AustralieFrV1, PascalFrancis, Curation, bibRecord, 004781

Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rn expansion

Identifieur interne : 004781 ( PascalFrancis/Curation ); précédent : 004780; suivant : 004782

Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rn expansion

Auteurs : M. Lepers [France] ; O. Dulieu [France]

Source :

The European physical journal. D, Atomic, molecular and optical physics : (Print) [ 1434-6060 ] ; 2011.

RBID : Pascal:12-0019050

Descripteurs français

Pascal (Inist)
- Photoassociation, Interaction longue distance, Interaction électrostatique, Atome froid, Etude théorique, Théorie perturbation, Courbe potentiel, Croisement évité, Etat fondamental, Etat rovibrationnel, Molécule ultrafroide, Métal alcalin, Collision atome molécule, Collision sous rayonnement, 3450R, 3380P, 3115M, Molécule froide.

English descriptors

KwdEn :
- Alkali metals, Atom-molecule collisions, Avoided crossing, Cold atom, Cold molecules, Electrostatic interaction, Ground states, Long range interaction, Perturbation theory, Photoassociation, Potential energy curve, Radiation assisted collision, Rotational-vibrational states, Theoretical study, Ultracold molecules.

Abstract

We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom. As the electrostatic energy is comparable to the dimer rotational structure, we develop a general description of the long-range interactions in the framework of the second-order degenerate perturbation theory, which allows for couplings between the dimer rotational levels. The resulting adiabatic potential energy curves exhibit avoided crossings, and cannot be expanded as the usual 1/Rⁿ series. We study in details the particular case Cs₂+Cs(6²P). Our results are found promising to achieve photoassociation of ultracold trimers.

A01	`01`	`1`		`@0 1434-6060`
A03		`1`		`@0 Eur. phys. j., D At. mol. opt. phys.`
A05				`@2 65`
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A08	`01`	`1`	`ENG`	`@1 Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rⁿexpansion`
A09	`01`	`1`	`ENG`	`@1 Cold Quantum Matter`
A11	`01`	`1`		`@1 LEPERS (M.)`
A11	`02`	`1`		`@1 DULIEU (O.)`
A12	`01`	`1`		`@1 BIRKL (Gerhard) @9 ed.`
A12	`02`	`1`		`@1 FOOT (Christopher) @9 ed.`
A12	`03`	`1`		`@1 FREEGARDE (Tim) @9 ed.`
A12	`04`	`1`		`@1 GRIMM (Rudolf) @9 ed.`
A12	`05`	`1`		`@1 HUTSON (Jeremy M.) @9 ed.`
A12	`06`	`1`		`@1 WEIDEMÜLLER (Matthias) @9 ed.`
A14	`01`			`@1 Laboratoire Aime Cotton, CNRS, Bât. 505, Univ. Paris-Sud @2 91405 Orsay @3 FRA @Z 1 aut. @Z 2 aut.`
A15	`01`			`@1 University of Darmstad @3 DEU @Z 1 aut.`
A15	`02`			`@1 University of Oxford @3 GBR @Z 2 aut.`
A15	`03`			`@1 University of Southampton @3 GBR @Z 3 aut.`
A15	`04`			`@1 University of Innsbruck @3 AUS @Z 4 aut.`
A15	`05`			`@1 University of Durham @3 GBR @Z 5 aut.`
A15	`06`			`@1 University of Heidelberg @3 DEU @Z 6 aut.`
A20				`@1 113-123`
A21				`@1 2011`
A23	`01`			`@0 ENG`
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A44				`@0 0000 @1 © 2012 INIST-CNRS. All rights reserved.`
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A64	`01`	`1`		`@0 The European physical journal. D, Atomic, molecular and optical physics : (Print)`
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C01	`01`		`ENG`	@0 We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom. As the electrostatic energy is comparable to the dimer rotational structure, we develop a general description of the long-range interactions in the framework of the second-order degenerate perturbation theory, which allows for couplings between the dimer rotational levels. The resulting adiabatic potential energy curves exhibit avoided crossings, and cannot be expanded as the usual 1/Rⁿ series. We study in details the particular case Cs₂+Cs(6²P). Our results are found promising to achieve photoassociation of ultracold trimers.
C02	`01`	`3`		`@0 001B30A15M`
C02	`02`	`3`		`@0 001B30D50R`
C02	`03`	`3`		`@0 001B30C80P`
C03	`01`	`3`	`FRE`	`@0 Photoassociation @5 03`
C03	`01`	`3`	`ENG`	`@0 Photoassociation @5 03`
C03	`02`	`X`	`FRE`	`@0 Interaction longue distance @5 04`
C03	`02`	`X`	`ENG`	`@0 Long range interaction @5 04`
C03	`02`	`X`	`SPA`	`@0 Interacción larga distancia @5 04`
C03	`03`	`X`	`FRE`	`@0 Interaction électrostatique @5 05`
C03	`03`	`X`	`ENG`	`@0 Electrostatic interaction @5 05`
C03	`03`	`X`	`SPA`	`@0 Interacción electrostática @5 05`
C03	`04`	`3`	`FRE`	`@0 Atome froid @5 11`
C03	`04`	`3`	`ENG`	`@0 Cold atom @5 11`
C03	`05`	`3`	`FRE`	`@0 Etude théorique @5 21`
C03	`05`	`3`	`ENG`	`@0 Theoretical study @5 21`
C03	`06`	`3`	`FRE`	`@0 Théorie perturbation @5 23`
C03	`06`	`3`	`ENG`	`@0 Perturbation theory @5 23`
C03	`07`	`X`	`FRE`	`@0 Courbe potentiel @5 24`
C03	`07`	`X`	`ENG`	`@0 Potential energy curve @5 24`
C03	`07`	`X`	`SPA`	`@0 Curva potencial @5 24`
C03	`08`	`X`	`FRE`	`@0 Croisement évité @5 25`
C03	`08`	`X`	`ENG`	`@0 Avoided crossing @5 25`
C03	`08`	`X`	`SPA`	`@0 Cruce evitado @5 25`
C03	`09`	`3`	`FRE`	`@0 Etat fondamental @5 41`
C03	`09`	`3`	`ENG`	`@0 Ground states @5 41`
C03	`10`	`3`	`FRE`	`@0 Etat rovibrationnel @5 42`
C03	`10`	`3`	`ENG`	`@0 Rotational-vibrational states @5 42`
C03	`11`	`3`	`FRE`	`@0 Molécule ultrafroide @2 NK @5 57`
C03	`11`	`3`	`ENG`	`@0 Ultracold molecules @2 NK @5 57`
C03	`12`	`3`	`FRE`	`@0 Métal alcalin @2 NC @5 61`
C03	`12`	`3`	`ENG`	`@0 Alkali metals @2 NC @5 61`
C03	`13`	`3`	`FRE`	`@0 Collision atome molécule @5 62`
C03	`13`	`3`	`ENG`	`@0 Atom-molecule collisions @5 62`
C03	`14`	`X`	`FRE`	`@0 Collision sous rayonnement @5 63`
C03	`14`	`X`	`ENG`	`@0 Radiation assisted collision @5 63`
C03	`14`	`X`	`SPA`	`@0 Colisión bajo radiación @5 63`
C03	`15`	`3`	`FRE`	`@0 3450R @4 INC @5 83`
C03	`16`	`3`	`FRE`	`@0 3380P @4 INC @5 84`
C03	`17`	`3`	`FRE`	`@0 3115M @4 INC @5 91`
C03	`18`	`3`	`FRE`	`@0 Molécule froide @4 CD @5 96`
C03	`18`	`3`	`ENG`	`@0 Cold molecules @4 CD @5 96`
N21				`@1 002`

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Le document en format XML

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<front><div type="abstract" xml:lang="en">We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom. As the electrostatic energy is comparable to the dimer rotational structure, we develop a general description of the long-range interactions in the framework of the second-order degenerate perturbation theory, which allows for couplings between the dimer rotational levels. The resulting adiabatic potential energy curves exhibit avoided crossings, and cannot be expanded as the usual 1/R<sup>n</sup>
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<s5>23</s5>
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<s5>23</s5>
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<s5>24</s5>
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<s5>24</s5>
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<s5>24</s5>
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<s5>25</s5>
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<s5>25</s5>
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<s5>41</s5>
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<s5>41</s5>
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<s5>42</s5>
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<s5>42</s5>
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<fC03 i1="11" i2="3" l="FRE"><s0>Molécule ultrafroide</s0>
<s2>NK</s2>
<s5>57</s5>
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<s2>NK</s2>
<s5>57</s5>
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<s2>NC</s2>
<s5>61</s5>
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<s2>NC</s2>
<s5>61</s5>
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<s5>62</s5>
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<s5>62</s5>
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<fC03 i1="14" i2="X" l="FRE"><s0>Collision sous rayonnement</s0>
<s5>63</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Radiation assisted collision</s0>
<s5>63</s5>
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<s5>63</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>3450R</s0>
<s4>INC</s4>
<s5>83</s5>
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<fC03 i1="16" i2="3" l="FRE"><s0>3380P</s0>
<s4>INC</s4>
<s5>84</s5>
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<fC03 i1="17" i2="3" l="FRE"><s0>3115M</s0>
<s4>INC</s4>
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</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Molécule froide</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fC03 i1="18" i2="3" l="ENG"><s0>Cold molecules</s0>
<s4>CD</s4>
<s5>96</s5>
</fC03>
<fN21><s1>002</s1>
</fN21>
</pA>
</standard>
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</record>

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   |area=    AustralieFrV1
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   |clé=     Pascal:12-0019050
   |texte=   Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rn expansion
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	Serveur d'exploration sur les relations entre la France et l'Australie
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Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rn expansion

Cold atom-molecule photoassociation: long-range interactions beyond the 1/Rn expansion

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