Differential cross sections for intermediate-energy electron scattering from α-tetrahydrofurfuryl alcohol: excitation of electronic-states.
Identifieur interne : 001C24 ( Ncbi/Curation ); précédent : 001C23; suivant : 001C25Differential cross sections for intermediate-energy electron scattering from α-tetrahydrofurfuryl alcohol: excitation of electronic-states.
Auteurs : L. Chiari [Australie] ; H V Duque [Australie] ; D B Jones [Australie] ; P A Thorn [Australie] ; Z. Pettifer [Australie] ; G B Da Silva [Australie] ; P. Limão-Vieira [Portugal] ; D. Duflot [France] ; M-J Hubin-Franskin [Belgique] ; J. Delwiche [Belgique] ; F. Blanco [Espagne] ; G. García [Espagne] ; M C A. Lopes [Brésil] ; K. Ratnavelu [Malaisie] ; R D White [Australie] ; M J Brunger [Australie]Source :
- The Journal of chemical physics [ 1089-7690 ] ; 2014.
Descripteurs français
- KwdFr :
- MESH :
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Furans.
- Electronics, Electrons, Energy Transfer, Models, Theoretical.
Abstract
We report on measurements of differential cross sections (DCSs) for electron impact excitation of a series of Rydberg electronic-states in α-tetrahydrofurfuryl alcohol (THFA). The energy range of these experiments was 20-50 eV, while the scattered electron was detected in the 10°-90° angular range. There are currently no other experimental data or theoretical computations against which we can directly compare the present measured results. Nonetheless, we are able to compare our THFA DCSs with earlier cross section measurements for Rydberg-state electronic excitation for tetrahydrofuran, a similar cyclic ether, from Do et al. [J. Chem. Phys. 134, 144302 (2011)]. In addition, "rotationally averaged" elastic DCSs, calculated using our independent atom model with screened additivity rule correction approach are also reported. Those latter results give integral cross sections consistent with the optical theorem, and supercede those from the only previous study of Milosavljević et al. [Eur. Phys. J. D 40, 107 (2006)].
DOI: 10.1063/1.4885856
PubMed: 25028013
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Chiari</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Duque, H V" sort="Duque, H V" uniqKey="Duque H" first="H V" last="Duque">H V Duque</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Jones, D B" sort="Jones, D B" uniqKey="Jones D" first="D B" last="Jones">D B Jones</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Thorn, P A" sort="Thorn, P A" uniqKey="Thorn P" first="P A" last="Thorn">P A Thorn</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Pettifer, Z" sort="Pettifer, Z" uniqKey="Pettifer Z" first="Z" last="Pettifer">Z. 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Lopes</name><affiliation wicri:level="2"><nlm:affiliation>Departamento de Física, Universidade Federal de Juiz de Fora, Juiz de Fora, MG, Brazil.</nlm:affiliation><country xml:lang="fr">Brésil</country><wicri:regionArea>Departamento de Física, Universidade Federal de Juiz de Fora, Juiz de Fora, MG</wicri:regionArea><placeName><region type="state">Minas Gerais</region></placeName></affiliation></author><author><name sortKey="Ratnavelu, K" sort="Ratnavelu, K" uniqKey="Ratnavelu K" first="K" last="Ratnavelu">K. 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Chiari</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Duque, H V" sort="Duque, H V" uniqKey="Duque H" first="H V" last="Duque">H V Duque</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Jones, D B" sort="Jones, D B" uniqKey="Jones D" first="D B" last="Jones">D B Jones</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Thorn, P A" sort="Thorn, P A" uniqKey="Thorn P" first="P A" last="Thorn">P A Thorn</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Pettifer, Z" sort="Pettifer, Z" uniqKey="Pettifer Z" first="Z" last="Pettifer">Z. Pettifer</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Da Silva, G B" sort="Da Silva, G B" uniqKey="Da Silva G" first="G B" last="Da Silva">G B Da Silva</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author><author><name sortKey="Limao Vieira, P" sort="Limao Vieira, P" uniqKey="Limao Vieira P" first="P" last="Limão-Vieira">P. Limão-Vieira</name><affiliation wicri:level="1"><nlm:affiliation>Laboratório de Colisões Atómicas e Moleculares, CEFITEC, Departamento de Física, Faculdade de Ciências e Tecnologia, Universidade Nova de Lisboa, 2829-516 Caparica, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>Laboratório de Colisões Atómicas e Moleculares, CEFITEC, Departamento de Física, Faculdade de Ciências e Tecnologia, Universidade Nova de Lisboa, 2829-516 Caparica</wicri:regionArea><wicri:noRegion>2829-516 Caparica</wicri:noRegion></affiliation></author><author><name sortKey="Duflot, D" sort="Duflot, D" uniqKey="Duflot D" first="D" last="Duflot">D. Duflot</name><affiliation wicri:level="1"><nlm:affiliation>Laboratoire de Physique des Lasers, Atomes et Molécules, UMR CNRS 8523, Université Lille, F-59655 Villeneuve d'Ascq Cedex, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire de Physique des Lasers, Atomes et Molécules, UMR CNRS 8523, Université Lille, F-59655 Villeneuve d'Ascq Cedex</wicri:regionArea><wicri:noRegion>59655 Villeneuve d'Ascq Cedex</wicri:noRegion><wicri:noRegion>59655 Villeneuve d'Ascq Cedex</wicri:noRegion></affiliation></author><author><name sortKey="Hubin Franskin, M J" sort="Hubin Franskin, M J" uniqKey="Hubin Franskin M" first="M-J" last="Hubin-Franskin">M-J Hubin-Franskin</name><affiliation wicri:level="4"><nlm:affiliation>Départment de Chimie, Université de Liège, Institut de Chimie-Bât. B6C, B-4000 Liège 1, Belgium.</nlm:affiliation><country xml:lang="fr">Belgique</country><wicri:regionArea>Départment de Chimie, Université de Liège, Institut de Chimie-Bât. B6C, B-4000 Liège 1</wicri:regionArea><orgName type="university">Université de Liège</orgName><placeName><settlement type="city">Liège</settlement><region type="region" nuts="1">Région wallonne</region><region type="province" nuts="1">Province de Liège</region></placeName></affiliation></author><author><name sortKey="Delwiche, J" sort="Delwiche, J" uniqKey="Delwiche J" first="J" last="Delwiche">J. Delwiche</name><affiliation wicri:level="4"><nlm:affiliation>Départment de Chimie, Université de Liège, Institut de Chimie-Bât. B6C, B-4000 Liège 1, Belgium.</nlm:affiliation><country xml:lang="fr">Belgique</country><wicri:regionArea>Départment de Chimie, Université de Liège, Institut de Chimie-Bât. B6C, B-4000 Liège 1</wicri:regionArea><orgName type="university">Université de Liège</orgName><placeName><settlement type="city">Liège</settlement><region type="region" nuts="1">Région wallonne</region><region type="province" nuts="1">Province de Liège</region></placeName></affiliation></author><author><name sortKey="Blanco, F" sort="Blanco, F" uniqKey="Blanco F" first="F" last="Blanco">F. Blanco</name><affiliation wicri:level="4"><nlm:affiliation>Departamento de Física Atómica, Molecular y Nuclear, Universidad Complutense de Madrid, Madrid E-28040, Spain.</nlm:affiliation><country xml:lang="fr">Espagne</country><wicri:regionArea>Departamento de Física Atómica, Molecular y Nuclear, Universidad Complutense de Madrid, Madrid E-28040</wicri:regionArea><placeName><settlement type="city">Madrid</settlement><region nuts="2" type="region">Communauté de Madrid</region><settlement type="city">Madrid</settlement></placeName><orgName type="university">Université complutense de Madrid</orgName></affiliation></author><author><name sortKey="Garcia, G" sort="Garcia, G" uniqKey="Garcia G" first="G" last="García">G. García</name><affiliation wicri:level="1"><nlm:affiliation>Instituto de Física Fundamental, CSIC, Madrid E-28006, Spain.</nlm:affiliation><country xml:lang="fr">Espagne</country><wicri:regionArea>Instituto de Física Fundamental, CSIC, Madrid E-28006</wicri:regionArea><placeName><settlement type="city">Madrid</settlement><region nuts="2" type="region">Communauté de Madrid</region></placeName></affiliation></author><author><name sortKey="Lopes, M C A" sort="Lopes, M C A" uniqKey="Lopes M" first="M C A" last="Lopes">M C A. Lopes</name><affiliation wicri:level="2"><nlm:affiliation>Departamento de Física, Universidade Federal de Juiz de Fora, Juiz de Fora, MG, Brazil.</nlm:affiliation><country xml:lang="fr">Brésil</country><wicri:regionArea>Departamento de Física, Universidade Federal de Juiz de Fora, Juiz de Fora, MG</wicri:regionArea><placeName><region type="state">Minas Gerais</region></placeName></affiliation></author><author><name sortKey="Ratnavelu, K" sort="Ratnavelu, K" uniqKey="Ratnavelu K" first="K" last="Ratnavelu">K. Ratnavelu</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Mathematical Sciences, University of Malaya, Kuala Lumpur, Malaysia.</nlm:affiliation><country xml:lang="fr">Malaisie</country><wicri:regionArea>Institute of Mathematical Sciences, University of Malaya, Kuala Lumpur</wicri:regionArea><wicri:noRegion>Kuala Lumpur</wicri:noRegion></affiliation></author><author><name sortKey="White, R D" sort="White, R D" uniqKey="White R" first="R D" last="White">R D White</name><affiliation wicri:level="1"><nlm:affiliation>School of Engineering and Physical Sciences, James Cook University, Townsville, 4810 Queensland, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Engineering and Physical Sciences, James Cook University, Townsville, 4810 Queensland</wicri:regionArea><wicri:noRegion>4810 Queensland</wicri:noRegion></affiliation></author><author><name sortKey="Brunger, M J" sort="Brunger, M J" uniqKey="Brunger M" first="M J" last="Brunger">M J Brunger</name><affiliation wicri:level="1"><nlm:affiliation>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001, Australia.</nlm:affiliation><country xml:lang="fr">Australie</country><wicri:regionArea>School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001</wicri:regionArea><wicri:noRegion>SA 5001</wicri:noRegion></affiliation></author></analytic><series><title level="j">The Journal of chemical physics</title><idno type="eISSN">1089-7690</idno><imprint><date when="2014" type="published">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Electronics</term><term>Electrons</term><term>Energy Transfer</term><term>Furans (chemistry)</term><term>Models, Theoretical</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Furanes ()</term><term>Modèles théoriques</term><term>Transfert d'énergie</term><term>Électronique</term><term>Électrons</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Furans</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Electronics</term><term>Electrons</term><term>Energy Transfer</term><term>Models, Theoretical</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Furanes</term><term>Modèles théoriques</term><term>Transfert d'énergie</term><term>Électronique</term><term>Électrons</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">We report on measurements of differential cross sections (DCSs) for electron impact excitation of a series of Rydberg electronic-states in α-tetrahydrofurfuryl alcohol (THFA). The energy range of these experiments was 20-50 eV, while the scattered electron was detected in the 10°-90° angular range. There are currently no other experimental data or theoretical computations against which we can directly compare the present measured results. Nonetheless, we are able to compare our THFA DCSs with earlier cross section measurements for Rydberg-state electronic excitation for tetrahydrofuran, a similar cyclic ether, from Do et al. [J. Chem. Phys. 134, 144302 (2011)]. In addition, "rotationally averaged" elastic DCSs, calculated using our independent atom model with screened additivity rule correction approach are also reported. Those latter results give integral cross sections consistent with the optical theorem, and supercede those from the only previous study of Milosavljević et al. [Eur. Phys. J. D 40, 107 (2006)].</div></front></TEI></record>Pour manipuler ce document sous Unix (Dilib)
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