Synthesis and Spectroscopic Characterization of Diphenylargentate, [(C6H5)2Ag](.).
Identifieur interne : 002953 ( Ncbi/Merge ); précédent : 002952; suivant : 002954Synthesis and Spectroscopic Characterization of Diphenylargentate, [(C6H5)2Ag](.).
Auteurs : M I S. Röhr [Allemagne] ; J. Petersen [Allemagne] ; C. Brunet [France] ; R. Antoine [France] ; M. Broyer [France] ; P. Dugourd [France] ; V. Bona I Kouteck [Allemagne] ; R A J. O'Hair [Australie] ; R. Mitri [Allemagne]Source :
- The journal of physical chemistry letters [ 1948-7185 ] ; 2012.
Abstract
We present the structural and optical properties of the isolated diphenylargentate anion, which has been synthesized by multistage mass spectrometry in a quadrupole ion trap. The experimental photodetachment spectrum has been obtained by action spectroscopy. Comparison with quantum chemical calculations of the electronic absorption spectrum allows for a precise characterization of the spectroscopic features, showing that in the low-energy regime, the optical properties of diphenylargentate bear a significant resemblance to those of atomic silver.
DOI: 10.1021/jz300280f
PubMed: 26288055
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O'Hair</name><affiliation wicri:level="4"><nlm:affiliation>#School of Chemistry, Bio21 Institute of Molecular Science and Biotechnology, ARC Centre of Excellence in Free Radical Chemistry and Biotechnology, The University of Melbourne, Melbourne, Victoria, 3010, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>#School of Chemistry, Bio21 Institute of Molecular Science and Biotechnology, ARC Centre of Excellence in Free Radical Chemistry and Biotechnology, The University of Melbourne, Melbourne, Victoria, 3010</wicri:regionArea><orgName type="university">Université de Melbourne</orgName><placeName><settlement type="city">Melbourne</settlement><region type="état">Victoria (État)</region></placeName></affiliation></author><author><name sortKey="Mitri, R" sort="Mitri, R" uniqKey="Mitri R" first="R" last="Mitri">R. Mitri</name><affiliation wicri:level="3"><nlm:affiliation>‡Fachbereich Physik, Freie Universität Berlin, Arnimallee 14, D-14195 Berlin, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>‡Fachbereich Physik, Freie Universität Berlin, Arnimallee 14, D-14195 Berlin</wicri:regionArea><placeName><region type="land" nuts="3">Berlin</region><settlement type="city">Berlin</settlement></placeName></affiliation></author></analytic><series><title level="j">The journal of physical chemistry letters</title><idno type="ISSN">1948-7185</idno><imprint><date when="2012" type="published">2012</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We present the structural and optical properties of the isolated diphenylargentate anion, which has been synthesized by multistage mass spectrometry in a quadrupole ion trap. The experimental photodetachment spectrum has been obtained by action spectroscopy. Comparison with quantum chemical calculations of the electronic absorption spectrum allows for a precise characterization of the spectroscopic features, showing that in the low-energy regime, the optical properties of diphenylargentate bear a significant resemblance to those of atomic silver.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">26288055</PMID><DateCreated><Year>2015</Year><Month>08</Month><Day>20</Day></DateCreated><DateCompleted><Year>2015</Year><Month>09</Month><Day>22</Day></DateCompleted><DateRevised><Year>2015</Year><Month>08</Month><Day>20</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Print">1948-7185</ISSN><JournalIssue CitedMedium="Print"><Volume>3</Volume><Issue>9</Issue><PubDate><Year>2012</Year><Month>May</Month><Day>03</Day></PubDate></JournalIssue><Title>The journal of physical chemistry letters</Title><ISOAbbreviation>J Phys Chem Lett</ISOAbbreviation></Journal><ArticleTitle>Synthesis and Spectroscopic Characterization of Diphenylargentate, [(C6H5)2Ag](.).</ArticleTitle><Pagination><MedlinePgn>1197-201</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/jz300280f</ELocationID><Abstract><AbstractText>We present the structural and optical properties of the isolated diphenylargentate anion, which has been synthesized by multistage mass spectrometry in a quadrupole ion trap. The experimental photodetachment spectrum has been obtained by action spectroscopy. Comparison with quantum chemical calculations of the electronic absorption spectrum allows for a precise characterization of the spectroscopic features, showing that in the low-energy regime, the optical properties of diphenylargentate bear a significant resemblance to those of atomic silver.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Röhr</LastName><ForeName>M I S</ForeName><Initials>MI</Initials><AffiliationInfo><Affiliation>†Institut für Chemie, Humboldt-Universität zu Berlin, Brook-Taylor-Strasse 2, D-12489 Berlin, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Petersen</LastName><ForeName>J</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>‡Fachbereich Physik, Freie Universität Berlin, Arnimallee 14, D-14195 Berlin, Germany.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Brunet</LastName><ForeName>C</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>§Université Lyon 1, CNRS, 43 Bd du 11 Novembre 1918, F-69622 Villeurbanne cedex, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Antoine</LastName><ForeName>R</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>§Université Lyon 1, CNRS, 43 Bd du 11 Novembre 1918, F-69622 Villeurbanne cedex, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Broyer</LastName><ForeName>M</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>§Université Lyon 1, CNRS, 43 Bd du 11 Novembre 1918, F-69622 Villeurbanne cedex, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Dugourd</LastName><ForeName>P</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>§Université Lyon 1, CNRS, 43 Bd du 11 Novembre 1918, F-69622 Villeurbanne cedex, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Bonačić-Koutecký</LastName><ForeName>V</ForeName><Initials>V</Initials><AffiliationInfo><Affiliation>†Institut für Chemie, Humboldt-Universität zu Berlin, Brook-Taylor-Strasse 2, D-12489 Berlin, Germany.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>⊥Interdisciplinary Center for Advanced Science and Technology, University of Split, Meštrovićevo Šetalište 45, HR-21000 Split, Croatia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>O'Hair</LastName><ForeName>R A J</ForeName><Initials>RA</Initials><AffiliationInfo><Affiliation>#School of Chemistry, Bio21 Institute of Molecular Science and Biotechnology, ARC Centre of Excellence in Free Radical Chemistry and Biotechnology, The University of Melbourne, Melbourne, Victoria, 3010, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Mitrić</LastName><ForeName>R</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>‡Fachbereich Physik, Freie Universität Berlin, Arnimallee 14, D-14195 Berlin, Germany.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2012</Year><Month>04</Month><Day>23</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>J Phys Chem Lett</MedlineTA><NlmUniqueID>101526034</NlmUniqueID><ISSNLinking>1948-7185</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">UV−vis spectroscopy</Keyword><Keyword MajorTopicYN="N">ab initio calculations</Keyword><Keyword MajorTopicYN="N">collision-induced dissociation</Keyword><Keyword MajorTopicYN="N">diphenylargentate anion</Keyword><Keyword MajorTopicYN="N">mass spectrometry</Keyword><Keyword MajorTopicYN="N">reaction intermediates</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2015</Year><Month>8</Month><Day>20</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2012</Year><Month>5</Month><Day>3</Day><Hour>0</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2012</Year><Month>5</Month><Day>3</Day><Hour>0</Hour><Minute>1</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">26288055</ArticleId><ArticleId IdType="doi">10.1021/jz300280f</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Allemagne</li><li>Australie</li><li>France</li></country><region><li>Berlin</li><li>Victoria (État)</li></region><settlement><li>Berlin</li><li>Melbourne</li></settlement><orgName><li>Université de Melbourne</li></orgName></list><tree><country name="Allemagne"><region name="Berlin"><name sortKey="Rohr, M I S" sort="Rohr, M I S" uniqKey="Rohr M" first="M I S" last="Röhr">M I S. Röhr</name></region><name sortKey="Bona I Kouteck, V" sort="Bona I Kouteck, V" uniqKey="Bona I Kouteck V" first="V" last="Bona I Kouteck">V. Bona I Kouteck</name><name sortKey="Mitri, R" sort="Mitri, R" uniqKey="Mitri R" first="R" last="Mitri">R. Mitri</name><name sortKey="Petersen, J" sort="Petersen, J" uniqKey="Petersen J" first="J" last="Petersen">J. Petersen</name></country><country name="France"><noRegion><name sortKey="Brunet, C" sort="Brunet, C" uniqKey="Brunet C" first="C" last="Brunet">C. Brunet</name></noRegion><name sortKey="Antoine, R" sort="Antoine, R" uniqKey="Antoine R" first="R" last="Antoine">R. Antoine</name><name sortKey="Broyer, M" sort="Broyer, M" uniqKey="Broyer M" first="M" last="Broyer">M. Broyer</name><name sortKey="Dugourd, P" sort="Dugourd, P" uniqKey="Dugourd P" first="P" last="Dugourd">P. Dugourd</name></country><country name="Australie"><region name="Victoria (État)"><name sortKey="O Hair, R A J" sort="O Hair, R A J" uniqKey="O Hair R" first="R A J" last="O'Hair">R A J. O'Hair</name></region></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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