AustralieFrV1, PascalFrancis, Curation, bibRecord, 002D31

Luminescence properties of poly(phenylene vinylene) derivatives

Identifieur interne : 002D31 ( PascalFrancis/Curation ); précédent : 002D30; suivant : 002D32

Luminescence properties of poly(phenylene vinylene) derivatives

Auteurs : Cuong Ton-That [Australie] ; Geoff Stockton [Australie] ; Matthew R. Phillips [Australie] ; Thien-Phap Nguyen [France] ; CHUN HAO HUANG [France] ; Ala Cojocaru [Moldavie]

Source :

Polymer international [ 0959-8103 ] ; 2008.

RBID : Pascal:08-0448198

Descripteurs français

Pascal (Inist)
- Phénylènevinylène dérivé polymère, Polymère conjugué, Polymère soufre, Etude expérimentale, Cathodoluminescence, Préparation, Photoluminescence, Conformation, Relation structure propriété, Effet substituant, Effet température, Propriété optique, Phénylènevinylène(2-[2-éthylhexyloxy]-5-méthoxy) polymère.

English descriptors

KwdEn :
- Cathodoluminescence, Conformation, Conjugated polymer, Experimental study, Optical properties, Phenylenevinylene derivative polymer, Photoluminescence, Preparation, Property structure relationship, Substituent effect, Sulfur containing polymer, Temperature effect.

Abstract

BACKGROUND: Conjugated polymers, especially those of the poly(phenylene vinylene) (PPV) family, are promising candidates as emission material in light-emitting devices. The aim of this work was to investigate the dependence of the luminescence properties of PPV-based derivatives on their polymer structure, especially side groups. RESULTS: Three PPV derivatives, BEHPPV, MEHPPV and MEHSPPV, were synthesised and characterised by photoluminescence (PL) and cathodoluminescence (CL) spectroscopies in the temperature range 10-300K. PL and CL spectra of the polymers exhibit similar luminescence peaks, which undergo a blue shift with increasing temperature. The shift in wavelength is accompanied by variations in the relative intensities of emission peaks. Both BEHPPV and MEHPPV display emission characteristics of the PPV backbone, but the peak of MEHPPV shifts to a longer wavelength in comparison with the corresponding peak of BEHPPV at the same temperature. The luminescence spectra of MEHSPPV, which has a sulfanyl incorporated in the side chain, are considerably different from those of the two other derivatives. CONCLUSIONS: The results demonstrate that the luminescence properties depend strongly on the chain conformations of the conjugated backbone, which are affected by polymer side chains.

A01	`01`	`1`		`@0 0959-8103`
A03		`1`		`@0 Polym. int.`
A05				`@2 57`
A06				`@2 3`
A08	`01`	`1`	`ENG`	`@1 Luminescence properties of poly(phenylene vinylene) derivatives`
A11	`01`	`1`		`@1 TON-THAT (Cuong)`
A11	`02`	`1`		`@1 STOCKTON (Geoff)`
A11	`03`	`1`		`@1 PHILLIPS (Matthew R.)`
A11	`04`	`1`		`@1 NGUYEN (Thien-Phap)`
A11	`05`	`1`		`@1 CHUN HAO HUANG`
A11	`06`	`1`		`@1 COJOCARU (Ala)`
A14	`01`			`@1 Department of Physics and Advanced Materials, University of Technology Sydney, PO Box 123 @2 NSW 2007 @3 AUS @Z 1 aut. @Z 2 aut. @Z 3 aut.`
A14	`02`			`@1 Institut des Matériaux Jean Rouxel, University of Nantes @2 44322 Nantes @3 FRA @Z 4 aut. @Z 5 aut.`
A14	`03`			`@1 Technical University of Moldova @2 Chisinau @3 MDA @Z 6 aut.`
A20				`@1 496-501`
A21				`@1 2008`
A23	`01`			`@0 ENG`
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A44				`@0 0000 @1 © 2008 INIST-CNRS. All rights reserved.`
A45				`@0 29 ref.`
A47	`01`	`1`		`@0 08-0448198`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Polymer international`
A66	`01`			`@0 GBR`
C01	`01`		`ENG`	@0 BACKGROUND: Conjugated polymers, especially those of the poly(phenylene vinylene) (PPV) family, are promising candidates as emission material in light-emitting devices. The aim of this work was to investigate the dependence of the luminescence properties of PPV-based derivatives on their polymer structure, especially side groups. RESULTS: Three PPV derivatives, BEHPPV, MEHPPV and MEHSPPV, were synthesised and characterised by photoluminescence (PL) and cathodoluminescence (CL) spectroscopies in the temperature range 10-300K. PL and CL spectra of the polymers exhibit similar luminescence peaks, which undergo a blue shift with increasing temperature. The shift in wavelength is accompanied by variations in the relative intensities of emission peaks. Both BEHPPV and MEHPPV display emission characteristics of the PPV backbone, but the peak of MEHPPV shifts to a longer wavelength in comparison with the corresponding peak of BEHPPV at the same temperature. The luminescence spectra of MEHSPPV, which has a sulfanyl incorporated in the side chain, are considerably different from those of the two other derivatives. CONCLUSIONS: The results demonstrate that the luminescence properties depend strongly on the chain conformations of the conjugated backbone, which are affected by polymer side chains.
C02	`01`	`X`		`@0 001D09D04D`
C03	`01`	`X`	`FRE`	`@0 Phénylènevinylène dérivé polymère @5 01`
C03	`01`	`X`	`ENG`	`@0 Phenylenevinylene derivative polymer @5 01`
C03	`01`	`X`	`SPA`	`@0 Fenilenovinileno derivado polimero @5 01`
C03	`02`	`X`	`FRE`	`@0 Polymère conjugué @5 02`
C03	`02`	`X`	`ENG`	`@0 Conjugated polymer @5 02`
C03	`02`	`X`	`SPA`	`@0 Polímero conjugado @5 02`
C03	`03`	`X`	`FRE`	`@0 Polymère soufre @2 NK @5 03`
C03	`03`	`X`	`ENG`	`@0 Sulfur containing polymer @2 NK @5 03`
C03	`03`	`X`	`SPA`	`@0 Polímero azufre @2 NK @5 03`
C03	`04`	`X`	`FRE`	`@0 Etude expérimentale @5 04`
C03	`04`	`X`	`ENG`	`@0 Experimental study @5 04`
C03	`04`	`X`	`SPA`	`@0 Estudio experimental @5 04`
C03	`05`	`X`	`FRE`	`@0 Cathodoluminescence @5 05`
C03	`05`	`X`	`ENG`	`@0 Cathodoluminescence @5 05`
C03	`05`	`X`	`SPA`	`@0 Catodoluminiscencia @5 05`
C03	`06`	`X`	`FRE`	`@0 Préparation @5 06`
C03	`06`	`X`	`ENG`	`@0 Preparation @5 06`
C03	`06`	`X`	`SPA`	`@0 Preparación @5 06`
C03	`07`	`X`	`FRE`	`@0 Photoluminescence @5 07`
C03	`07`	`X`	`ENG`	`@0 Photoluminescence @5 07`
C03	`07`	`X`	`SPA`	`@0 Fotoluminiscencia @5 07`
C03	`08`	`X`	`FRE`	`@0 Conformation @5 08`
C03	`08`	`X`	`ENG`	`@0 Conformation @5 08`
C03	`08`	`X`	`SPA`	`@0 Conformación @5 08`
C03	`09`	`X`	`FRE`	`@0 Relation structure propriété @5 09`
C03	`09`	`X`	`ENG`	`@0 Property structure relationship @5 09`
C03	`09`	`X`	`SPA`	`@0 Relación estructura propiedad @5 09`
C03	`10`	`X`	`FRE`	`@0 Effet substituant @5 10`
C03	`10`	`X`	`ENG`	`@0 Substituent effect @5 10`
C03	`10`	`X`	`SPA`	`@0 Efecto sustituyente @5 10`
C03	`11`	`X`	`FRE`	`@0 Effet température @5 11`
C03	`11`	`X`	`ENG`	`@0 Temperature effect @5 11`
C03	`11`	`X`	`SPA`	`@0 Efecto temperatura @5 11`
C03	`12`	`X`	`FRE`	`@0 Propriété optique @5 31`
C03	`12`	`X`	`ENG`	`@0 Optical properties @5 31`
C03	`12`	`X`	`SPA`	`@0 Propiedad óptica @5 31`
C03	`13`	`X`	`FRE`	`@0 Phénylènevinylène(2-[2-éthylhexyloxy]-5-méthoxy) polymère @4 INC @5 41`
N21				`@1 294`

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Le document en format XML

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<author><name sortKey="Phillips, Matthew R" sort="Phillips, Matthew R" uniqKey="Phillips M" first="Matthew R." last="Phillips">Matthew R. Phillips</name>
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<sZ>2 aut.</sZ>
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<author><name sortKey="Nguyen, Thien Phap" sort="Nguyen, Thien Phap" uniqKey="Nguyen T" first="Thien-Phap" last="Nguyen">Thien-Phap Nguyen</name>
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<s2>44322 Nantes</s2>
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<sZ>5 aut.</sZ>
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<country>France</country>
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<author><name sortKey="Chun Hao Huang" sort="Chun Hao Huang" uniqKey="Chun Hao Huang" last="Chun Hao Huang">CHUN HAO HUANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Institut des Matériaux Jean Rouxel, University of Nantes</s1>
<s2>44322 Nantes</s2>
<s3>FRA</s3>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>France</country>
</affiliation>
</author>
<author><name sortKey="Cojocaru, Ala" sort="Cojocaru, Ala" uniqKey="Cojocaru A" first="Ala" last="Cojocaru">Ala Cojocaru</name>
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<s2>Chisinau</s2>
<s3>MDA</s3>
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<country>Moldavie</country>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Cathodoluminescence</term>
<term>Conformation</term>
<term>Conjugated polymer</term>
<term>Experimental study</term>
<term>Optical properties</term>
<term>Phenylenevinylene derivative polymer</term>
<term>Photoluminescence</term>
<term>Preparation</term>
<term>Property structure relationship</term>
<term>Substituent effect</term>
<term>Sulfur containing polymer</term>
<term>Temperature effect</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Phénylènevinylène dérivé polymère</term>
<term>Polymère conjugué</term>
<term>Polymère soufre</term>
<term>Etude expérimentale</term>
<term>Cathodoluminescence</term>
<term>Préparation</term>
<term>Photoluminescence</term>
<term>Conformation</term>
<term>Relation structure propriété</term>
<term>Effet substituant</term>
<term>Effet température</term>
<term>Propriété optique</term>
<term>Phénylènevinylène(2-[2-éthylhexyloxy]-5-méthoxy) polymère</term>
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<front><div type="abstract" xml:lang="en">BACKGROUND: Conjugated polymers, especially those of the poly(phenylene vinylene) (PPV) family, are promising candidates as emission material in light-emitting devices. The aim of this work was to investigate the dependence of the luminescence properties of PPV-based derivatives on their polymer structure, especially side groups. RESULTS: Three PPV derivatives, BEHPPV, MEHPPV and MEHSPPV, were synthesised and characterised by photoluminescence (PL) and cathodoluminescence (CL) spectroscopies in the temperature range 10-300K. PL and CL spectra of the polymers exhibit similar luminescence peaks, which undergo a blue shift with increasing temperature. The shift in wavelength is accompanied by variations in the relative intensities of emission peaks. Both BEHPPV and MEHPPV display emission characteristics of the PPV backbone, but the peak of MEHPPV shifts to a longer wavelength in comparison with the corresponding peak of BEHPPV at the same temperature. The luminescence spectra of MEHSPPV, which has a sulfanyl incorporated in the side chain, are considerably different from those of the two other derivatives. CONCLUSIONS: The results demonstrate that the luminescence properties depend strongly on the chain conformations of the conjugated backbone, which are affected by polymer side chains.</div>
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<fA11 i1="01" i2="1"><s1>TON-THAT (Cuong)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>STOCKTON (Geoff)</s1>
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<fA11 i1="03" i2="1"><s1>PHILLIPS (Matthew R.)</s1>
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<fA11 i1="04" i2="1"><s1>NGUYEN (Thien-Phap)</s1>
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<fA11 i1="05" i2="1"><s1>CHUN HAO HUANG</s1>
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<fA11 i1="06" i2="1"><s1>COJOCARU (Ala)</s1>
</fA11>
<fA14 i1="01"><s1>Department of Physics and Advanced Materials, University of Technology Sydney, PO Box 123</s1>
<s2>NSW 2007</s2>
<s3>AUS</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Institut des Matériaux Jean Rouxel, University of Nantes</s1>
<s2>44322 Nantes</s2>
<s3>FRA</s3>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</fA14>
<fA14 i1="03"><s1>Technical University of Moldova</s1>
<s2>Chisinau</s2>
<s3>MDA</s3>
<sZ>6 aut.</sZ>
</fA14>
<fA20><s1>496-501</s1>
</fA20>
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<fA47 i1="01" i2="1"><s0>08-0448198</s0>
</fA47>
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<fA66 i1="01"><s0>GBR</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>BACKGROUND: Conjugated polymers, especially those of the poly(phenylene vinylene) (PPV) family, are promising candidates as emission material in light-emitting devices. The aim of this work was to investigate the dependence of the luminescence properties of PPV-based derivatives on their polymer structure, especially side groups. RESULTS: Three PPV derivatives, BEHPPV, MEHPPV and MEHSPPV, were synthesised and characterised by photoluminescence (PL) and cathodoluminescence (CL) spectroscopies in the temperature range 10-300K. PL and CL spectra of the polymers exhibit similar luminescence peaks, which undergo a blue shift with increasing temperature. The shift in wavelength is accompanied by variations in the relative intensities of emission peaks. Both BEHPPV and MEHPPV display emission characteristics of the PPV backbone, but the peak of MEHPPV shifts to a longer wavelength in comparison with the corresponding peak of BEHPPV at the same temperature. The luminescence spectra of MEHSPPV, which has a sulfanyl incorporated in the side chain, are considerably different from those of the two other derivatives. CONCLUSIONS: The results demonstrate that the luminescence properties depend strongly on the chain conformations of the conjugated backbone, which are affected by polymer side chains.</s0>
</fC01>
<fC02 i1="01" i2="X"><s0>001D09D04D</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Phénylènevinylène dérivé polymère</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Phenylenevinylene derivative polymer</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Fenilenovinileno derivado polimero</s0>
<s5>01</s5>
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<fC03 i1="02" i2="X" l="FRE"><s0>Polymère conjugué</s0>
<s5>02</s5>
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<s5>02</s5>
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<fC03 i1="02" i2="X" l="SPA"><s0>Polímero conjugado</s0>
<s5>02</s5>
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<fC03 i1="03" i2="X" l="FRE"><s0>Polymère soufre</s0>
<s2>NK</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Sulfur containing polymer</s0>
<s2>NK</s2>
<s5>03</s5>
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<fC03 i1="03" i2="X" l="SPA"><s0>Polímero azufre</s0>
<s2>NK</s2>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE"><s0>Etude expérimentale</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG"><s0>Experimental study</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA"><s0>Estudio experimental</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Cathodoluminescence</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Cathodoluminescence</s0>
<s5>05</s5>
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<fC03 i1="05" i2="X" l="SPA"><s0>Catodoluminiscencia</s0>
<s5>05</s5>
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<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Preparation</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Preparación</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Photoluminescence</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Photoluminescence</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Fotoluminiscencia</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Conformation</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Conformation</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Conformación</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Relation structure propriété</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Property structure relationship</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Relación estructura propiedad</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Effet substituant</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Substituent effect</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Efecto sustituyente</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Effet température</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Temperature effect</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Efecto temperatura</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Propriété optique</s0>
<s5>31</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Optical properties</s0>
<s5>31</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Propiedad óptica</s0>
<s5>31</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Phénylènevinylène(2-[2-éthylhexyloxy]-5-méthoxy) polymère</s0>
<s4>INC</s4>
<s5>41</s5>
</fC03>
<fN21><s1>294</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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Luminescence properties of poly(phenylene vinylene) derivatives

Luminescence properties of poly(phenylene vinylene) derivatives

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