Observation of a new electronic state of CO perturbing W ¹Π(v=1).
Identifieur interne : 001F12 ( Ncbi/Merge ); précédent : 001F11; suivant : 001F13Observation of a new electronic state of CO perturbing W ¹Π(v=1).
Auteurs : A N Heays [Pays-Bas] ; M. Eidelsberg [France] ; G. Stark [États-Unis] ; J L Lemaire [France] ; L. Gavilan [France] ; S R Federman [États-Unis] ; B R Lewis [Australie] ; J R Lyons [États-Unis] ; N. De Oliveira [France] ; D. Joyeux [France]Source :
- The Journal of chemical physics [ 1089-7690 ] ; 2014.
Abstract
We observe photoabsorption of the W(1) ← X(0) band in five carbon monoxide isotopologues with a vacuum-ultraviolet Fourier-transform spectrometer and a synchrotron radiation source. We deduce transition energies, integrated cross sections, and natural linewidths of the observed rotational transitions and find a perturbation affecting these. Following a deperturbation analysis of all five isotopologues, the perturbing state is assigned to the v = 0 level of a previously unobserved (1)Π state predicted by ab initio calculations to occur with the correct symmetry and equilibrium internuclear distance. We label this new state E″ (1)Π. Both of the interacting levels W(1) and E″(0) are predissociated, leading to dramatic interference effects in their corresponding linewidths.
DOI: 10.1063/1.4897326
PubMed: 25318726
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O. Box 9513, 2300 RA Leiden, The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Leiden Observatory, Leiden University, P. O. Box 9513, 2300 RA Leiden</wicri:regionArea><wicri:noRegion>2300 RA Leiden</wicri:noRegion></affiliation></author><author><name sortKey="Eidelsberg, M" sort="Eidelsberg, M" uniqKey="Eidelsberg M" first="M" last="Eidelsberg">M. Eidelsberg</name><affiliation wicri:level="1"><nlm:affiliation>Observatoire de Paris, LERMA and UMR 8112 du CNRS, 5 place Jules Janssen, 92195 Meudon, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Observatoire de Paris, LERMA and UMR 8112 du CNRS, 5 place Jules Janssen, 92195 Meudon</wicri:regionArea><wicri:noRegion>92195 Meudon</wicri:noRegion><wicri:noRegion>92195 Meudon</wicri:noRegion></affiliation></author><author><name sortKey="Stark, G" sort="Stark, G" uniqKey="Stark G" first="G" last="Stark">G. 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Terrace Rd, Tempe, Arizona 85281, USA.</nlm:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>School of Earth and Space Exploration, Arizona State University, 781 S. Terrace Rd, Tempe, Arizona 85281</wicri:regionArea><wicri:noRegion>Arizona 85281</wicri:noRegion></affiliation></author><author><name sortKey="De Oliveira, N" sort="De Oliveira, N" uniqKey="De Oliveira N" first="N" last="De Oliveira">N. De Oliveira</name><affiliation wicri:level="1"><nlm:affiliation>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex</wicri:regionArea><wicri:noRegion>91192 Gif sur Yvette Cedex</wicri:noRegion><wicri:noRegion>91192 Gif sur Yvette Cedex</wicri:noRegion></affiliation></author><author><name sortKey="Joyeux, D" sort="Joyeux, D" uniqKey="Joyeux D" first="D" last="Joyeux">D. Joyeux</name><affiliation wicri:level="1"><nlm:affiliation>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex</wicri:regionArea><wicri:noRegion>91192 Gif sur Yvette Cedex</wicri:noRegion><wicri:noRegion>91192 Gif sur Yvette Cedex</wicri:noRegion></affiliation></author></analytic><series><title level="j">The Journal of chemical physics</title><idno type="eISSN">1089-7690</idno><imprint><date when="2014" type="published">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We observe photoabsorption of the W(1) ← X(0) band in five carbon monoxide isotopologues with a vacuum-ultraviolet Fourier-transform spectrometer and a synchrotron radiation source. We deduce transition energies, integrated cross sections, and natural linewidths of the observed rotational transitions and find a perturbation affecting these. Following a deperturbation analysis of all five isotopologues, the perturbing state is assigned to the v = 0 level of a previously unobserved (1)Π state predicted by ab initio calculations to occur with the correct symmetry and equilibrium internuclear distance. We label this new state E″ (1)Π. Both of the interacting levels W(1) and E″(0) are predissociated, leading to dramatic interference effects in their corresponding linewidths.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">25318726</PMID><DateCreated><Year>2014</Year><Month>10</Month><Day>16</Day></DateCreated><DateCompleted><Year>2015</Year><Month>05</Month><Day>15</Day></DateCompleted><DateRevised><Year>2014</Year><Month>10</Month><Day>16</Day></DateRevised><Article PubModel="Print"><Journal><ISSN IssnType="Electronic">1089-7690</ISSN><JournalIssue CitedMedium="Internet"><Volume>141</Volume><Issue>14</Issue><PubDate><Year>2014</Year><Month>Oct</Month><Day>14</Day></PubDate></JournalIssue><Title>The Journal of chemical physics</Title><ISOAbbreviation>J Chem Phys</ISOAbbreviation></Journal><ArticleTitle>Observation of a new electronic state of CO perturbing W ¹Π(v=1).</ArticleTitle><Pagination><MedlinePgn>144311</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1063/1.4897326</ELocationID><Abstract><AbstractText>We observe photoabsorption of the W(1) ← X(0) band in five carbon monoxide isotopologues with a vacuum-ultraviolet Fourier-transform spectrometer and a synchrotron radiation source. We deduce transition energies, integrated cross sections, and natural linewidths of the observed rotational transitions and find a perturbation affecting these. Following a deperturbation analysis of all five isotopologues, the perturbing state is assigned to the v = 0 level of a previously unobserved (1)Π state predicted by ab initio calculations to occur with the correct symmetry and equilibrium internuclear distance. We label this new state E″ (1)Π. Both of the interacting levels W(1) and E″(0) are predissociated, leading to dramatic interference effects in their corresponding linewidths.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Heays</LastName><ForeName>A N</ForeName><Initials>AN</Initials><AffiliationInfo><Affiliation>Leiden Observatory, Leiden University, P. O. Box 9513, 2300 RA Leiden, The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Eidelsberg</LastName><ForeName>M</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>Observatoire de Paris, LERMA and UMR 8112 du CNRS, 5 place Jules Janssen, 92195 Meudon, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Stark</LastName><ForeName>G</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Department of Physics, Wellesley College, Wellesley, Massachusetts 02481, USA.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lemaire</LastName><ForeName>J L</ForeName><Initials>JL</Initials><AffiliationInfo><Affiliation>Observatoire de Paris, LERMA and UMR 8112 du CNRS, 5 place Jules Janssen, 92195 Meudon, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Gavilan</LastName><ForeName>L</ForeName><Initials>L</Initials><AffiliationInfo><Affiliation>Observatoire de Paris, LERMA and UMR 8112 du CNRS, 5 place Jules Janssen, 92195 Meudon, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Federman</LastName><ForeName>S R</ForeName><Initials>SR</Initials><AffiliationInfo><Affiliation>Department of Physics and Astronomy, University of Toledo, Toledo, Ohio 43606, USA.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lewis</LastName><ForeName>B R</ForeName><Initials>BR</Initials><AffiliationInfo><Affiliation>Research School of Physics and Engineering, The Australian National University, ACT 0200 Canberra, Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lyons</LastName><ForeName>J R</ForeName><Initials>JR</Initials><AffiliationInfo><Affiliation>School of Earth and Space Exploration, Arizona State University, 781 S. Terrace Rd, Tempe, Arizona 85281, USA.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>de Oliveira</LastName><ForeName>N</ForeName><Initials>N</Initials><AffiliationInfo><Affiliation>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Joyeux</LastName><ForeName>D</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Synchrotron SOLEIL, Orme de Merisiers, St. Aubin, BP 48, 91192 Gif sur Yvette Cedex, France.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>J Chem Phys</MedlineTA><NlmUniqueID>0375360</NlmUniqueID><ISSNLinking>0021-9606</ISSNLinking></MedlineJournalInfo></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2014</Year><Month>10</Month><Day>17</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2014</Year><Month>10</Month><Day>17</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2014</Year><Month>10</Month><Day>17</Day><Hour>6</Hour><Minute>1</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">25318726</ArticleId><ArticleId IdType="doi">10.1063/1.4897326</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Australie</li><li>France</li><li>Pays-Bas</li><li>États-Unis</li></country></list><tree><country name="Pays-Bas"><noRegion><name sortKey="Heays, A N" sort="Heays, A N" uniqKey="Heays A" first="A N" last="Heays">A N Heays</name></noRegion></country><country name="France"><noRegion><name sortKey="Eidelsberg, M" sort="Eidelsberg, M" uniqKey="Eidelsberg M" first="M" last="Eidelsberg">M. Eidelsberg</name></noRegion><name sortKey="De Oliveira, N" sort="De Oliveira, N" uniqKey="De Oliveira N" first="N" last="De Oliveira">N. De Oliveira</name><name sortKey="Gavilan, L" sort="Gavilan, L" uniqKey="Gavilan L" first="L" last="Gavilan">L. Gavilan</name><name sortKey="Joyeux, D" sort="Joyeux, D" uniqKey="Joyeux D" first="D" last="Joyeux">D. Joyeux</name><name sortKey="Lemaire, J L" sort="Lemaire, J L" uniqKey="Lemaire J" first="J L" last="Lemaire">J L Lemaire</name></country><country name="États-Unis"><noRegion><name sortKey="Stark, G" sort="Stark, G" uniqKey="Stark G" first="G" last="Stark">G. 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