Orange Peel Oxidative Gasification on Ni Catalysts Promoted with CaO, CeO2 or K2O.
Identifieur interne : 000144 ( PubMed/Checkpoint ); précédent : 000143; suivant : 000145Orange Peel Oxidative Gasification on Ni Catalysts Promoted with CaO, CeO2 or K2O.
Auteurs : G. Vargas ; B. Zapata ; M A Valenzuela ; S. AlfaroSource :
- Journal of nanoscience and nanotechnology [ 1533-4880 ] ; 2015.
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Gases, Nickel, Oxides.
- chemical : Cerium, Ethylenes, Hydrogen.
- chemistry : Citrus sinensis.
- Biomass, Catalysis, Hot Temperature, Oxidation-Reduction, Thermogravimetry.
Abstract
Orange peel can be considered as an attractive raw material to be gasified for hydrogen or syngas production. In this work, the catalytic evaluation of several silica-supported nickel catalysts in the oxidative degradation of waste orange peel is reported. It was found that the catalytic gasification with the K2O-Ni/silica catalyst produces more hydrogen than the non-catalytic route at 600 degrees C. Surprisingly, a significant amount of ethene was obtained with the CeO2-Ni/silica catalyst, which was explained in terms of an oxidative dehydrogenation reaction of ethane formed during biomass or tar decomposition.
PubMed: 26716225
Affiliations:
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Alfaro</name></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2015">2015</date><idno type="RBID">pubmed:26716225</idno><idno type="pmid">26716225</idno><idno type="wicri:Area/PubMed/Corpus">000137</idno><idno type="wicri:Area/PubMed/Curation">000137</idno><idno type="wicri:Area/PubMed/Checkpoint">000137</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Orange Peel Oxidative Gasification on Ni Catalysts Promoted with CaO, CeO2 or K2O.</title><author><name sortKey="Vargas, G" sort="Vargas, G" uniqKey="Vargas G" first="G" last="Vargas">G. Vargas</name></author><author><name sortKey="Zapata, B" sort="Zapata, B" uniqKey="Zapata B" first="B" last="Zapata">B. Zapata</name></author><author><name sortKey="Valenzuela, M A" sort="Valenzuela, M A" uniqKey="Valenzuela M" first="M A" last="Valenzuela">M A Valenzuela</name></author><author><name sortKey="Alfaro, S" sort="Alfaro, S" uniqKey="Alfaro S" first="S" last="Alfaro">S. Alfaro</name></author></analytic><series><title level="j">Journal of nanoscience and nanotechnology</title><idno type="ISSN">1533-4880</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Biomass</term><term>Catalysis</term><term>Cerium</term><term>Citrus sinensis (chemistry)</term><term>Ethylenes</term><term>Gases (chemistry)</term><term>Hot Temperature</term><term>Hydrogen</term><term>Nickel (chemistry)</term><term>Oxidation-Reduction</term><term>Oxides (chemistry)</term><term>Thermogravimetry</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Gases</term><term>Nickel</term><term>Oxides</term></keywords><keywords scheme="MESH" type="chemical" xml:lang="en"><term>Cerium</term><term>Ethylenes</term><term>Hydrogen</term></keywords><keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Citrus sinensis</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Biomass</term><term>Catalysis</term><term>Hot Temperature</term><term>Oxidation-Reduction</term><term>Thermogravimetry</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Orange peel can be considered as an attractive raw material to be gasified for hydrogen or syngas production. In this work, the catalytic evaluation of several silica-supported nickel catalysts in the oxidative degradation of waste orange peel is reported. It was found that the catalytic gasification with the K2O-Ni/silica catalyst produces more hydrogen than the non-catalytic route at 600 degrees C. Surprisingly, a significant amount of ethene was obtained with the CeO2-Ni/silica catalyst, which was explained in terms of an oxidative dehydrogenation reaction of ethane formed during biomass or tar decomposition.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">26716225</PMID><DateCreated><Year>2015</Year><Month>12</Month><Day>30</Day></DateCreated><DateCompleted><Year>2016</Year><Month>04</Month><Day>08</Day></DateCompleted><DateRevised><Year>2015</Year><Month>12</Month><Day>30</Day></DateRevised><Article PubModel="Print"><Journal><ISSN IssnType="Print">1533-4880</ISSN><JournalIssue CitedMedium="Print"><Volume>15</Volume><Issue>9</Issue><PubDate><Year>2015</Year><Month>Sep</Month></PubDate></JournalIssue><Title>Journal of nanoscience and nanotechnology</Title><ISOAbbreviation>J Nanosci Nanotechnol</ISOAbbreviation></Journal><ArticleTitle>Orange Peel Oxidative Gasification on Ni Catalysts Promoted with CaO, CeO2 or K2O.</ArticleTitle><Pagination><MedlinePgn>6663-8</MedlinePgn></Pagination><Abstract><AbstractText>Orange peel can be considered as an attractive raw material to be gasified for hydrogen or syngas production. In this work, the catalytic evaluation of several silica-supported nickel catalysts in the oxidative degradation of waste orange peel is reported. It was found that the catalytic gasification with the K2O-Ni/silica catalyst produces more hydrogen than the non-catalytic route at 600 degrees C. Surprisingly, a significant amount of ethene was obtained with the CeO2-Ni/silica catalyst, which was explained in terms of an oxidative dehydrogenation reaction of ethane formed during biomass or tar decomposition.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Vargas</LastName><ForeName>G</ForeName><Initials>G</Initials></Author><Author ValidYN="Y"><LastName>Zapata</LastName><ForeName>B</ForeName><Initials>B</Initials></Author><Author ValidYN="Y"><LastName>Valenzuela</LastName><ForeName>M A</ForeName><Initials>MA</Initials></Author><Author ValidYN="Y"><LastName>Alfaro</LastName><ForeName>S</ForeName><Initials>S</Initials></Author></AuthorList><Language>ENG</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>J Nanosci Nanotechnol</MedlineTA><NlmUniqueID>101088195</NlmUniqueID><ISSNLinking>1533-4880</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D005030">Ethylenes</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D005740">Gases</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D010087">Oxides</NameOfSubstance></Chemical><Chemical><RegistryNumber>30K4522N6T</RegistryNumber><NameOfSubstance UI="D002563">Cerium</NameOfSubstance></Chemical><Chemical><RegistryNumber>619G5K328Y</RegistryNumber><NameOfSubstance UI="C030583">ceric oxide</NameOfSubstance></Chemical><Chemical><RegistryNumber>7OV03QG267</RegistryNumber><NameOfSubstance UI="D009532">Nickel</NameOfSubstance></Chemical><Chemical><RegistryNumber>7YNJ3PO35Z</RegistryNumber><NameOfSubstance UI="D006859">Hydrogen</NameOfSubstance></Chemical><Chemical><RegistryNumber>91GW059KN7</RegistryNumber><NameOfSubstance UI="C036216">ethylene</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D018533" MajorTopicYN="Y">Biomass</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002384" MajorTopicYN="N">Catalysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002563" MajorTopicYN="N">Cerium</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D032084" MajorTopicYN="N">Citrus sinensis</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D005030" MajorTopicYN="N">Ethylenes</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D005740" MajorTopicYN="N">Gases</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D006358" MajorTopicYN="N">Hot Temperature</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D006859" MajorTopicYN="N">Hydrogen</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D009532" MajorTopicYN="N">Nickel</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D010084" MajorTopicYN="N">Oxidation-Reduction</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010087" MajorTopicYN="N">Oxides</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D013818" MajorTopicYN="N">Thermogravimetry</DescriptorName></MeshHeading></MeshHeadingList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2015</Year><Month>12</Month><Day>31</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2015</Year><Month>12</Month><Day>31</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2016</Year><Month>4</Month><Day>9</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">26716225</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list></list><tree><noCountry><name sortKey="Alfaro, S" sort="Alfaro, S" uniqKey="Alfaro S" first="S" last="Alfaro">S. Alfaro</name><name sortKey="Valenzuela, M A" sort="Valenzuela, M A" uniqKey="Valenzuela M" first="M A" last="Valenzuela">M A Valenzuela</name><name sortKey="Vargas, G" sort="Vargas, G" uniqKey="Vargas G" first="G" last="Vargas">G. Vargas</name><name sortKey="Zapata, B" sort="Zapata, B" uniqKey="Zapata B" first="B" last="Zapata">B. Zapata</name></noCountry></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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