Nonlinear magnetoelectric effect in paraelectric state of Co4Nb2O9 single crystal.
Identifieur interne : 000237 ( PubMed/Corpus ); précédent : 000236; suivant : 000238Nonlinear magnetoelectric effect in paraelectric state of Co4Nb2O9 single crystal.
Auteurs : Yiming Cao ; Guochu Deng ; P Emysl Beran ; Zhenjie Feng ; Baojuan Kang ; Jincang Zhang ; Nicolas Guiblin ; Brahim Dkhil ; Wei Ren ; Shixun CaoSource :
- Scientific reports [ 2045-2322 ] ; 2017.
Abstract
We report the structural, magnetoelectric (ME), magnetic and electric control of magnetic properties in Co4Nb2O9 (CNO) single crystal. A detailed ME measurement reveals a nonlinear ME effect instead of a linear ME effect in CNO single crystal. By fitting the magnetization-electric field (M-E) curve, it can be found that the linear ([Formula: see text]) and quadratic (γ) coefficients equal to ~8.27 ps/m and ~-6.46 ps/MV for upper branch, as well as ~8.38 ps/m and ~6.75 ps/MV for the lower branch. More importantly, a pronounced response was observed under a small cooling magnetic field, which cannot even cause the spin flop. This suggests a magnetoelectric effect can occur at paraelectric state for CNO single crystal. Furthermore, we also found that the magnetization of every axis responds to electric field applied along a-axis, but fails to do so when the electric field is applied c-axis. Such findings supply a direct evidence to the magnetic structure and ME coupling mechanism indirectly reflected by our neutron experiment.
DOI: 10.1038/s41598-017-14169-3
PubMed: 29074870
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Nonlinear magnetoelectric effect in paraelectric state of Co4Nb2O9 single crystal.</title><author><name sortKey="Cao, Yiming" sort="Cao, Yiming" uniqKey="Cao Y" first="Yiming" last="Cao">Yiming Cao</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Deng, Guochu" sort="Deng, Guochu" uniqKey="Deng G" first="Guochu" last="Deng">Guochu Deng</name><affiliation><nlm:affiliation>Australian Nuclear Science and Technology Organisation, New Illawarra Road, Lucas Heights, NSW 2234, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Beran, P Emysl" sort="Beran, P Emysl" uniqKey="Beran P" first="P Emysl" last="Beran">P Emysl Beran</name><affiliation><nlm:affiliation>Nuclear Physics Institute CAS, 25068, Rez, Czech Republic.</nlm:affiliation></affiliation></author><author><name sortKey="Feng, Zhenjie" sort="Feng, Zhenjie" uniqKey="Feng Z" first="Zhenjie" last="Feng">Zhenjie Feng</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Kang, Baojuan" sort="Kang, Baojuan" uniqKey="Kang B" first="Baojuan" last="Kang">Baojuan Kang</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Zhang, Jincang" sort="Zhang, Jincang" uniqKey="Zhang J" first="Jincang" last="Zhang">Jincang Zhang</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Guiblin, Nicolas" sort="Guiblin, Nicolas" uniqKey="Guiblin N" first="Nicolas" last="Guiblin">Nicolas Guiblin</name><affiliation><nlm:affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</nlm:affiliation></affiliation></author><author><name sortKey="Dkhil, Brahim" sort="Dkhil, Brahim" uniqKey="Dkhil B" first="Brahim" last="Dkhil">Brahim Dkhil</name><affiliation><nlm:affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</nlm:affiliation></affiliation></author><author><name sortKey="Ren, Wei" sort="Ren, Wei" uniqKey="Ren W" first="Wei" last="Ren">Wei Ren</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Cao, Shixun" sort="Cao, Shixun" uniqKey="Cao S" first="Shixun" last="Cao">Shixun Cao</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China. sxcao@shu.edu.cn.</nlm:affiliation></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2017">2017</date><idno type="RBID">pubmed:29074870</idno><idno type="pmid">29074870</idno><idno type="doi">10.1038/s41598-017-14169-3</idno><idno type="wicri:Area/PubMed/Corpus">000237</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">000237</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Nonlinear magnetoelectric effect in paraelectric state of Co4Nb2O9 single crystal.</title><author><name sortKey="Cao, Yiming" sort="Cao, Yiming" uniqKey="Cao Y" first="Yiming" last="Cao">Yiming Cao</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Deng, Guochu" sort="Deng, Guochu" uniqKey="Deng G" first="Guochu" last="Deng">Guochu Deng</name><affiliation><nlm:affiliation>Australian Nuclear Science and Technology Organisation, New Illawarra Road, Lucas Heights, NSW 2234, Australia.</nlm:affiliation></affiliation></author><author><name sortKey="Beran, P Emysl" sort="Beran, P Emysl" uniqKey="Beran P" first="P Emysl" last="Beran">P Emysl Beran</name><affiliation><nlm:affiliation>Nuclear Physics Institute CAS, 25068, Rez, Czech Republic.</nlm:affiliation></affiliation></author><author><name sortKey="Feng, Zhenjie" sort="Feng, Zhenjie" uniqKey="Feng Z" first="Zhenjie" last="Feng">Zhenjie Feng</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Kang, Baojuan" sort="Kang, Baojuan" uniqKey="Kang B" first="Baojuan" last="Kang">Baojuan Kang</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Zhang, Jincang" sort="Zhang, Jincang" uniqKey="Zhang J" first="Jincang" last="Zhang">Jincang Zhang</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Guiblin, Nicolas" sort="Guiblin, Nicolas" uniqKey="Guiblin N" first="Nicolas" last="Guiblin">Nicolas Guiblin</name><affiliation><nlm:affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</nlm:affiliation></affiliation></author><author><name sortKey="Dkhil, Brahim" sort="Dkhil, Brahim" uniqKey="Dkhil B" first="Brahim" last="Dkhil">Brahim Dkhil</name><affiliation><nlm:affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</nlm:affiliation></affiliation></author><author><name sortKey="Ren, Wei" sort="Ren, Wei" uniqKey="Ren W" first="Wei" last="Ren">Wei Ren</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</nlm:affiliation></affiliation></author><author><name sortKey="Cao, Shixun" sort="Cao, Shixun" uniqKey="Cao S" first="Shixun" last="Cao">Shixun Cao</name><affiliation><nlm:affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China. sxcao@shu.edu.cn.</nlm:affiliation></affiliation></author></analytic><series><title level="j">Scientific reports</title><idno type="eISSN">2045-2322</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We report the structural, magnetoelectric (ME), magnetic and electric control of magnetic properties in Co4Nb2O9 (CNO) single crystal. A detailed ME measurement reveals a nonlinear ME effect instead of a linear ME effect in CNO single crystal. By fitting the magnetization-electric field (M-E) curve, it can be found that the linear ([Formula: see text]) and quadratic (γ) coefficients equal to ~8.27 ps/m and ~-6.46 ps/MV for upper branch, as well as ~8.38 ps/m and ~6.75 ps/MV for the lower branch. More importantly, a pronounced response was observed under a small cooling magnetic field, which cannot even cause the spin flop. This suggests a magnetoelectric effect can occur at paraelectric state for CNO single crystal. Furthermore, we also found that the magnetization of every axis responds to electric field applied along a-axis, but fails to do so when the electric field is applied c-axis. Such findings supply a direct evidence to the magnetic structure and ME coupling mechanism indirectly reflected by our neutron experiment.</div></front></TEI><pubmed><MedlineCitation Status="In-Data-Review" Owner="NLM"><PMID Version="1">29074870</PMID><DateCreated><Year>2017</Year><Month>10</Month><Day>27</Day></DateCreated><DateRevised><Year>2017</Year><Month>11</Month><Day>01</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">2045-2322</ISSN><JournalIssue CitedMedium="Internet"><Volume>7</Volume><Issue>1</Issue><PubDate><Year>2017</Year><Month>Oct</Month><Day>26</Day></PubDate></JournalIssue><Title>Scientific reports</Title><ISOAbbreviation>Sci Rep</ISOAbbreviation></Journal><ArticleTitle>Nonlinear magnetoelectric effect in paraelectric state of Co4Nb2O9 single crystal.</ArticleTitle><Pagination><MedlinePgn>14079</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1038/s41598-017-14169-3</ELocationID><Abstract><AbstractText>We report the structural, magnetoelectric (ME), magnetic and electric control of magnetic properties in Co4Nb2O9 (CNO) single crystal. A detailed ME measurement reveals a nonlinear ME effect instead of a linear ME effect in CNO single crystal. By fitting the magnetization-electric field (M-E) curve, it can be found that the linear ([Formula: see text]) and quadratic (γ) coefficients equal to ~8.27 ps/m and ~-6.46 ps/MV for upper branch, as well as ~8.38 ps/m and ~6.75 ps/MV for the lower branch. More importantly, a pronounced response was observed under a small cooling magnetic field, which cannot even cause the spin flop. This suggests a magnetoelectric effect can occur at paraelectric state for CNO single crystal. Furthermore, we also found that the magnetization of every axis responds to electric field applied along a-axis, but fails to do so when the electric field is applied c-axis. Such findings supply a direct evidence to the magnetic structure and ME coupling mechanism indirectly reflected by our neutron experiment.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Cao</LastName><ForeName>Yiming</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Center for Magnetic Materials and Devices, Key Laboratory for Advanced Functional and Low Dimensional Materials of Yunnan Higher Education Institute, Qujing Normal University, Qujing, 655011, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Deng</LastName><ForeName>Guochu</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Australian Nuclear Science and Technology Organisation, New Illawarra Road, Lucas Heights, NSW 2234, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Beran</LastName><ForeName>Přemysl</ForeName><Initials>P</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-1217-3131</Identifier><AffiliationInfo><Affiliation>Nuclear Physics Institute CAS, 25068, Rez, Czech Republic.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Feng</LastName><ForeName>Zhenjie</ForeName><Initials>Z</Initials><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Kang</LastName><ForeName>Baojuan</ForeName><Initials>B</Initials><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Jincang</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Guiblin</LastName><ForeName>Nicolas</ForeName><Initials>N</Initials><AffiliationInfo><Affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Dkhil</LastName><ForeName>Brahim</ForeName><Initials>B</Initials><AffiliationInfo><Affiliation>Laboratoire Structures, Propriétés et Modélisation des Solides, CentraleSupélec, CNRS-UMR 8580, Université Paris-Saclay, 91192, Gif-sur-Yvette, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ren</LastName><ForeName>Wei</ForeName><Initials>W</Initials><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai, 200444, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Cao</LastName><ForeName>Shixun</ForeName><Initials>S</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-3915-2621</Identifier><AffiliationInfo><Affiliation>Department of Physics, International Center of Quantum and Molecular Structures, and Materials Genome Institute, Shanghai University, Shanghai, 200444, China. sxcao@shu.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai, 200444, China. sxcao@shu.edu.cn.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>10</Month><Day>26</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Sci Rep</MedlineTA><NlmUniqueID>101563288</NlmUniqueID><ISSNLinking>2045-2322</ISSNLinking></MedlineJournalInfo><CommentsCorrectionsList><CommentsCorrections RefType="Cites"><RefSource>Nat Mater. 2007 Jan;6(1):13-20</RefSource><PMID Version="1">17199121</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Sci Rep. 2015 Feb 05;5:8254</RefSource><PMID Version="1">25653008</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Nature. 2006 Aug 17;442(7104):759-65</RefSource><PMID Version="1">16915279</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Sci Rep. 2014 Jan 27;4:3860</RefSource><PMID Version="1">24463631</PMID></CommentsCorrections><CommentsCorrections RefType="Cites"><RefSource>Adv Mater. 2013 Mar 13;25(10):1435-9</RefSource><PMID Version="1">23303469</PMID></CommentsCorrections></CommentsCorrectionsList></MedlineCitation><PubmedData><History><PubMedPubDate 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