Single-molecule femtochemistry: molecular imaging at the space-time limit.
Identifieur interne : 001299 ( Main/Exploration ); précédent : 001298; suivant : 001300Single-molecule femtochemistry: molecular imaging at the space-time limit.
Auteurs : Hrvoje Petek [États-Unis]Source :
- ACS nano [ 1936-086X ] ; 2014.
Abstract
Through a combination of light and electron probes, it may be possible to record single-molecule dynamics with simultaneous sub-Ångstrom spatial and femtosecond temporal resolution. Single-molecule femtochemistry is becoming a realistic prospect through a melding of laser spectroscopy and electron microscopy techniques. The paper by Lee et al. in this issue of ACS Nano takes a significant step toward chemical imaging at the space-time limit of chemical processes. By imaging electroluminescence spectra of single porphyrin molecules with submolecular resolution, the authors extract the implicit femtosecond dynamics of the coupled electron orbital-molecular skeletal motion triggered by a reduction-oxidation scattering process.
DOI: 10.1021/nn4064538
PubMed: 24400854
Affiliations:
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