Perfluorinated Aromatic Spacers for Sensitizing Europium(III) Centers in Dinuclear Oligomers: Better than the Best by Chemical Design?
Identifieur interne : 003956 ( Istex/Curation ); précédent : 003955; suivant : 003957Perfluorinated Aromatic Spacers for Sensitizing Europium(III) Centers in Dinuclear Oligomers: Better than the Best by Chemical Design?
Auteurs : Jean-François Lemonnier [Suisse] ; Lucille Babel [Suisse] ; Laure Guénée [Suisse] ; Prasun Mukherjee [États-Unis] ; David H. Waldeck [États-Unis, Suisse] ; Svetlana V. Eliseeva [France] ; Stéphane Petoud [France, Suisse] ; Claude Piguet [Suisse]Source :
- Angewandte Chemie [ 0044-8249 ] ; 2012-11-05.
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Abstract
Die verschiedenen Schritte bei der Sensibilisierung durch EuIII‐Komplexe konnten mithilfe einer einfachen Methode aufgeklärt werden. Die Einführung einer zunehmenden Zahl an elektronenziehenden Fluoratomen an einer starren Phenylbrücke zwischen zwei dreizähnigen Bindestellen (siehe Bild; O rot, N dunkelblau) wirkt sich in rationaler Weise auf Quantenausbeute, Intersystem‐Crossing und Energietransferprozesse aus.
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DOI: 10.1002/ange.201205082
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Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation></author><author><name sortKey="Babel, Lucille" sort="Babel, Lucille" uniqKey="Babel L" first="Lucille" last="Babel">Lucille Babel</name><affiliation wicri:level="1"><mods:affiliation>Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation></author><author><name sortKey="Guenee, Laure" sort="Guenee, Laure" uniqKey="Guenee L" first="Laure" last="Guénée">Laure Guénée</name><affiliation wicri:level="1"><mods:affiliation>Laboratory of Crystallography, University of Geneva, 24 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>Laboratory of Crystallography, University of Geneva, 24 quai E. Ansermet</wicri:regionArea></affiliation></author><author><name sortKey="Mukherjee, Prasun" sort="Mukherjee, Prasun" uniqKey="Mukherjee P" first="Prasun" last="Mukherjee">Prasun Mukherjee</name><affiliation wicri:level="1"><mods:affiliation>Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)</mods:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh</wicri:regionArea></affiliation></author><author><name sortKey="Waldeck, David H" sort="Waldeck, David H" uniqKey="Waldeck D" first="David H." last="Waldeck">David H. Waldeck</name><affiliation wicri:level="1"><mods:affiliation>Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)</mods:affiliation><country xml:lang="fr">États-Unis</country><wicri:regionArea>Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh</wicri:regionArea></affiliation><affiliation wicri:level="1"><mods:affiliation>E-mail: dave@pitt.edu</mods:affiliation><country wicri:rule="url">États-Unis</country></affiliation><affiliation wicri:level="1"><mods:affiliation>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation></author><author><name sortKey="Eliseeva, Svetlana V" sort="Eliseeva, Svetlana V" uniqKey="Eliseeva S" first="Svetlana V." last="Eliseeva">Svetlana V. Eliseeva</name><affiliation wicri:level="1"><mods:affiliation>Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)</mods:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron</wicri:regionArea></affiliation></author><author><name sortKey="Petoud, Stephane" sort="Petoud, Stephane" uniqKey="Petoud S" first="Stéphane" last="Petoud">Stéphane Petoud</name><affiliation wicri:level="1"><mods:affiliation>Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)</mods:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron</wicri:regionArea></affiliation><affiliation wicri:level="1"><mods:affiliation>E-mail: stephane.petoud@cnrs‐orleans.fr</mods:affiliation><country wicri:rule="url">France</country></affiliation><affiliation wicri:level="1"><mods:affiliation>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation></author><author><name sortKey="Piguet, Claude" sort="Piguet, Claude" uniqKey="Piguet C" first="Claude" last="Piguet">Claude Piguet</name><affiliation wicri:level="1"><mods:affiliation>Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation><affiliation wicri:level="1"><mods:affiliation>E-mail: claude.piguet@unige.ch</mods:affiliation><country wicri:rule="url">Suisse</country></affiliation><affiliation wicri:level="1"><mods:affiliation>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet, CH‐1211 Geneva 4 (Switzerland)</mods:affiliation><country xml:lang="fr">Suisse</country><wicri:regionArea>David H. Waldeck, Department of Chemistry, University of Pittsburgh, 219 Parkman Avenue, Pittsburgh, PA 15260 (USA)Stéphane Petoud, Centre de Biophysique Moléculaire, CNRS UPR 4301, Rue Charles Sadron, F‐45071 Orléans Cedex 2 (France)Claude Piguet, Department of Inorganic Analytical Chemistry, University of Geneva, 30 quai E. Ansermet</wicri:regionArea></affiliation></author></analytic><monogr></monogr><series><title level="j" type="main">Angewandte Chemie</title><title level="j" type="alt">ANGEWANDTE CHEMIE</title><idno type="ISSN">0044-8249</idno><idno type="eISSN">1521-3757</idno><imprint><biblScope unit="vol">124</biblScope><biblScope unit="issue">45</biblScope><biblScope unit="page" from="11464">11464</biblScope><biblScope unit="page" to="11467">11467</biblScope><biblScope unit="page-count">4</biblScope><publisher>WILEY‐VCH Verlag</publisher><pubPlace>Weinheim</pubPlace><date type="published" when="2012-11-05">2012-11-05</date></imprint><idno type="ISSN">0044-8249</idno></series></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0044-8249</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Chem</term><term>Dalton trans</term><term>Global quantum</term><term>Global quantum yields</term><term>Hisc</term><term>Intersystem</term><term>Intrinsic quantum</term><term>Kisc</term><term>Ligand</term><term>Magnetic dipolar</term><term>Phys</term><term>Piguet</term><term>Rate constants</term><term>Sensitization</term><term>Sensitization mechanism</term><term>Simple method</term><term>Triplet state</term><term>Various contributions</term><term>Verlag gmbh</term><term>Weinheim angew</term></keywords><keywords scheme="Teeft" xml:lang="en"><term>Chem</term><term>Dalton trans</term><term>Global quantum</term><term>Global quantum yields</term><term>Hisc</term><term>Intersystem</term><term>Intrinsic quantum</term><term>Kisc</term><term>Ligand</term><term>Magnetic dipolar</term><term>Phys</term><term>Piguet</term><term>Rate constants</term><term>Sensitization</term><term>Sensitization mechanism</term><term>Simple method</term><term>Triplet state</term><term>Various contributions</term><term>Verlag gmbh</term><term>Weinheim angew</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract">Die verschiedenen Schritte bei der Sensibilisierung durch EuIII‐Komplexe konnten mithilfe einer einfachen Methode aufgeklärt werden. Die Einführung einer zunehmenden Zahl an elektronenziehenden Fluoratomen an einer starren Phenylbrücke zwischen zwei dreizähnigen Bindestellen (siehe Bild; O rot, N dunkelblau) wirkt sich in rationaler Weise auf Quantenausbeute, Intersystem‐Crossing und Energietransferprozesse aus.</div></front></TEI></record>Pour manipuler ce document sous Unix (Dilib)
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