High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States.
Identifieur interne : 001393 ( PubMed/Curation ); précédent : 001392; suivant : 001394High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States.
Auteurs : Thibault Chervy [France] ; Jialiang Xu [République populaire de Chine] ; Yulong Duan [Pays-Bas] ; Chunliang Wang [France] ; Loïc Mager [France] ; Maurice Frerejean [Pays-Bas] ; Joris A W. Münninghoff [Pays-Bas] ; Paul Tinnemans [Pays-Bas] ; James A. Hutchison [France] ; Cyriaque Genet [France] ; Alan E. Rowan [Pays-Bas] ; Theo Rasing [Pays-Bas] ; Thomas W. Ebbesen [France]Source :
- Nano letters [ 1530-6992 ] ; 2016.
Abstract
We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.
DOI: 10.1021/acs.nanolett.6b02567
PubMed: 27960510
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Münninghoff</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen</wicri:regionArea></affiliation></author><author><name sortKey="Tinnemans, Paul" sort="Tinnemans, Paul" uniqKey="Tinnemans P" first="Paul" last="Tinnemans">Paul Tinnemans</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen</wicri:regionArea></affiliation></author><author><name sortKey="Hutchison, James A" sort="Hutchison, James A" uniqKey="Hutchison J" first="James A" last="Hutchison">James A. Hutchison</name><affiliation wicri:level="1"><nlm:affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg</wicri:regionArea></affiliation></author><author><name sortKey="Genet, Cyriaque" sort="Genet, Cyriaque" uniqKey="Genet C" first="Cyriaque" last="Genet">Cyriaque Genet</name><affiliation wicri:level="1"><nlm:affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg</wicri:regionArea></affiliation></author><author><name sortKey="Rowan, Alan E" sort="Rowan, Alan E" uniqKey="Rowan A" first="Alan E" last="Rowan">Alan E. Rowan</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen</wicri:regionArea></affiliation></author><author><name sortKey="Rasing, Theo" sort="Rasing, Theo" uniqKey="Rasing T" first="Theo" last="Rasing">Theo Rasing</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen</wicri:regionArea></affiliation></author><author><name sortKey="Ebbesen, Thomas W" sort="Ebbesen, Thomas W" uniqKey="Ebbesen T" first="Thomas W" last="Ebbesen">Thomas W. Ebbesen</name><affiliation wicri:level="1"><nlm:affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg</wicri:regionArea></affiliation></author></analytic><series><title level="j">Nano letters</title><idno type="eISSN">1530-6992</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.</div></front></TEI><pubmed><MedlineCitation Status="In-Data-Review" Owner="NLM"><PMID Version="1">27960510</PMID><DateCreated><Year>2016</Year><Month>12</Month><Day>14</Day></DateCreated><DateRevised><Year>2016</Year><Month>12</Month><Day>15</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1530-6992</ISSN><JournalIssue CitedMedium="Internet"><Volume>16</Volume><Issue>12</Issue><PubDate><Year>2016</Year><Month>Dec</Month><Day>14</Day></PubDate></JournalIssue><Title>Nano letters</Title><ISOAbbreviation>Nano Lett.</ISOAbbreviation></Journal><ArticleTitle>High-Efficiency Second-Harmonic Generation from Hybrid Light-Matter States.</ArticleTitle><Pagination><MedlinePgn>7352-7356</MedlinePgn></Pagination><Abstract><AbstractText>We report a novel approach to modify the second order nonlinear optical (NLO) susceptibility of organic nanofiber crystals by hybridization with the optical modes of microcavities in the strong coupling regime. The wavelength dependence of the SHG efficiency displays two intense peaks corresponding to the so-formed light-matter hybrid states. Our results demonstrate an enhancement of the resonant SHG efficiency of the lower polariton by 2 orders of magnitude for the collectively coupled molecules as compared to that of the same material outside the microcavity. This study is a proof of principle that opens a new direction for NLO of organic materials in subwavelength resonators.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Chervy</LastName><ForeName>Thibault</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Xu</LastName><ForeName>Jialiang</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>School of Chemical Engineering and Technology, Tianjin University , Yaguan Road 135, 300350 Tianjin, People's Republic of China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Duan</LastName><ForeName>Yulong</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Chunliang</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Mager</LastName><ForeName>Loïc</ForeName><Initials>L</Initials><AffiliationInfo><Affiliation>IPCMS, University of Strasbourg and CNRS , 23 rue du Loess, 67034 Strasbourg, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Frerejean</LastName><ForeName>Maurice</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Münninghoff</LastName><ForeName>Joris A W</ForeName><Initials>JA</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tinnemans</LastName><ForeName>Paul</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Hutchison</LastName><ForeName>James A</ForeName><Initials>JA</Initials><AffiliationInfo><Affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Genet</LastName><ForeName>Cyriaque</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Rowan</LastName><ForeName>Alan E</ForeName><Initials>AE</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Australian Institute for Bioengineering and Nanotechnology (AIBN), The University of Queensland , Brisbane, Queensland 4072, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Rasing</LastName><ForeName>Theo</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Institute for Molecules and Materials (IMM), Radboud University , Heyendaalseweg 135, 6525AJ Nijmegen, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ebbesen</LastName><ForeName>Thomas W</ForeName><Initials>TW</Initials><AffiliationInfo><Affiliation>ISIS and icFRC, University of Strasbourg and CNRS , 8 allée Gaspard Monge, 67000 Strasbourg, France.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>11</Month><Day>21</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>Nano Lett</MedlineTA><NlmUniqueID>101088070</NlmUniqueID><ISSNLinking>1530-6984</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Second harmonic generation</Keyword><Keyword MajorTopicYN="N">cavity</Keyword><Keyword MajorTopicYN="N">polariton state</Keyword><Keyword MajorTopicYN="N">self-assembly</Keyword><Keyword MajorTopicYN="N">strong coupling</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2016</Year><Month>12</Month><Day>15</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2016</Year><Month>12</Month><Day>15</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2016</Year><Month>12</Month><Day>15</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">27960510</ArticleId><ArticleId IdType="doi">10.1021/acs.nanolett.6b02567</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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