AustralieFrV1, PascalFrancis, Checkpoint, bibRecord, 001793

Photoelectrochemical and photocatalytic activity of tungsten doped TiO2 nanotube layers in the near visible region

Identifieur interne : 001793 ( PascalFrancis/Checkpoint ); précédent : 001792; suivant : 001794

Photoelectrochemical and photocatalytic activity of tungsten doped TiO2 nanotube layers in the near visible region

Auteurs : C. Das [Allemagne] ; I. Paramasivam [Allemagne] ; N. Liu [Allemagne] ; P. Schmuki [Allemagne]

Source :

Electrochimica acta [ 0013-4686 ] ; 2011.

RBID : Pascal:12-0325026

Descripteurs français

Pascal (Inist)
- Photoélectrochimie, Photocatalyse, Tungstène VI Oxyde, Matériau dopé, Titane IV Oxyde, Nanotube, Anodisation, Titane alliage, Tungstène alliage, Alliage binaire, Rayonnement visible, Courant photoélectrique, Microscopie électronique balayage, Photolyse, Rhodamine, Cinétique, Structure surface, Morphologie, Colorant basique, Colorant xanthénique.

English descriptors

KwdEn :
- Anodizing, Basic dye, Binary alloy, Doped materials, Kinetics, Morphology, Nanotube, Photocatalysis, Photoelectric current, Photoelectrochemistry, Photolysis, Rhodamine, Scanning electron microscopy, Surface structure, Titanium IV Oxides, Titanium alloy, Tungsten VI Oxides, Tungsten alloy, Visible radiation, Xanthene dye.

Abstract

In the present work we study the effect of WO₃ doping on the photo-electrochemical behavior of self-organized TiO₂ nanotube layers. Mixed oxide nanotubes were grown by anodization of Ti-W alloys containing 0.2 and 9% W, with a thicknesses of the oxide nanotube layers adjusted to about 1.1-1.2 μm. We show that by WO₃ doping, the near visible photoresponse and photocatalytic performance can drastically be enhanced. While a content of 9 at% WO₃ in photoresponse experiments is most beneficial, in long term experiments a higher efficiency is observed for the 0.2 at% W content. This is due to a gradual leaching of W₀3 (dissolution into the electrolyte) for the higher WO₃ content. This demonstrates that under optimized WO₃ doping conditions a lasting visible light activation of TiO₂ nanotubes can be achieved.

Affiliations:

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<front><div type="abstract" xml:lang="en">In the present work we study the effect of WO<sub>3</sub>
 doping on the photo-electrochemical behavior of self-organized TiO<sub>2</sub>
 nanotube layers. Mixed oxide nanotubes were grown by anodization of Ti-W alloys containing 0.2 and 9% W, with a thicknesses of the oxide nanotube layers adjusted to about 1.1-1.2 μm. We show that by WO<sub>3</sub>
 doping, the near visible photoresponse and photocatalytic performance can drastically be enhanced. While a content of 9 at% WO<sub>3</sub>
 in photoresponse experiments is most beneficial, in long term experiments a higher efficiency is observed for the 0.2 at% W content. This is due to a gradual leaching of W<sub>0</sub>
3 (dissolution into the electrolyte) for the higher WO<sub>3</sub>
 content. This demonstrates that under optimized WO<sub>3</sub>
 doping conditions a lasting visible light activation of TiO<sub>2</sub>
 nanotubes can be achieved.</div>
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<fC01 i1="01" l="ENG"><s0>In the present work we study the effect of WO<sub>3</sub>
 doping on the photo-electrochemical behavior of self-organized TiO<sub>2</sub>
 nanotube layers. Mixed oxide nanotubes were grown by anodization of Ti-W alloys containing 0.2 and 9% W, with a thicknesses of the oxide nanotube layers adjusted to about 1.1-1.2 μm. We show that by WO<sub>3</sub>
 doping, the near visible photoresponse and photocatalytic performance can drastically be enhanced. While a content of 9 at% WO<sub>3</sub>
 in photoresponse experiments is most beneficial, in long term experiments a higher efficiency is observed for the 0.2 at% W content. This is due to a gradual leaching of W<sub>0</sub>
3 (dissolution into the electrolyte) for the higher WO<sub>3</sub>
 content. This demonstrates that under optimized WO<sub>3</sub>
 doping conditions a lasting visible light activation of TiO<sub>2</sub>
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<fC03 i1="05" i2="X" l="SPA"><s0>Titanio IV Óxido</s0>
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<s2>NA</s2>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Nanotube</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Nanotube</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Nanotubo</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Anodisation</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Anodizing</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Anodización</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Titane alliage</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Titanium alloy</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Titanio aleación</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Tungstène alliage</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Tungsten alloy</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Wolframio aleación</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Alliage binaire</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Binary alloy</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Aleación binaria</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Rayonnement visible</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Visible radiation</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Radiación visible</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Courant photoélectrique</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Photoelectric current</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Corriente fotoeléctrica</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Microscopie électronique balayage</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Scanning electron microscopy</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Microscopía electrónica barrido</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Photolyse</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Photolysis</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Fotolisis</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="X" l="FRE"><s0>Rhodamine</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="ENG"><s0>Rhodamine</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="SPA"><s0>Rodamina</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Cinétique</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Kinetics</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Cinética</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Structure surface</s0>
<s5>32</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Surface structure</s0>
<s5>32</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Estructura superficie</s0>
<s5>32</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Morphologie</s0>
<s5>33</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Morphology</s0>
<s5>33</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Morfología</s0>
<s5>33</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Colorant basique</s0>
<s5>34</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Basic dye</s0>
<s5>34</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Colorante básico</s0>
<s5>34</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Colorant xanthénique</s0>
<s5>35</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Xanthene dye</s0>
<s5>35</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Colorante xanténico</s0>
<s5>35</s5>
</fC03>
<fN21><s1>247</s1>
</fN21>
</pA>
<pR><fA30 i1="01" i2="1" l="ENG"><s1>International Society of Electrochemistry (ISE) Meeting</s1>
<s2>61</s2>
<s3>Nice FRA</s3>
<s4>2010-09-26</s4>
</fA30>
</pR>
</standard>
</inist>
<affiliations><list><country><li>Allemagne</li>
</country>
<region><li>Bavière</li>
<li>District de Moyenne-Franconie</li>
</region>
<settlement><li>Erlangen</li>
</settlement>
</list>
<tree><country name="Allemagne"><region name="Bavière"><name sortKey="Das, C" sort="Das, C" uniqKey="Das C" first="C." last="Das">C. Das</name>
</region>
<name sortKey="Liu, N" sort="Liu, N" uniqKey="Liu N" first="N." last="Liu">N. Liu</name>
<name sortKey="Paramasivam, I" sort="Paramasivam, I" uniqKey="Paramasivam I" first="I." last="Paramasivam">I. Paramasivam</name>
<name sortKey="Schmuki, P" sort="Schmuki, P" uniqKey="Schmuki P" first="P." last="Schmuki">P. Schmuki</name>
</country>
</tree>
</affiliations>
</record>

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Photoelectrochemical and photocatalytic activity of tungsten doped TiO2 nanotube layers in the near visible region

Photoelectrochemical and photocatalytic activity of tungsten doped TiO2 nanotube layers in the near visible region

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