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Major 20th century changes of water-soluble humic-like substances (HULISWS) aerosol over Europe inferred from Alpine ice cores

Identifieur interne : 000634 ( PascalFrancis/Corpus ); précédent : 000633; suivant : 000635

Major 20th century changes of water-soluble humic-like substances (HULISWS) aerosol over Europe inferred from Alpine ice cores

Auteurs : J. Guilhermet ; S. Preunkert ; D. Voisin ; C. Baduel ; M. Legrand

Source :

RBID : Pascal:14-0009278

Descripteurs français

English descriptors

Abstract

Using a newly developed method dedicated to measurements of water-soluble humic-like substances (HULISWS) in atmospheric aerosol samples, the carbon mass quantification of HULISWS in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULISWS with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULISWS concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULISWS concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULISWS sources in winter and summer. HULISWS are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULISWS signal is found to be unusual in ice samples corresponding to World War II.

Notice en format standard (ISO 2709)

Pour connaître la documentation sur le format Inist Standard.

pA  
A01 01  1    @0 2169-897X
A03   1    @0 J. geophys. res., Atmos. : (Print)
A05       @2 118
A06       @2 9
A08 01  1  ENG  @1 Major 20th century changes of water-soluble humic-like substances (HULISWS) aerosol over Europe inferred from Alpine ice cores
A11 01  1    @1 GUILHERMET (J.)
A11 02  1    @1 PREUNKERT (S.)
A11 03  1    @1 VOISIN (D.)
A11 04  1    @1 BADUEL (C.)
A11 05  1    @1 LEGRAND (M.)
A14 01      @1 UJF-Grenoble 1/CNRS, Laboratoire de Glaciologie et Géophysique de l'Environnement (LGGE) UMR 5183 @2 Grenoble 38041 @3 FRA @Z 1 aut. @Z 2 aut. @Z 3 aut. @Z 4 aut. @Z 5 aut.
A14 02      @1 National Research Centre for Environmental Toxicology (Entox) @2 Coopers Plains, Queensland 4108 @3 AUS @Z 4 aut.
A20       @1 3869-3878
A21       @1 2013
A23 01      @0 ENG
A43 01      @1 INIST @2 3144D1 @5 354000140724180320
A44       @0 0000 @1 © 2014 INIST-CNRS. All rights reserved.
A45       @0 1 p.1/2
A47 01  1    @0 14-0009278
A60       @1 P
A61       @0 A
A64 01  1    @0 Journal of geophysical research. Atmospheres : (Print)
A66 01      @0 USA
C01 01    ENG  @0 Using a newly developed method dedicated to measurements of water-soluble humic-like substances (HULISWS) in atmospheric aerosol samples, the carbon mass quantification of HULISWS in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULISWS with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULISWS concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULISWS concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULISWS sources in winter and summer. HULISWS are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULISWS signal is found to be unusual in ice samples corresponding to World War II.
C02 01  2    @0 001E02D
C03 01  X  FRE  @0 Siècle 20eme @5 01
C03 01  X  ENG  @0 Century 20th @5 01
C03 01  X  SPA  @0 Siglo 20 @5 01
C03 02  2  FRE  @0 Aérosol @5 02
C03 02  2  ENG  @0 aerosols @5 02
C03 02  2  SPA  @0 Aerosol @5 02
C03 03  2  FRE  @0 Carotte @5 03
C03 03  2  ENG  @0 drill cores @5 03
C03 03  2  SPA  @0 Testigo @5 03
C03 04  X  FRE  @0 Carbone organique total @5 04
C03 04  X  ENG  @0 Total organic carbon @5 04
C03 04  X  SPA  @0 Carbono orgánico total @5 04
C03 05  2  FRE  @0 Matière organique @5 05
C03 05  2  ENG  @0 organic materials @5 05
C03 05  2  SPA  @0 Materia orgánica @5 05
C03 06  2  FRE  @0 Variation saisonnière @5 06
C03 06  2  ENG  @0 seasonal variations @5 06
C03 06  2  SPA  @0 Variación estacional @5 06
C03 07  2  FRE  @0 Analyse tendance @5 09
C03 07  2  ENG  @0 trend-surface analysis @5 09
C03 07  2  SPA  @0 Análisis tendencia @5 09
C03 08  X  FRE  @0 Facteur biogène @5 10
C03 08  X  ENG  @0 Biogenic factor @5 10
C03 08  X  SPA  @0 Factor biógeno @5 10
C03 09  X  FRE  @0 Précurseur @5 11
C03 09  X  ENG  @0 Precursor @5 11
C03 09  X  SPA  @0 Precursor @5 11
C03 10  2  FRE  @0 Glace @5 12
C03 10  2  ENG  @0 ice @5 12
C03 10  2  SPA  @0 Hielo @5 12
C03 11  2  FRE  @0 Europe @2 564 @5 21
C03 11  2  ENG  @0 Europe @2 564 @5 21
C03 11  2  SPA  @0 Europa @2 564 @5 21
C03 12  2  FRE  @0 Alpes Françaises @2 NG @5 22
C03 12  2  ENG  @0 French Alps @2 NG @5 22
C03 12  2  SPA  @0 Alpes Franceses @2 NG @5 22
C07 01  2  FRE  @0 Alpes @2 NG
C07 01  2  ENG  @0 Alps @2 NG
C07 01  2  SPA  @0 Alpes @2 NG
N21       @1 006

Format Inist (serveur)

NO : PASCAL 14-0009278 INIST
ET : Major 20th century changes of water-soluble humic-like substances (HULISWS) aerosol over Europe inferred from Alpine ice cores
AU : GUILHERMET (J.); PREUNKERT (S.); VOISIN (D.); BADUEL (C.); LEGRAND (M.)
AF : UJF-Grenoble 1/CNRS, Laboratoire de Glaciologie et Géophysique de l'Environnement (LGGE) UMR 5183/Grenoble 38041/France (1 aut., 2 aut., 3 aut., 4 aut., 5 aut.); National Research Centre for Environmental Toxicology (Entox)/Coopers Plains, Queensland 4108/Australie (4 aut.)
DT : Publication en série; Niveau analytique
SO : Journal of geophysical research. Atmospheres : (Print); ISSN 2169-897X; Etats-Unis; Da. 2013; Vol. 118; No. 9; Pp. 3869-3878; Bibl. 1 p.1/2
LA : Anglais
EA : Using a newly developed method dedicated to measurements of water-soluble humic-like substances (HULISWS) in atmospheric aerosol samples, the carbon mass quantification of HULISWS in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULISWS with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULISWS concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULISWS concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULISWS sources in winter and summer. HULISWS are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULISWS signal is found to be unusual in ice samples corresponding to World War II.
CC : 001E02D
FD : Siècle 20eme; Aérosol; Carotte; Carbone organique total; Matière organique; Variation saisonnière; Analyse tendance; Facteur biogène; Précurseur; Glace; Europe; Alpes Françaises
FG : Alpes
ED : Century 20th; aerosols; drill cores; Total organic carbon; organic materials; seasonal variations; trend-surface analysis; Biogenic factor; Precursor; ice; Europe; French Alps
EG : Alps
SD : Siglo 20; Aerosol; Testigo; Carbono orgánico total; Materia orgánica; Variación estacional; Análisis tendencia; Factor biógeno; Precursor; Hielo; Europa; Alpes Franceses
LO : INIST-3144D1.354000140724180320
ID : 14-0009278

Links to Exploration step

Pascal:14-0009278

Le document en format XML

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<div type="abstract" xml:lang="en">Using a newly developed method dedicated to measurements of water-soluble humic-like substances (HULIS
<sub>WS</sub>
) in atmospheric aerosol samples, the carbon mass quantification of HULIS
<sub>WS</sub>
in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULIS
<sub>WS</sub>
with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULIS
<sub>WS</sub>
concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULIS
<sub>WS</sub>
concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULIS
<sub>WS</sub>
sources in winter and summer. HULIS
<sub>WS</sub>
are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULIS
<sub>WS</sub>
signal is found to be unusual in ice samples corresponding to World War II.</div>
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<sub>WS</sub>
) in atmospheric aerosol samples, the carbon mass quantification of HULIS
<sub>WS</sub>
in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULIS
<sub>WS</sub>
with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULIS
<sub>WS</sub>
concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULIS
<sub>WS</sub>
concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULIS
<sub>WS</sub>
sources in winter and summer. HULIS
<sub>WS</sub>
are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULIS
<sub>WS</sub>
signal is found to be unusual in ice samples corresponding to World War II.</s0>
</fC01>
<fC02 i1="01" i2="2">
<s0>001E02D</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE">
<s0>Siècle 20eme</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG">
<s0>Century 20th</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA">
<s0>Siglo 20</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="2" l="FRE">
<s0>Aérosol</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="2" l="ENG">
<s0>aerosols</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="2" l="SPA">
<s0>Aerosol</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="2" l="FRE">
<s0>Carotte</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="2" l="ENG">
<s0>drill cores</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="2" l="SPA">
<s0>Testigo</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE">
<s0>Carbone organique total</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG">
<s0>Total organic carbon</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA">
<s0>Carbono orgánico total</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="2" l="FRE">
<s0>Matière organique</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="2" l="ENG">
<s0>organic materials</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="2" l="SPA">
<s0>Materia orgánica</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="2" l="FRE">
<s0>Variation saisonnière</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="2" l="ENG">
<s0>seasonal variations</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="2" l="SPA">
<s0>Variación estacional</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="2" l="FRE">
<s0>Analyse tendance</s0>
<s5>09</s5>
</fC03>
<fC03 i1="07" i2="2" l="ENG">
<s0>trend-surface analysis</s0>
<s5>09</s5>
</fC03>
<fC03 i1="07" i2="2" l="SPA">
<s0>Análisis tendencia</s0>
<s5>09</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE">
<s0>Facteur biogène</s0>
<s5>10</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG">
<s0>Biogenic factor</s0>
<s5>10</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA">
<s0>Factor biógeno</s0>
<s5>10</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE">
<s0>Précurseur</s0>
<s5>11</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG">
<s0>Precursor</s0>
<s5>11</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA">
<s0>Precursor</s0>
<s5>11</s5>
</fC03>
<fC03 i1="10" i2="2" l="FRE">
<s0>Glace</s0>
<s5>12</s5>
</fC03>
<fC03 i1="10" i2="2" l="ENG">
<s0>ice</s0>
<s5>12</s5>
</fC03>
<fC03 i1="10" i2="2" l="SPA">
<s0>Hielo</s0>
<s5>12</s5>
</fC03>
<fC03 i1="11" i2="2" l="FRE">
<s0>Europe</s0>
<s2>564</s2>
<s5>21</s5>
</fC03>
<fC03 i1="11" i2="2" l="ENG">
<s0>Europe</s0>
<s2>564</s2>
<s5>21</s5>
</fC03>
<fC03 i1="11" i2="2" l="SPA">
<s0>Europa</s0>
<s2>564</s2>
<s5>21</s5>
</fC03>
<fC03 i1="12" i2="2" l="FRE">
<s0>Alpes Françaises</s0>
<s2>NG</s2>
<s5>22</s5>
</fC03>
<fC03 i1="12" i2="2" l="ENG">
<s0>French Alps</s0>
<s2>NG</s2>
<s5>22</s5>
</fC03>
<fC03 i1="12" i2="2" l="SPA">
<s0>Alpes Franceses</s0>
<s2>NG</s2>
<s5>22</s5>
</fC03>
<fC07 i1="01" i2="2" l="FRE">
<s0>Alpes</s0>
<s2>NG</s2>
</fC07>
<fC07 i1="01" i2="2" l="ENG">
<s0>Alps</s0>
<s2>NG</s2>
</fC07>
<fC07 i1="01" i2="2" l="SPA">
<s0>Alpes</s0>
<s2>NG</s2>
</fC07>
<fN21>
<s1>006</s1>
</fN21>
</pA>
</standard>
<server>
<NO>PASCAL 14-0009278 INIST</NO>
<ET>Major 20th century changes of water-soluble humic-like substances (HULIS
<sub>WS</sub>
) aerosol over Europe inferred from Alpine ice cores</ET>
<AU>GUILHERMET (J.); PREUNKERT (S.); VOISIN (D.); BADUEL (C.); LEGRAND (M.)</AU>
<AF>UJF-Grenoble 1/CNRS, Laboratoire de Glaciologie et Géophysique de l'Environnement (LGGE) UMR 5183/Grenoble 38041/France (1 aut., 2 aut., 3 aut., 4 aut., 5 aut.); National Research Centre for Environmental Toxicology (Entox)/Coopers Plains, Queensland 4108/Australie (4 aut.)</AF>
<DT>Publication en série; Niveau analytique</DT>
<SO>Journal of geophysical research. Atmospheres : (Print); ISSN 2169-897X; Etats-Unis; Da. 2013; Vol. 118; No. 9; Pp. 3869-3878; Bibl. 1 p.1/2</SO>
<LA>Anglais</LA>
<EA>Using a newly developed method dedicated to measurements of water-soluble humic-like substances (HULIS
<sub>WS</sub>
) in atmospheric aerosol samples, the carbon mass quantification of HULIS
<sub>WS</sub>
in an Alpine ice core is achieved for the first time. The method is based on the extraction of HULIS
<sub>WS</sub>
with a weak anion-exchanger resin and the subsequent quantification of the extracted carbon fraction with a total organic carbon (TOC) analyzer. Measurements were performed along a Col du Dôme (4250 m above sea level, French Alps) ice core covering the 1920-2004 time period. The HULIS
<sub>WS</sub>
concentrations exhibit a well-marked seasonal cycle with winter minima close to 7 ppbC and summer maxima ranging between 10 and 50 ppbC. Whereas the winter HULIS
<sub>WS</sub>
concentrations remained unchanged over the twentieth century, the summer concentrations increased from 20 ppbC prior to the Second World War to 35 ppbC in the 1970-1990s. These different trends reflect the different types of HULIS
<sub>WS</sub>
sources in winter and summer. HULIS
<sub>WS</sub>
are mainly primarily emitted by domestic wood burning in winter and secondary in summer being produced from biogenic precursors. For unknown reason, the HULIS
<sub>WS</sub>
signal is found to be unusual in ice samples corresponding to World War II.</EA>
<CC>001E02D</CC>
<FD>Siècle 20eme; Aérosol; Carotte; Carbone organique total; Matière organique; Variation saisonnière; Analyse tendance; Facteur biogène; Précurseur; Glace; Europe; Alpes Françaises</FD>
<FG>Alpes</FG>
<ED>Century 20th; aerosols; drill cores; Total organic carbon; organic materials; seasonal variations; trend-surface analysis; Biogenic factor; Precursor; ice; Europe; French Alps</ED>
<EG>Alps</EG>
<SD>Siglo 20; Aerosol; Testigo; Carbono orgánico total; Materia orgánica; Variación estacional; Análisis tendencia; Factor biógeno; Precursor; Hielo; Europa; Alpes Franceses</SD>
<LO>INIST-3144D1.354000140724180320</LO>
<ID>14-0009278</ID>
</server>
</inist>
</record>

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