>
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<AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Chao</LastName>
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<Keyword MajorTopicYN="N">Distribution of the pyrolysis products</Keyword>
<Keyword MajorTopicYN="N">Interaction</Keyword>
<Keyword MajorTopicYN="N">Tire waste</Keyword>
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<CoiStatement>Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.</CoiStatement>
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