Ferrotoroidic ground state in a heterometallic {Cr(III)Dy(III)6} complex displaying slow magnetic relaxation.
Identifieur interne : 000368 ( PubMed/Curation ); précédent : 000367; suivant : 000369Ferrotoroidic ground state in a heterometallic {Cr(III)Dy(III)6} complex displaying slow magnetic relaxation.
Auteurs : Kuduva R. Vignesh [Inde] ; Alessandro Soncini [Australie] ; Stuart K. Langley [Royaume-Uni] ; Wolfgang Wernsdorfer [Allemagne] ; Keith S. Murray [Australie] ; Gopalan Rajaraman [Inde]Source :
- Nature communications [ 2041-1723 ] ; 2017.
Abstract
Toroidal quantum states are most promising for building quantum computing and information storage devices, as they are insensitive to homogeneous magnetic fields, but interact with charge and spin currents, allowing this moment to be manipulated purely by electrical means. Coupling molecular toroids into larger toroidal moments via ferrotoroidic interactions can be pivotal not only to enhance ground state toroidicity, but also to develop materials displaying ferrotoroidic ordered phases, which sustain linear magneto-electric coupling and multiferroic behavior. However, engineering ferrotoroidic coupling is known to be a challenging task. Here we have isolated a {Cr(III)Dy(III)6} complex that exhibits the much sought-after ferrotoroidic ground state with an enhanced toroidal moment, solely arising from intramolecular dipolar interactions. Moreover, a theoretical analysis of the observed sub-Kelvin zero-field hysteretic spin dynamics of {Cr(III)Dy(III)6} reveals the pivotal role played by ferrotoroidic states in slowing down the magnetic relaxation, in spite of large calculated single-ion quantum tunneling rates.
DOI: 10.1038/s41467-017-01102-5
PubMed: 29044098
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Coupling molecular toroids into larger toroidal moments via ferrotoroidic interactions can be pivotal not only to enhance ground state toroidicity, but also to develop materials displaying ferrotoroidic ordered phases, which sustain linear magneto-electric coupling and multiferroic behavior. However, engineering ferrotoroidic coupling is known to be a challenging task. Here we have isolated a {Cr(III)Dy(III)6} complex that exhibits the much sought-after ferrotoroidic ground state with an enhanced toroidal moment, solely arising from intramolecular dipolar interactions. Moreover, a theoretical analysis of the observed sub-Kelvin zero-field hysteretic spin dynamics of {Cr(III)Dy(III)6} reveals the pivotal role played by ferrotoroidic states in slowing down the magnetic relaxation, in spite of large calculated single-ion quantum tunneling rates.</div></front></TEI><pubmed><MedlineCitation Status="In-Data-Review" Owner="NLM"><PMID Version="1">29044098</PMID><DateCreated><Year>2017</Year><Month>10</Month><Day>18</Day></DateCreated><DateRevised><Year>2017</Year><Month>10</Month><Day>22</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">2041-1723</ISSN><JournalIssue CitedMedium="Internet"><Volume>8</Volume><Issue>1</Issue><PubDate><Year>2017</Year><Month>Oct</Month><Day>18</Day></PubDate></JournalIssue><Title>Nature communications</Title><ISOAbbreviation>Nat Commun</ISOAbbreviation></Journal><ArticleTitle>Ferrotoroidic ground state in a heterometallic {Cr(III)Dy(III)6} complex displaying slow magnetic relaxation.</ArticleTitle><Pagination><MedlinePgn>1023</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1038/s41467-017-01102-5</ELocationID><Abstract><AbstractText>Toroidal quantum states are most promising for building quantum computing and information storage devices, as they are insensitive to homogeneous magnetic fields, but interact with charge and spin currents, allowing this moment to be manipulated purely by electrical means. Coupling molecular toroids into larger toroidal moments via ferrotoroidic interactions can be pivotal not only to enhance ground state toroidicity, but also to develop materials displaying ferrotoroidic ordered phases, which sustain linear magneto-electric coupling and multiferroic behavior. However, engineering ferrotoroidic coupling is known to be a challenging task. Here we have isolated a {Cr(III)Dy(III)6} complex that exhibits the much sought-after ferrotoroidic ground state with an enhanced toroidal moment, solely arising from intramolecular dipolar interactions. Moreover, a theoretical analysis of the observed sub-Kelvin zero-field hysteretic spin dynamics of {Cr(III)Dy(III)6} reveals the pivotal role played by ferrotoroidic states in slowing down the magnetic relaxation, in spite of large calculated single-ion quantum tunneling rates.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Vignesh</LastName><ForeName>Kuduva R</ForeName><Initials>KR</Initials><AffiliationInfo><Affiliation>IITB-Monash Research Academy, IIT Bombay, Mumbai, 400076, India.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Soncini</LastName><ForeName>Alessandro</ForeName><Initials>A</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-6779-7304</Identifier><AffiliationInfo><Affiliation>School of Chemistry, University of Melbourne, Melbourne, VIC, 3010, Australia. asoncini@unimelb.edu.au.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Langley</LastName><ForeName>Stuart K</ForeName><Initials>SK</Initials><AffiliationInfo><Affiliation>School of Science and the Environment, Division of Chemistry, Manchester Metropolitan University, Manchester, M15 6BH, UK.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wernsdorfer</LastName><ForeName>Wolfgang</ForeName><Initials>W</Initials><AffiliationInfo><Affiliation>Institute Neel, CNRS, F-38000 Grenoble, France and Institute of Nanotechnology, Karlsruhe Institute of Technology, 76344, Eggenstein-Leopoldshafen, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Murray</LastName><ForeName>Keith S</ForeName><Initials>KS</Initials><AffiliationInfo><Affiliation>School of Chemistry, Monash University, Melbourne, VIC, 3800, Australia. keith.murray@monash.edu.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Rajaraman</LastName><ForeName>Gopalan</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Indian Institute of Technology Bombay, Mumbai, 400076, India. rajaraman@chem.iitb.ac.in.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>10</Month><Day>18</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Nat Commun</MedlineTA><NlmUniqueID>101528555</NlmUniqueID><ISSNLinking>2041-1723</ISSNLinking></MedlineJournalInfo><CommentsCorrectionsList><CommentsCorrections RefType="Cites"><RefSource>Phys Rev Lett. 2008 Jun 20;100(24):247205</RefSource><PMID Version="1">18643625</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Inorg Chem. 2010 Dec 20;49(24):11587-94</RefSource><PMID Version="1">21070004</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Science. 2010 Dec 10;330(6010):1510-2</RefSource><PMID 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