Core-shell nanostructured hybrid composites for volatile organic compound detection.
Identifieur interne : 002D72 ( PubMed/Checkpoint ); précédent : 002D71; suivant : 002D73Core-shell nanostructured hybrid composites for volatile organic compound detection.
Auteurs : Tran Thanh Tung [France] ; Dusan Losic [Australie] ; Seung Jun Park ; Jean-Francois Feller [France] ; Taeyoung KimSource :
- International journal of nanomedicine [ 1178-2013 ] ; 2015.
Descripteurs français
- KwdFr :
- MESH :
English descriptors
- KwdEn :
- MESH :
- chemical , analysis : Volatile Organic Compounds.
- chemical , chemistry : Bridged Bicyclo Compounds, Heterocyclic, Ionic Liquids, Magnetite Nanoparticles, Polymers.
- chemistry : Nanocomposites.
Abstract
We report a high-performance chemiresistive sensor for detection of volatile organic compound (VOC) vapors based on core-shell hybridized nanostructures of Fe3O4 magnetic nanoparticles (MNPs) and poly(3,4-ethylenedioxythiophene) (PEDOT)-conducting polymers. The MNPs were prepared using microwave-assisted synthesis in the presence of polymerized ionic liquids (PILs), which were used as a linker to couple the MNP and PEDOT. The resulting PEDOT-PIL-modified Fe3O4 hybrids were then explored as a sensing channel material for a chemiresistive sensor to detect VOC vapors. The PEDOT-PIL-modified Fe3O4 sensor exhibited a tunable response, with high sensitivity (down to a concentration of 1 ppm) and low noise level, to VOCs; these VOCs include acetone vapor, which is present in the exhaled breath of potential lung cancer patients. The present sensor, based on the hybrid nanostructured sensing materials, exhibited a 38.8% higher sensitivity and an 11% lower noise level than its PEDOT-PIL-only counterpart. This approach of embedding MNPs in conducting polymers could lead to the development of new electronic noses, which have significant potential for the use in the early diagnosis of lung cancer via the detection of VOC biomarkers.
DOI: 10.2147/IJN.S88305
PubMed: 26357471
Affiliations:
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Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>School of Chemical Engineering, The University of Adelaide, North Terrace, Adelaide, SA, Australia ; Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient</wicri:regionArea><placeName><region type="region">Région Bretagne</region><region type="old region">Région Bretagne</region><settlement type="city">Lorient</settlement></placeName></affiliation></author><author><name sortKey="Losic, Dusan" sort="Losic, Dusan" uniqKey="Losic D" first="Dusan" last="Losic">Dusan Losic</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical Engineering, The University of Adelaide, North Terrace, Adelaide, SA, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical Engineering, The University of Adelaide, North Terrace, Adelaide, SA</wicri:regionArea><wicri:noRegion>SA</wicri:noRegion></affiliation></author><author><name sortKey="Park, Seung Jun" sort="Park, Seung Jun" uniqKey="Park S" first="Seung Jun" last="Park">Seung Jun Park</name><affiliation><nlm:affiliation>Department of Bionanotechnology, Gachon University, Sujeong-gu, Seongnam-si, Gyeonggi-do South Korea.</nlm:affiliation><wicri:noCountry code="subField">Gyeonggi-do South Korea</wicri:noCountry></affiliation></author><author><name sortKey="Feller, Jean Francois" sort="Feller, Jean Francois" uniqKey="Feller J" first="Jean-Francois" last="Feller">Jean-Francois Feller</name><affiliation wicri:level="3"><nlm:affiliation>Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient</wicri:regionArea><placeName><region type="region">Région Bretagne</region><region type="old region">Région Bretagne</region><settlement type="city">Lorient</settlement></placeName></affiliation></author><author><name sortKey="Kim, Taeyoung" sort="Kim, Taeyoung" uniqKey="Kim T" first="Taeyoung" last="Kim">Taeyoung Kim</name><affiliation><nlm:affiliation>Department of Bionanotechnology, Gachon University, Sujeong-gu, Seongnam-si, Gyeonggi-do South Korea.</nlm:affiliation><wicri:noCountry code="subField">Gyeonggi-do South Korea</wicri:noCountry></affiliation></author></analytic><series><title level="j">International journal of nanomedicine</title><idno type="eISSN">1178-2013</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Bridged Bicyclo Compounds, Heterocyclic (chemistry)</term><term>Ionic Liquids (chemistry)</term><term>Magnetite Nanoparticles (chemistry)</term><term>Nanocomposites (chemistry)</term><term>Polymers (chemistry)</term><term>Volatile Organic Compounds (analysis)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Composés hétérocycliques bicycliques ()</term><term>Composés organiques volatils (analyse)</term><term>Liquides ioniques ()</term><term>Nanocomposites ()</term><term>Nanoparticules de magnétite ()</term><term>Polymères ()</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Volatile Organic Compounds</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Bridged Bicyclo Compounds, Heterocyclic</term><term>Ionic Liquids</term><term>Magnetite Nanoparticles</term><term>Polymers</term></keywords><keywords scheme="MESH" qualifier="analyse" xml:lang="fr"><term>Composés organiques volatils</term></keywords><keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Nanocomposites</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Composés hétérocycliques bicycliques</term><term>Liquides ioniques</term><term>Nanocomposites</term><term>Nanoparticules de magnétite</term><term>Polymères</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We report a high-performance chemiresistive sensor for detection of volatile organic compound (VOC) vapors based on core-shell hybridized nanostructures of Fe3O4 magnetic nanoparticles (MNPs) and poly(3,4-ethylenedioxythiophene) (PEDOT)-conducting polymers. The MNPs were prepared using microwave-assisted synthesis in the presence of polymerized ionic liquids (PILs), which were used as a linker to couple the MNP and PEDOT. The resulting PEDOT-PIL-modified Fe3O4 hybrids were then explored as a sensing channel material for a chemiresistive sensor to detect VOC vapors. The PEDOT-PIL-modified Fe3O4 sensor exhibited a tunable response, with high sensitivity (down to a concentration of 1 ppm) and low noise level, to VOCs; these VOCs include acetone vapor, which is present in the exhaled breath of potential lung cancer patients. The present sensor, based on the hybrid nanostructured sensing materials, exhibited a 38.8% higher sensitivity and an 11% lower noise level than its PEDOT-PIL-only counterpart. This approach of embedding MNPs in conducting polymers could lead to the development of new electronic noses, which have significant potential for the use in the early diagnosis of lung cancer via the detection of VOC biomarkers.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">26357471</PMID><DateCreated><Year>2015</Year><Month>09</Month><Day>11</Day></DateCreated><DateCompleted><Year>2016</Year><Month>03</Month><Day>28</Day></DateCompleted><DateRevised><Year>2017</Year><Month>02</Month><Day>20</Day></DateRevised><Article PubModel="Electronic-eCollection"><Journal><ISSN IssnType="Electronic">1178-2013</ISSN><JournalIssue CitedMedium="Internet"><Volume>10 Spec Iss</Volume><PubDate><Year>2015</Year></PubDate></JournalIssue><Title>International journal of nanomedicine</Title><ISOAbbreviation>Int J Nanomedicine</ISOAbbreviation></Journal><ArticleTitle>Core-shell nanostructured hybrid composites for volatile organic compound detection.</ArticleTitle><Pagination><MedlinePgn>203-14</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.2147/IJN.S88305</ELocationID><Abstract><AbstractText>We report a high-performance chemiresistive sensor for detection of volatile organic compound (VOC) vapors based on core-shell hybridized nanostructures of Fe3O4 magnetic nanoparticles (MNPs) and poly(3,4-ethylenedioxythiophene) (PEDOT)-conducting polymers. The MNPs were prepared using microwave-assisted synthesis in the presence of polymerized ionic liquids (PILs), which were used as a linker to couple the MNP and PEDOT. The resulting PEDOT-PIL-modified Fe3O4 hybrids were then explored as a sensing channel material for a chemiresistive sensor to detect VOC vapors. The PEDOT-PIL-modified Fe3O4 sensor exhibited a tunable response, with high sensitivity (down to a concentration of 1 ppm) and low noise level, to VOCs; these VOCs include acetone vapor, which is present in the exhaled breath of potential lung cancer patients. The present sensor, based on the hybrid nanostructured sensing materials, exhibited a 38.8% higher sensitivity and an 11% lower noise level than its PEDOT-PIL-only counterpart. This approach of embedding MNPs in conducting polymers could lead to the development of new electronic noses, which have significant potential for the use in the early diagnosis of lung cancer via the detection of VOC biomarkers.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Tung</LastName><ForeName>Tran Thanh</ForeName><Initials>TT</Initials><AffiliationInfo><Affiliation>School of Chemical Engineering, The University of Adelaide, North Terrace, Adelaide, SA, Australia ; Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Losic</LastName><ForeName>Dusan</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>School of Chemical Engineering, The University of Adelaide, North Terrace, Adelaide, SA, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Park</LastName><ForeName>Seung Jun</ForeName><Initials>SJ</Initials><AffiliationInfo><Affiliation>Department of Bionanotechnology, Gachon University, Sujeong-gu, Seongnam-si, Gyeonggi-do South Korea.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Feller</LastName><ForeName>Jean-Francois</ForeName><Initials>JF</Initials><AffiliationInfo><Affiliation>Smart Plastics Group, European University of Brittany (UEB), LIMATB-UBS, Lorient, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Kim</LastName><ForeName>TaeYoung</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Department of Bionanotechnology, Gachon University, Sujeong-gu, Seongnam-si, Gyeonggi-do South Korea.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2015</Year><Month>08</Month><Day>28</Day></ArticleDate></Article><MedlineJournalInfo><Country>New Zealand</Country><MedlineTA>Int J Nanomedicine</MedlineTA><NlmUniqueID>101263847</NlmUniqueID><ISSNLinking>1176-9114</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D019086">Bridged Bicyclo Compounds, Heterocyclic</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D052578">Ionic Liquids</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D058185">Magnetite Nanoparticles</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D011108">Polymers</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D055549">Volatile Organic Compounds</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance 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name="France"><region name="Région Bretagne"><name sortKey="Tung, Tran Thanh" sort="Tung, Tran Thanh" uniqKey="Tung T" first="Tran Thanh" last="Tung">Tran Thanh Tung</name></region><name sortKey="Feller, Jean Francois" sort="Feller, Jean Francois" uniqKey="Feller J" first="Jean-Francois" last="Feller">Jean-Francois Feller</name></country><country name="Australie"><noRegion><name sortKey="Losic, Dusan" sort="Losic, Dusan" uniqKey="Losic D" first="Dusan" last="Losic">Dusan Losic</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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