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Influence of point defects on the thermoluminescence of α-Al2O3 : Application to dosimetry

Identifieur interne : 006280 ( PascalFrancis/Corpus ); précédent : 006279; suivant : 006281

Influence of point defects on the thermoluminescence of α-Al2O3 : Application to dosimetry

Auteurs : E. Papin ; P. Grosseau ; B. Guilhot ; M. Benabdesselam ; P. Iacconi

Source :

RBID : Pascal:99-0414270

Descripteurs français

English descriptors

Abstract

Doped α-alumina powders have been synthesised by thermal treatment of γ-alumina under a controlled atmosphere. Two TL peaks, located at 200°C and 365°C, have been detected in almost all samples. Their intensity is strongly dependent on the atmosphere and on the nature of introduced dopants. The influence of these parameters on point defects concentrations is analysed, and compared with TL intensity variations. It is suggested that aluminium vacancies are the trap defects responsible for these two peaks and, depending on the preparation conditions, F centres or Cr3+ can be the recombination centres. Two powders have been selected for dosimetry use. Their sensitivity to X ray radiation have been compared with that of Al2O3:C powder (TLD-800). The TLD-800 dosimetric peak corresponds exactly to their 200°C peak.

Notice en format standard (ISO 2709)

Pour connaître la documentation sur le format Inist Standard.

pA  
A01 01  1    @0 0144-8420
A02 01      @0 RPDODE
A03   1    @0 Radiat. prot. dosim.
A05       @2 84
A06       @2 1-4
A08 01  1  ENG  @1 Influence of point defects on the thermoluminescence of α-Al2O3 : Application to dosimetry
A09 01  1  ENG  @1 Solid state dosimetry. Part I
A11 01  1    @1 PAPIN (E.)
A11 02  1    @1 GROSSEAU (P.)
A11 03  1    @1 GUILHOT (B.)
A11 04  1    @1 BENABDESSELAM (M.)
A11 05  1    @1 IACCONI (P.)
A12 01  1    @1 DELGADO (A.) @9 ed.
A12 02  1    @1 GOMEZ ROS (J. M.) @9 ed.
A12 03  1    @1 BOS (A. J. J.) @9 ed.
A12 04  1    @1 BØTTER-JENSEN (L.) @9 ed.
A12 05  1    @1 HOROWITZ (Y. S.) @9 ed.
A12 06  1    @1 JULIUS (H. W.) @9 ed.
A12 07  1    @1 KLEMIC (G.) @9 ed.
A12 08  1    @1 KRON (T.) @9 ed.
A14 01      @1 SPIN-CRESA, Ecole Nationale Supérieure des Mines, 158, cours Fauriel @2 42023 Saint-Etienne @3 FRA @Z 1 aut. @Z 2 aut. @Z 3 aut.
A14 02      @1 LPES-CRESA, Université de Nice-Sophia Antipolis, Parc Valrose @2 06108 Nice @3 FRA @Z 4 aut. @Z 5 aut.
A15 01      @1 CIEMAT @3 ESP @Z 1 aut.
A15 02      @1 Delft T. University @3 NLD @Z 3 aut.
A15 03      @1 Ben Gurion University @3 ISR @Z 5 aut.
A15 04      @1 TNO @3 NLD @Z 6 aut.
A15 05      @1 EML (DOE) @3 USA @Z 7 aut.
A15 06      @1 Newcastle Mater Misericordiae Hospital @3 AUS @Z 8 aut.
A20       @1 91-94
A21       @1 1999
A23 01      @0 ENG
A43 01      @1 INIST @2 19318 @5 354000085782220200
A44       @0 0000 @1 © 1999 INIST-CNRS. All rights reserved.
A45       @0 12 ref.
A47 01  1    @0 99-0414270
A60       @1 P @2 C
A61       @0 A
A64 01  1    @0 Radiation protection dosimetry
A66 01      @0 GBR
C01 01    ENG  @0 Doped α-alumina powders have been synthesised by thermal treatment of γ-alumina under a controlled atmosphere. Two TL peaks, located at 200°C and 365°C, have been detected in almost all samples. Their intensity is strongly dependent on the atmosphere and on the nature of introduced dopants. The influence of these parameters on point defects concentrations is analysed, and compared with TL intensity variations. It is suggested that aluminium vacancies are the trap defects responsible for these two peaks and, depending on the preparation conditions, F centres or Cr3+ can be the recombination centres. Two powders have been selected for dosimetry use. Their sensitivity to X ray radiation have been compared with that of Al2O3:C powder (TLD-800). The TLD-800 dosimetric peak corresponds exactly to their 200°C peak.
C02 01  X    @0 002A08F05
C03 01  X  FRE  @0 Dosimètre thermoluminescent @5 01
C03 01  X  ENG  @0 Thermoluminescent dosimeter @5 01
C03 01  X  SPA  @0 Dosímetro termoluminescente @5 01
C03 02  X  FRE  @0 Traitement thermique @5 02
C03 02  X  ENG  @0 Heat treatment @5 02
C03 02  X  SPA  @0 Tratamiento térmico @5 02
C03 03  X  FRE  @0 Etude comparative @5 03
C03 03  X  ENG  @0 Comparative study @5 03
C03 03  X  SPA  @0 Estudio comparativo @5 03
C03 04  X  FRE  @0 Composé dopé @5 04
C03 04  X  ENG  @0 Doped compound @5 04
C03 04  X  SPA  @0 Compuesto drogado @5 04
C03 05  X  FRE  @0 Synthèse chimique @5 05
C03 05  X  ENG  @0 Chemical synthesis @5 05
C03 05  X  SPA  @0 Síntesis química @5 05
C03 06  X  FRE  @0 Alumine @2 NK @5 06
C03 06  X  ENG  @0 Alumina @2 NK @5 06
C03 06  X  SPA  @0 Alúmina @2 NK @5 06
C03 07  X  FRE  @0 Estimation paramètre @5 07
C03 07  X  ENG  @0 Parameter estimation @5 07
C03 07  X  SPA  @0 Estimación parámetro @5 07
C03 08  X  FRE  @0 Mesure concentration @5 08
C03 08  X  ENG  @0 Concentration measurement @5 08
C03 08  X  SPA  @0 Medición concentración @5 08
C03 09  X  FRE  @0 Défaut @5 09
C03 09  X  ENG  @0 Defect @5 09
C03 09  X  SPA  @0 Defecto @5 09
C03 10  X  FRE  @0 Processus recombinaison @5 10
C03 10  X  ENG  @0 Recombination process @5 10
C03 10  X  SPA  @0 Proceso recombinación @5 10
C03 11  X  FRE  @0 Analyse sensibilité @5 11
C03 11  X  ENG  @0 Sensitivity analysis @5 11
C03 11  X  SPA  @0 Análisis sensibilidad @5 11
N21       @1 263
pR  
A30 01  1  ENG  @1 International Conference on Solid State Dosimetry @2 12 @3 Burgos ESP @4 1998-07-05

Format Inist (serveur)

NO : PASCAL 99-0414270 INIST
ET : Influence of point defects on the thermoluminescence of α-Al2O3 : Application to dosimetry
AU : PAPIN (E.); GROSSEAU (P.); GUILHOT (B.); BENABDESSELAM (M.); IACCONI (P.); DELGADO (A.); GOMEZ ROS (J. M.); BOS (A. J. J.); BØTTER-JENSEN (L.); HOROWITZ (Y. S.); JULIUS (H. W.); KLEMIC (G.); KRON (T.)
AF : SPIN-CRESA, Ecole Nationale Supérieure des Mines, 158, cours Fauriel/42023 Saint-Etienne/France (1 aut., 2 aut., 3 aut.); LPES-CRESA, Université de Nice-Sophia Antipolis, Parc Valrose/06108 Nice/France (4 aut., 5 aut.); CIEMAT/Espagne (1 aut.); Delft T. University/Pays-Bas (3 aut.); Ben Gurion University/Israël (5 aut.); TNO/Pays-Bas (6 aut.); EML (DOE)/Etats-Unis (7 aut.); Newcastle Mater Misericordiae Hospital/Australie (8 aut.)
DT : Publication en série; Congrès; Niveau analytique
SO : Radiation protection dosimetry; ISSN 0144-8420; Coden RPDODE; Royaume-Uni; Da. 1999; Vol. 84; No. 1-4; Pp. 91-94; Bibl. 12 ref.
LA : Anglais
EA : Doped α-alumina powders have been synthesised by thermal treatment of γ-alumina under a controlled atmosphere. Two TL peaks, located at 200°C and 365°C, have been detected in almost all samples. Their intensity is strongly dependent on the atmosphere and on the nature of introduced dopants. The influence of these parameters on point defects concentrations is analysed, and compared with TL intensity variations. It is suggested that aluminium vacancies are the trap defects responsible for these two peaks and, depending on the preparation conditions, F centres or Cr3+ can be the recombination centres. Two powders have been selected for dosimetry use. Their sensitivity to X ray radiation have been compared with that of Al2O3:C powder (TLD-800). The TLD-800 dosimetric peak corresponds exactly to their 200°C peak.
CC : 002A08F05
FD : Dosimètre thermoluminescent; Traitement thermique; Etude comparative; Composé dopé; Synthèse chimique; Alumine; Estimation paramètre; Mesure concentration; Défaut; Processus recombinaison; Analyse sensibilité
ED : Thermoluminescent dosimeter; Heat treatment; Comparative study; Doped compound; Chemical synthesis; Alumina; Parameter estimation; Concentration measurement; Defect; Recombination process; Sensitivity analysis
SD : Dosímetro termoluminescente; Tratamiento térmico; Estudio comparativo; Compuesto drogado; Síntesis química; Alúmina; Estimación parámetro; Medición concentración; Defecto; Proceso recombinación; Análisis sensibilidad
LO : INIST-19318.354000085782220200
ID : 99-0414270

Links to Exploration step

Pascal:99-0414270

Le document en format XML

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<div type="abstract" xml:lang="en">Doped α-alumina powders have been synthesised by thermal treatment of γ-alumina under a controlled atmosphere. Two TL peaks, located at 200°C and 365°C, have been detected in almost all samples. Their intensity is strongly dependent on the atmosphere and on the nature of introduced dopants. The influence of these parameters on point defects concentrations is analysed, and compared with TL intensity variations. It is suggested that aluminium vacancies are the trap defects responsible for these two peaks and, depending on the preparation conditions, F centres or Cr
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<sup>3+</sup>
can be the recombination centres. Two powders have been selected for dosimetry use. Their sensitivity to X ray radiation have been compared with that of Al
<sub>2</sub>
O
<sub>3</sub>
:C powder (TLD-800). The TLD-800 dosimetric peak corresponds exactly to their 200°C peak.</s0>
</fC01>
<fC02 i1="01" i2="X">
<s0>002A08F05</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE">
<s0>Dosimètre thermoluminescent</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG">
<s0>Thermoluminescent dosimeter</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA">
<s0>Dosímetro termoluminescente</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE">
<s0>Traitement thermique</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG">
<s0>Heat treatment</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA">
<s0>Tratamiento térmico</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE">
<s0>Etude comparative</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG">
<s0>Comparative study</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA">
<s0>Estudio comparativo</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE">
<s0>Composé dopé</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG">
<s0>Doped compound</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA">
<s0>Compuesto drogado</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE">
<s0>Synthèse chimique</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG">
<s0>Chemical synthesis</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA">
<s0>Síntesis química</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE">
<s0>Alumine</s0>
<s2>NK</s2>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG">
<s0>Alumina</s0>
<s2>NK</s2>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA">
<s0>Alúmina</s0>
<s2>NK</s2>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE">
<s0>Estimation paramètre</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG">
<s0>Parameter estimation</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA">
<s0>Estimación parámetro</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE">
<s0>Mesure concentration</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG">
<s0>Concentration measurement</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA">
<s0>Medición concentración</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE">
<s0>Défaut</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG">
<s0>Defect</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA">
<s0>Defecto</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE">
<s0>Processus recombinaison</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG">
<s0>Recombination process</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA">
<s0>Proceso recombinación</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE">
<s0>Analyse sensibilité</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG">
<s0>Sensitivity analysis</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA">
<s0>Análisis sensibilidad</s0>
<s5>11</s5>
</fC03>
<fN21>
<s1>263</s1>
</fN21>
</pA>
<pR>
<fA30 i1="01" i2="1" l="ENG">
<s1>International Conference on Solid State Dosimetry</s1>
<s2>12</s2>
<s3>Burgos ESP</s3>
<s4>1998-07-05</s4>
</fA30>
</pR>
</standard>
<server>
<NO>PASCAL 99-0414270 INIST</NO>
<ET>Influence of point defects on the thermoluminescence of α-Al
<sub>2</sub>
O
<sub>3</sub>
: Application to dosimetry</ET>
<AU>PAPIN (E.); GROSSEAU (P.); GUILHOT (B.); BENABDESSELAM (M.); IACCONI (P.); DELGADO (A.); GOMEZ ROS (J. M.); BOS (A. J. J.); BØTTER-JENSEN (L.); HOROWITZ (Y. S.); JULIUS (H. W.); KLEMIC (G.); KRON (T.)</AU>
<AF>SPIN-CRESA, Ecole Nationale Supérieure des Mines, 158, cours Fauriel/42023 Saint-Etienne/France (1 aut., 2 aut., 3 aut.); LPES-CRESA, Université de Nice-Sophia Antipolis, Parc Valrose/06108 Nice/France (4 aut., 5 aut.); CIEMAT/Espagne (1 aut.); Delft T. University/Pays-Bas (3 aut.); Ben Gurion University/Israël (5 aut.); TNO/Pays-Bas (6 aut.); EML (DOE)/Etats-Unis (7 aut.); Newcastle Mater Misericordiae Hospital/Australie (8 aut.)</AF>
<DT>Publication en série; Congrès; Niveau analytique</DT>
<SO>Radiation protection dosimetry; ISSN 0144-8420; Coden RPDODE; Royaume-Uni; Da. 1999; Vol. 84; No. 1-4; Pp. 91-94; Bibl. 12 ref.</SO>
<LA>Anglais</LA>
<EA>Doped α-alumina powders have been synthesised by thermal treatment of γ-alumina under a controlled atmosphere. Two TL peaks, located at 200°C and 365°C, have been detected in almost all samples. Their intensity is strongly dependent on the atmosphere and on the nature of introduced dopants. The influence of these parameters on point defects concentrations is analysed, and compared with TL intensity variations. It is suggested that aluminium vacancies are the trap defects responsible for these two peaks and, depending on the preparation conditions, F centres or Cr
<sup>3+</sup>
can be the recombination centres. Two powders have been selected for dosimetry use. Their sensitivity to X ray radiation have been compared with that of Al
<sub>2</sub>
O
<sub>3</sub>
:C powder (TLD-800). The TLD-800 dosimetric peak corresponds exactly to their 200°C peak.</EA>
<CC>002A08F05</CC>
<FD>Dosimètre thermoluminescent; Traitement thermique; Etude comparative; Composé dopé; Synthèse chimique; Alumine; Estimation paramètre; Mesure concentration; Défaut; Processus recombinaison; Analyse sensibilité</FD>
<ED>Thermoluminescent dosimeter; Heat treatment; Comparative study; Doped compound; Chemical synthesis; Alumina; Parameter estimation; Concentration measurement; Defect; Recombination process; Sensitivity analysis</ED>
<SD>Dosímetro termoluminescente; Tratamiento térmico; Estudio comparativo; Compuesto drogado; Síntesis química; Alúmina; Estimación parámetro; Medición concentración; Defecto; Proceso recombinación; Análisis sensibilidad</SD>
<LO>INIST-19318.354000085782220200</LO>
<ID>99-0414270</ID>
</server>
</inist>
</record>

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