Hydrophilic Organic Electrodes on Flexible Hydrogels.
Identifieur interne : 002392 ( PubMed/Corpus ); précédent : 002391; suivant : 002393Hydrophilic Organic Electrodes on Flexible Hydrogels.
Auteurs : Thierry Moser ; Coralie Celma ; Audrey Lebert ; Eric Charrault ; Robert Brooke ; Peter J. Murphy ; Gareth Browne ; Richard Young ; Timothy Higgs ; Drew EvansSource :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2016.
English descriptors
- KwdEn :
- MESH :
Abstract
Prompted by the rapidly developing field of wearable electronics, research into biocompatible substrates and coatings is intensifying. Acrylate-based hydrogel polymers have gained widespread use as biocompatible articles in applications such as contact and intraocular lenses. Surface treatments and/or coatings present one strategy to further enhance the performance of these hydrogels or even realize novel functionality. In this study, the conductive polymer poly(3,4-ethylenedioxythiophene) (PEDOT) is deposited from the vapor phase onto hydrated hydrogel substrates and blended with biocompatibilizing coconstituents incorporating polyethylene glycol (PEG) and polydimethyl siloxane (PDMS) moieties. Plasma pretreatment of the dehydrated hydrogel substrate modifies its surface topography and chemical composition to facilitate the attachment of conductive PEDOT-based surface layers. Manipulating the vapor phase polymerization process and constituent composition, the PEDOT-based coating is engineered to be both hydrophilic (i.e. to promote biocompatibility) and highly conductive. The fabrication of this conductively coated hydrogel has implications for the future of wearable electronic devices.
DOI: 10.1021/acsami.5b10831
PubMed: 26698297
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Murphy</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Browne, Gareth" sort="Browne, Gareth" uniqKey="Browne G" first="Gareth" last="Browne">Gareth Browne</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Young, Richard" sort="Young, Richard" uniqKey="Young R" first="Richard" last="Young">Richard Young</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Higgs, Timothy" sort="Higgs, Timothy" uniqKey="Higgs T" first="Timothy" last="Higgs">Timothy Higgs</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Evans, Drew" sort="Evans, Drew" uniqKey="Evans D" first="Drew" last="Evans">Drew Evans</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2016">2016</date><idno type="RBID">pubmed:26698297</idno><idno type="pmid">26698297</idno><idno type="doi">10.1021/acsami.5b10831</idno><idno type="wicri:Area/PubMed/Corpus">002392</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">002392</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Hydrophilic Organic Electrodes on Flexible Hydrogels.</title><author><name sortKey="Moser, Thierry" sort="Moser, Thierry" uniqKey="Moser T" first="Thierry" last="Moser">Thierry Moser</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Celma, Coralie" sort="Celma, Coralie" uniqKey="Celma C" first="Coralie" last="Celma">Coralie Celma</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Lebert, Audrey" sort="Lebert, Audrey" uniqKey="Lebert A" first="Audrey" last="Lebert">Audrey Lebert</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Charrault, Eric" sort="Charrault, Eric" uniqKey="Charrault E" first="Eric" last="Charrault">Eric Charrault</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Brooke, Robert" sort="Brooke, Robert" uniqKey="Brooke R" first="Robert" last="Brooke">Robert Brooke</name><affiliation><nlm:affiliation>Department of Science and Technology, Laboratory of Organic Electronics, Linkoping University , SE-601 74 Norrkoping, Sweden.</nlm:affiliation></affiliation></author><author><name sortKey="Murphy, Peter J" sort="Murphy, Peter J" uniqKey="Murphy P" first="Peter J" last="Murphy">Peter J. Murphy</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Browne, Gareth" sort="Browne, Gareth" uniqKey="Browne G" first="Gareth" last="Browne">Gareth Browne</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Young, Richard" sort="Young, Richard" uniqKey="Young R" first="Richard" last="Young">Richard Young</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Higgs, Timothy" sort="Higgs, Timothy" uniqKey="Higgs T" first="Timothy" last="Higgs">Timothy Higgs</name><affiliation><nlm:affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</nlm:affiliation></affiliation></author><author><name sortKey="Evans, Drew" sort="Evans, Drew" uniqKey="Evans D" first="Drew" last="Evans">Drew Evans</name><affiliation><nlm:affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</nlm:affiliation></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Bridged Bicyclo Compounds, Heterocyclic (chemistry)</term><term>Dimethylpolysiloxanes (chemistry)</term><term>Electric Conductivity</term><term>Electrodes</term><term>Hydrogels (chemistry)</term><term>Hydrophobic and Hydrophilic Interactions</term><term>Microscopy, Atomic Force</term><term>Plasma Gases (chemistry)</term><term>Polyethylene Glycols (chemistry)</term><term>Polymers (chemistry)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Bridged Bicyclo Compounds, Heterocyclic</term><term>Dimethylpolysiloxanes</term><term>Hydrogels</term><term>Plasma Gases</term><term>Polyethylene Glycols</term><term>Polymers</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Electric Conductivity</term><term>Electrodes</term><term>Hydrophobic and Hydrophilic Interactions</term><term>Microscopy, Atomic Force</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Prompted by the rapidly developing field of wearable electronics, research into biocompatible substrates and coatings is intensifying. Acrylate-based hydrogel polymers have gained widespread use as biocompatible articles in applications such as contact and intraocular lenses. Surface treatments and/or coatings present one strategy to further enhance the performance of these hydrogels or even realize novel functionality. In this study, the conductive polymer poly(3,4-ethylenedioxythiophene) (PEDOT) is deposited from the vapor phase onto hydrated hydrogel substrates and blended with biocompatibilizing coconstituents incorporating polyethylene glycol (PEG) and polydimethyl siloxane (PDMS) moieties. Plasma pretreatment of the dehydrated hydrogel substrate modifies its surface topography and chemical composition to facilitate the attachment of conductive PEDOT-based surface layers. Manipulating the vapor phase polymerization process and constituent composition, the PEDOT-based coating is engineered to be both hydrophilic (i.e. to promote biocompatibility) and highly conductive. The fabrication of this conductively coated hydrogel has implications for the future of wearable electronic devices.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">26698297</PMID><DateCreated><Year>2016</Year><Month>01</Month><Day>13</Day></DateCreated><DateCompleted><Year>2016</Year><Month>10</Month><Day>24</Day></DateCompleted><DateRevised><Year>2017</Year><Month>01</Month><Day>03</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1944-8252</ISSN><JournalIssue CitedMedium="Internet"><Volume>8</Volume><Issue>1</Issue><PubDate><Year>2016</Year><Month>Jan</Month><Day>13</Day></PubDate></JournalIssue><Title>ACS applied materials & interfaces</Title><ISOAbbreviation>ACS Appl Mater Interfaces</ISOAbbreviation></Journal><ArticleTitle>Hydrophilic Organic Electrodes on Flexible Hydrogels.</ArticleTitle><Pagination><MedlinePgn>974-82</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/acsami.5b10831</ELocationID><Abstract><AbstractText>Prompted by the rapidly developing field of wearable electronics, research into biocompatible substrates and coatings is intensifying. Acrylate-based hydrogel polymers have gained widespread use as biocompatible articles in applications such as contact and intraocular lenses. Surface treatments and/or coatings present one strategy to further enhance the performance of these hydrogels or even realize novel functionality. In this study, the conductive polymer poly(3,4-ethylenedioxythiophene) (PEDOT) is deposited from the vapor phase onto hydrated hydrogel substrates and blended with biocompatibilizing coconstituents incorporating polyethylene glycol (PEG) and polydimethyl siloxane (PDMS) moieties. Plasma pretreatment of the dehydrated hydrogel substrate modifies its surface topography and chemical composition to facilitate the attachment of conductive PEDOT-based surface layers. Manipulating the vapor phase polymerization process and constituent composition, the PEDOT-based coating is engineered to be both hydrophilic (i.e. to promote biocompatibility) and highly conductive. The fabrication of this conductively coated hydrogel has implications for the future of wearable electronic devices.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Moser</LastName><ForeName>Thierry</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Department of Materials Science, ETH, Zurich , Wolfgang-Pauli-Strasse 10, 8093 Zurich, Zurich, Switzerland.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Celma</LastName><ForeName>Coralie</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>European School of Chemistry, Polymer and Materials Science, Universite de Strasbourg , Strasbourg F-67087, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lebert</LastName><ForeName>Audrey</ForeName><Initials>A</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>ENSCBP, Polytechnique Institute of Bordeaux , Pessac 33607, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Charrault</LastName><ForeName>Eric</ForeName><Initials>E</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Brooke</LastName><ForeName>Robert</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Department of Science and Technology, Laboratory of Organic Electronics, Linkoping University , SE-601 74 Norrkoping, Sweden.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Murphy</LastName><ForeName>Peter J</ForeName><Initials>PJ</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Browne</LastName><ForeName>Gareth</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Young</LastName><ForeName>Richard</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Higgs</LastName><ForeName>Timothy</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Contamac Limited, Saffron Walden, Essex CB11 3 AU, United Kingdom.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Evans</LastName><ForeName>Drew</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Thin Film Coatings Group, Future Industries Institute, University of South Australia , Mawson Lakes, South Australia 5095, Australia.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>01</Month><Day>04</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Appl Mater Interfaces</MedlineTA><NlmUniqueID>101504991</NlmUniqueID><ISSNLinking>1944-8244</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D019086">Bridged Bicyclo Compounds, Heterocyclic</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D004129">Dimethylpolysiloxanes</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D020100">Hydrogels</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D058626">Plasma Gases</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D011108">Polymers</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="C121383">poly(3,4-ethylene dioxythiophene)</NameOfSubstance></Chemical><Chemical><RegistryNumber>30IQX730WE</RegistryNumber><NameOfSubstance UI="D011092">Polyethylene Glycols</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D019086" MajorTopicYN="N">Bridged Bicyclo Compounds, Heterocyclic</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D004129" MajorTopicYN="N">Dimethylpolysiloxanes</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D004553" MajorTopicYN="N">Electric Conductivity</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D004566" MajorTopicYN="N">Electrodes</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D020100" MajorTopicYN="N">Hydrogels</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D057927" MajorTopicYN="Y">Hydrophobic and Hydrophilic Interactions</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D018625" MajorTopicYN="N">Microscopy, Atomic Force</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D058626" MajorTopicYN="N">Plasma Gases</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D011092" MajorTopicYN="N">Polyethylene Glycols</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D011108" MajorTopicYN="N">Polymers</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">conducting polymers</Keyword><Keyword MajorTopicYN="N">contact lens</Keyword><Keyword MajorTopicYN="N">hydrophilicity</Keyword><Keyword MajorTopicYN="N">plasma treatment</Keyword><Keyword MajorTopicYN="N">vapor phase polymerization</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2015</Year><Month>12</Month><Day>25</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2015</Year><Month>12</Month><Day>25</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2016</Year><Month>10</Month><Day>25</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">26698297</ArticleId><ArticleId IdType="doi">10.1021/acsami.5b10831</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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