High and Stable Ionic Conductivity in 2D Nanofluidic Ion Channels between Boron Nitride Layers.
Identifieur interne : 000D02 ( PubMed/Curation ); précédent : 000D01; suivant : 000D03High and Stable Ionic Conductivity in 2D Nanofluidic Ion Channels between Boron Nitride Layers.
Auteurs : Si Qin [Australie] ; Dan Liu [Australie] ; Guang Wang [Australie] ; David Portehault [France] ; Christopher J. Garvey [Australie] ; Yury Gogotsi [États-Unis] ; Weiwei Lei [Australie] ; Ying Chen [Australie]Source :
- Journal of the American Chemical Society [ 1520-5126 ] ; 2017.
Abstract
Achieving a high rate of ionic transport through porous membranes and ionic channels is important in numerous applications ranging from energy storage to water desalination, but it still remains a challenge. Herein we show that ions can quickly pass through interlayer spaces in hydrated boron nitride (BN) membranes. Measurements of surface-charge governed ionic currents between BN nanosheets in a variety of salt solutions (KCl, NaCl and CaCl2) at low salt concentrations (<10(-4) M) showed several orders of magnitude higher ionic conductivity compared to that of the bulk solution. Moreover, due to the outstanding chemical and thermal stability of BN, the ionic conduits remain fully functional at temperatures up to 90 °C. The BN conduits can operate in acidic and basic environments and do not degrade after immersing in solutions with extreme pH (pH ∼ 0 or 14) for 1 week. Those excellent properties make the BN ionic conduits attractive for applications in nanofluidic devices and membrane separation.
DOI: 10.1021/jacs.6b11100
PubMed: 28418247
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Garvey</name><affiliation wicri:level="1"><nlm:affiliation>Australia Nuclear Science and Technology Organization (ANSTO) , Sydney, New South Wales 2232, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>Australia Nuclear Science and Technology Organization (ANSTO) , Sydney, New South Wales 2232</wicri:regionArea></affiliation></author><author><name sortKey="Gogotsi, Yury" sort="Gogotsi, Yury" uniqKey="Gogotsi Y" first="Yury" last="Gogotsi">Yury Gogotsi</name><affiliation wicri:level="1"><nlm:affiliation>A. J. Drexel Nanomaterials Institute and Materials Science and Engineering Department, Drexel University , 3141 Chestnut Street, Philadelphia, Pennsylvania 19104, United States.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>A. J. Drexel Nanomaterials Institute and Materials Science and Engineering Department, Drexel University , 3141 Chestnut Street, Philadelphia, Pennsylvania 19104</wicri:regionArea></affiliation></author><author><name sortKey="Lei, Weiwei" sort="Lei, Weiwei" uniqKey="Lei W" first="Weiwei" last="Lei">Weiwei Lei</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216</wicri:regionArea></affiliation></author><author><name sortKey="Chen, Ying" sort="Chen, Ying" uniqKey="Chen Y" first="Ying" last="Chen">Ying Chen</name><affiliation wicri:level="1"><nlm:affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216</wicri:regionArea></affiliation></author></analytic><series><title level="j">Journal of the American Chemical Society</title><idno type="eISSN">1520-5126</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Achieving a high rate of ionic transport through porous membranes and ionic channels is important in numerous applications ranging from energy storage to water desalination, but it still remains a challenge. Herein we show that ions can quickly pass through interlayer spaces in hydrated boron nitride (BN) membranes. Measurements of surface-charge governed ionic currents between BN nanosheets in a variety of salt solutions (KCl, NaCl and CaCl2) at low salt concentrations (<10(-4) M) showed several orders of magnitude higher ionic conductivity compared to that of the bulk solution. Moreover, due to the outstanding chemical and thermal stability of BN, the ionic conduits remain fully functional at temperatures up to 90 °C. The BN conduits can operate in acidic and basic environments and do not degrade after immersing in solutions with extreme pH (pH ∼ 0 or 14) for 1 week. Those excellent properties make the BN ionic conduits attractive for applications in nanofluidic devices and membrane separation.</div></front></TEI><pubmed><MedlineCitation Status="In-Data-Review" Owner="NLM"><PMID Version="1">28418247</PMID><DateCreated><Year>2017</Year><Month>04</Month><Day>18</Day></DateCreated><DateRevised><Year>2017</Year><Month>05</Month><Day>10</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1520-5126</ISSN><JournalIssue CitedMedium="Internet"><Volume>139</Volume><Issue>18</Issue><PubDate><Year>2017</Year><Month>May</Month><Day>10</Day></PubDate></JournalIssue><Title>Journal of the American Chemical Society</Title><ISOAbbreviation>J. Am. Chem. Soc.</ISOAbbreviation></Journal><ArticleTitle>High and Stable Ionic Conductivity in 2D Nanofluidic Ion Channels between Boron Nitride Layers.</ArticleTitle><Pagination><MedlinePgn>6314-6320</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/jacs.6b11100</ELocationID><Abstract><AbstractText>Achieving a high rate of ionic transport through porous membranes and ionic channels is important in numerous applications ranging from energy storage to water desalination, but it still remains a challenge. Herein we show that ions can quickly pass through interlayer spaces in hydrated boron nitride (BN) membranes. Measurements of surface-charge governed ionic currents between BN nanosheets in a variety of salt solutions (KCl, NaCl and CaCl2) at low salt concentrations (<10(-4) M) showed several orders of magnitude higher ionic conductivity compared to that of the bulk solution. Moreover, due to the outstanding chemical and thermal stability of BN, the ionic conduits remain fully functional at temperatures up to 90 °C. The BN conduits can operate in acidic and basic environments and do not degrade after immersing in solutions with extreme pH (pH ∼ 0 or 14) for 1 week. Those excellent properties make the BN ionic conduits attractive for applications in nanofluidic devices and membrane separation.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Qin</LastName><ForeName>Si</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Dan</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Guang</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Portehault</LastName><ForeName>David</ForeName><Initials>D</Initials><Identifier Source="ORCID">http://orcid.org/0000-0003-4914-4913</Identifier><AffiliationInfo><Affiliation>Sorbonne Universités, UPMC Université Paris 06, CNRS, Collège de France, Laboratoire de Chimie de la Matière Condensée de Paris (LCMCP), 11 place Marcelin Berthelot, F-75005 Paris, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Garvey</LastName><ForeName>Christopher J</ForeName><Initials>CJ</Initials><AffiliationInfo><Affiliation>Australia Nuclear Science and Technology Organization (ANSTO) , Sydney, New South Wales 2232, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Gogotsi</LastName><ForeName>Yury</ForeName><Initials>Y</Initials><Identifier Source="ORCID">http://orcid.org/0000-0001-9423-4032</Identifier><AffiliationInfo><Affiliation>A. J. Drexel Nanomaterials Institute and Materials Science and Engineering Department, Drexel University , 3141 Chestnut Street, Philadelphia, Pennsylvania 19104, United States.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lei</LastName><ForeName>Weiwei</ForeName><Initials>W</Initials><Identifier Source="ORCID">http://orcid.org/0000-0003-2698-299X</Identifier><AffiliationInfo><Affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Chen</LastName><ForeName>Ying</ForeName><Initials>Y</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-7322-2224</Identifier><AffiliationInfo><Affiliation>Institute for Frontier Materials (IFM), Deakin University , 75 Pigdons Road, Waurn Ponds, Victoria 3216, Australia.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>05</Month><Day>01</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>J Am Chem Soc</MedlineTA><NlmUniqueID>7503056</NlmUniqueID><ISSNLinking>0002-7863</ISSNLinking></MedlineJournalInfo></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="pubmed"><Year>2017</Year><Month>4</Month><Day>19</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2017</Year><Month>4</Month><Day>19</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2017</Year><Month>4</Month><Day>19</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">28418247</ArticleId><ArticleId IdType="doi">10.1021/jacs.6b11100</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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