Effect of partial substitution of co with Fe on the properties of LaNi3.55Mn0.4Al0.3Co0.75-xFex (x=0, 0.15, 0.55) alloys electrodes
Identifieur interne : 000373 ( PascalFrancis/Checkpoint ); précédent : 000372; suivant : 000374Effect of partial substitution of co with Fe on the properties of LaNi3.55Mn0.4Al0.3Co0.75-xFex (x=0, 0.15, 0.55) alloys electrodes
Auteurs : C. Khaldi [Tunisie] ; H. Mathlouthi [Tunisie] ; Jilani Lamloumi [Tunisie] ; A. Percheron-Guegan [France]Source :
- Journal of alloys and compounds [ 0925-8388 ] ; 2003.
Descripteurs français
- Pascal (Inist)
- Voltammétrie cyclique, Corrosion, Processus réversible, Oxydoréduction, Etude expérimentale, Diffusivité, Coefficient diffusion, Fer alliage, Matériau électrode, Cobalt alliage, Aluminium alliage, Manganèse alliage, Lanthane alliage, Nickel alliage, Alliage LaNiMnAlCoFe, Al Co Fe La Mn Ni, 8245F, 8245A.
- Wicri :
- topic : Corrosion.
English descriptors
- KwdEn :
Abstract
The effect of iron substitution on the electrochemical behaviour of LaNi3.55Mn0.4Al0.3Co0.75-xFex compounds (x=0, 0.15, 0.55) has been studied by chronopotentiometry and cyclic voltammetry techniques. The maximum capacity decreases linearly from 308 to 239 mAhg-1 when the iron content increases from 0 to 7.3 wt.% (x=0.55). This decrease can be explained by the corrosion of the alloy in the aqueous KOH electrolyte. In spite of this decrease and of the long time needed for the activation, a good stability of discharge capacity was observed in LaNi3.35Mn0.4Al0.3Co0.75-xFex compounds. The reversibility of the electrochemical redox reaction of LaNi3.55Mn0.4Al0.3Co0.75-xFex alloy electrodes has been observed in the alloys least rich in iron. The hydrogen diffusivity in LaNi3.55Mn0.4Al0.3Co0.75-xFex alloy electrodes decreases when increasing the iron content. The obtained values of the hydrogen diffusion coefficient DH, varies between 2.1×10-7 and 8.2×10-9 cm2s-1 depending on the iron content of the electrode.
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Pascal:03-0527740Le document en format XML
<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Effect of partial substitution of co with Fe on the properties of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> (x=0, 0.15, 0.55) alloys electrodes</title><author><name sortKey="Khaldi, C" sort="Khaldi, C" uniqKey="Khaldi C" first="C." last="Khaldi">C. Khaldi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName></affiliation></author><author><name sortKey="Mathlouthi, H" sort="Mathlouthi, H" uniqKey="Mathlouthi H" first="H." last="Mathlouthi">H. Mathlouthi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName></affiliation></author><author><name sortKey="Lamloumi, J" sort="Lamloumi, J" uniqKey="Lamloumi J" first="J." last="Lamloumi">Jilani Lamloumi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName><placeName><settlement type="city">Tunis</settlement><region type="region" nuts="2">Gouvernorat de Tunis</region></placeName><orgName type="university" n="3">Université de Tunis</orgName></affiliation></author><author><name sortKey="Percheron Guegan, A" sort="Percheron Guegan, A" uniqKey="Percheron Guegan A" first="A." last="Percheron-Guegan">A. 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G.L.T, CNRS, 2-8 Rue Henri Dunant</s1><s2>94320, Thiais</s2><s3>FRA</s3><sZ>4 aut.</sZ></inist:fA14><country>France</country><wicri:noRegion>Thiais</wicri:noRegion><wicri:noRegion>2-8 Rue Henri Dunant</wicri:noRegion><wicri:noRegion>94320, Thiais</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">INIST</idno><idno type="inist">03-0527740</idno><date when="2003">2003</date><idno type="stanalyst">PASCAL 03-0527740 INIST</idno><idno type="RBID">Pascal:03-0527740</idno><idno type="wicri:Area/PascalFrancis/Corpus">000364</idno><idno type="wicri:Area/PascalFrancis/Curation">000077</idno><idno type="wicri:Area/PascalFrancis/Checkpoint">000373</idno><idno type="wicri:explorRef" wicri:stream="PascalFrancis" wicri:step="Checkpoint">000373</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Effect of partial substitution of co with Fe on the properties of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> (x=0, 0.15, 0.55) alloys electrodes</title><author><name sortKey="Khaldi, C" sort="Khaldi, C" uniqKey="Khaldi C" first="C." last="Khaldi">C. Khaldi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName></affiliation></author><author><name sortKey="Mathlouthi, H" sort="Mathlouthi, H" uniqKey="Mathlouthi H" first="H." last="Mathlouthi">H. Mathlouthi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName></affiliation></author><author><name sortKey="Lamloumi, J" sort="Lamloumi, J" uniqKey="Lamloumi J" first="J." last="Lamloumi">Jilani Lamloumi</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Tunisie</country><placeName><settlement type="city">Tunis</settlement><region nuts="2">Gouvernorat de Tunis</region></placeName><placeName><settlement type="city">Tunis</settlement><region type="region" nuts="2">Gouvernorat de Tunis</region></placeName><orgName type="university" n="3">Université de Tunis</orgName></affiliation></author><author><name sortKey="Percheron Guegan, A" sort="Percheron Guegan, A" uniqKey="Percheron Guegan A" first="A." last="Percheron-Guegan">A. Percheron-Guegan</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>L.C.M.T.R. G.L.T, CNRS, 2-8 Rue Henri Dunant</s1><s2>94320, Thiais</s2><s3>FRA</s3><sZ>4 aut.</sZ></inist:fA14><country>France</country><wicri:noRegion>Thiais</wicri:noRegion><wicri:noRegion>2-8 Rue Henri Dunant</wicri:noRegion><wicri:noRegion>94320, Thiais</wicri:noRegion></affiliation></author></analytic><series><title level="j" type="main">Journal of alloys and compounds</title><title level="j" type="abbreviated">J. alloys compd.</title><idno type="ISSN">0925-8388</idno><imprint><date when="2003">2003</date></imprint></series></biblStruct></sourceDesc><seriesStmt><title level="j" type="main">Journal of alloys and compounds</title><title level="j" type="abbreviated">J. alloys compd.</title><idno type="ISSN">0925-8388</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Aluminium alloy</term><term>Cobalt alloy</term><term>Corrosion</term><term>Cyclic voltammetry</term><term>Diffusion coefficient</term><term>Diffusivity</term><term>Electrode material</term><term>Experimental study</term><term>Iron alloy</term><term>Lanthanum alloy</term><term>Manganèse alloy</term><term>Nickel alloy</term><term>Oxidation reduction</term><term>Reversible processes</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Voltammétrie cyclique</term><term>Corrosion</term><term>Processus réversible</term><term>Oxydoréduction</term><term>Etude expérimentale</term><term>Diffusivité</term><term>Coefficient diffusion</term><term>Fer alliage</term><term>Matériau électrode</term><term>Cobalt alliage</term><term>Aluminium alliage</term><term>Manganèse alliage</term><term>Lanthane alliage</term><term>Nickel alliage</term><term>Alliage LaNiMnAlCoFe</term><term>Al Co Fe La Mn Ni</term><term>8245F</term><term>8245A</term></keywords><keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Corrosion</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The effect of iron substitution on the electrochemical behaviour of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> compounds (x=0, 0.15, 0.55) has been studied by chronopotentiometry and cyclic voltammetry techniques. The maximum capacity decreases linearly from 308 to 239 mAhg<sup>-1</sup> when the iron content increases from 0 to 7.3 wt.% (x=0.55). This decrease can be explained by the corrosion of the alloy in the aqueous KOH electrolyte. In spite of this decrease and of the long time needed for the activation, a good stability of discharge capacity was observed in LaNi<sub>3.35</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> compounds. The reversibility of the electrochemical redox reaction of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> alloy electrodes has been observed in the alloys least rich in iron. The hydrogen diffusivity in LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> alloy electrodes decreases when increasing the iron content. The obtained values of the hydrogen diffusion coefficient D<sub>H</sub>, varies between 2.1×10<sup>-7</sup> and 8.2×10<sup>-9</sup> cm<sup>2</sup>s<sup>-1</sup> depending on the iron content of the electrode.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0925-8388</s0></fA01><fA03 i2="1"><s0>J. alloys compd.</s0></fA03><fA05><s2>360</s2></fA05><fA08 i1="01" i2="1" l="ENG"><s1>Effect of partial substitution of co with Fe on the properties of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> (x=0, 0.15, 0.55) alloys electrodes</s1></fA08><fA11 i1="01" i2="1"><s1>KHALDI (C.)</s1></fA11><fA11 i1="02" i2="1"><s1>MATHLOUTHI (H.)</s1></fA11><fA11 i1="03" i2="1"><s1>LAMLOUMI (J.)</s1></fA11><fA11 i1="04" i2="1"><s1>PERCHERON-GUEGAN (A.)</s1></fA11><fA14 i1="01"><s1>L.M.M.P, ESSTT, 5 Avenue Taha Hussein</s1><s2>1008 Tunis</s2><s3>TUN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ></fA14><fA14 i1="02"><s1>L.C.M.T.R. G.L.T, CNRS, 2-8 Rue Henri Dunant</s1><s2>94320, Thiais</s2><s3>FRA</s3><sZ>4 aut.</sZ></fA14><fA20><s1>266-271</s1></fA20><fA21><s1>2003</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>1151</s2><s5>354000113392730450</s5></fA43><fA44><s0>0000</s0><s1>© 2003 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>12 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>03-0527740</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Journal of alloys and compounds</s0></fA64><fA66 i1="01"><s0>CHE</s0></fA66><fC01 i1="01" l="ENG"><s0>The effect of iron substitution on the electrochemical behaviour of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> compounds (x=0, 0.15, 0.55) has been studied by chronopotentiometry and cyclic voltammetry techniques. The maximum capacity decreases linearly from 308 to 239 mAhg<sup>-1</sup> when the iron content increases from 0 to 7.3 wt.% (x=0.55). This decrease can be explained by the corrosion of the alloy in the aqueous KOH electrolyte. In spite of this decrease and of the long time needed for the activation, a good stability of discharge capacity was observed in LaNi<sub>3.35</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> compounds. The reversibility of the electrochemical redox reaction of LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> alloy electrodes has been observed in the alloys least rich in iron. The hydrogen diffusivity in LaNi<sub>3.55</sub>Mn<sub>0.4</sub>Al<sub>0.3</sub>Co<sub>0.75-x</sub>Fe<sub>x</sub> alloy electrodes decreases when increasing the iron content. The obtained values of the hydrogen diffusion coefficient D<sub>H</sub>, varies between 2.1×10<sup>-7</sup> and 8.2×10<sup>-9</sup> cm<sup>2</sup>s<sup>-1</sup> depending on the iron content of the electrode.</s0></fC01><fC02 i1="01" i2="X"><s0>001C01H02</s0></fC02><fC02 i1="02" i2="X"><s0>001C01H05</s0></fC02><fC03 i1="01" i2="X" l="FRE"><s0>Voltammétrie cyclique</s0><s5>02</s5></fC03><fC03 i1="01" i2="X" l="ENG"><s0>Cyclic voltammetry</s0><s5>02</s5></fC03><fC03 i1="01" i2="X" l="SPA"><s0>Voltametría cíclica</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="FRE"><s0>Corrosion</s0><s5>03</s5></fC03><fC03 i1="02" i2="X" l="ENG"><s0>Corrosion</s0><s5>03</s5></fC03><fC03 i1="02" i2="X" l="SPA"><s0>Corrosión</s0><s5>03</s5></fC03><fC03 i1="03" i2="3" l="FRE"><s0>Processus réversible</s0><s5>04</s5></fC03><fC03 i1="03" i2="3" l="ENG"><s0>Reversible processes</s0><s5>04</s5></fC03><fC03 i1="04" i2="X" l="FRE"><s0>Oxydoréduction</s0><s5>05</s5></fC03><fC03 i1="04" i2="X" l="ENG"><s0>Oxidation reduction</s0><s5>05</s5></fC03><fC03 i1="04" i2="X" l="SPA"><s0>Oxidación reducción</s0><s5>05</s5></fC03><fC03 i1="05" i2="X" l="FRE"><s0>Etude expérimentale</s0><s5>06</s5></fC03><fC03 i1="05" i2="X" l="ENG"><s0>Experimental study</s0><s5>06</s5></fC03><fC03 i1="05" i2="X" l="SPA"><s0>Estudio experimental</s0><s5>06</s5></fC03><fC03 i1="06" i2="X" l="FRE"><s0>Diffusivité</s0><s5>07</s5></fC03><fC03 i1="06" i2="X" l="ENG"><s0>Diffusivity</s0><s5>07</s5></fC03><fC03 i1="06" i2="X" l="SPA"><s0>Difusibilidad</s0><s5>07</s5></fC03><fC03 i1="07" i2="X" l="FRE"><s0>Coefficient diffusion</s0><s5>08</s5></fC03><fC03 i1="07" i2="X" l="ENG"><s0>Diffusion coefficient</s0><s5>08</s5></fC03><fC03 i1="07" i2="X" l="SPA"><s0>Coeficiente difusión</s0><s5>08</s5></fC03><fC03 i1="08" i2="X" l="FRE"><s0>Fer alliage</s0><s5>15</s5></fC03><fC03 i1="08" i2="X" l="ENG"><s0>Iron alloy</s0><s5>15</s5></fC03><fC03 i1="08" i2="X" l="SPA"><s0>Hierro aleación</s0><s5>15</s5></fC03><fC03 i1="09" i2="X" l="FRE"><s0>Matériau électrode</s0><s5>16</s5></fC03><fC03 i1="09" i2="X" l="ENG"><s0>Electrode material</s0><s5>16</s5></fC03><fC03 i1="09" i2="X" l="SPA"><s0>Material electrodo</s0><s5>16</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Cobalt alliage</s0><s5>17</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Cobalt alloy</s0><s5>17</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Cobalto aleación</s0><s5>17</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Aluminium alliage</s0><s5>18</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Aluminium alloy</s0><s5>18</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Aluminio aleación</s0><s5>18</s5></fC03><fC03 i1="12" i2="X" l="FRE"><s0>Manganèse alliage</s0><s5>19</s5></fC03><fC03 i1="12" i2="X" l="ENG"><s0>Manganèse alloy</s0><s5>19</s5></fC03><fC03 i1="12" i2="X" l="SPA"><s0>Manganeso aleación</s0><s5>19</s5></fC03><fC03 i1="13" i2="X" l="FRE"><s0>Lanthane alliage</s0><s5>20</s5></fC03><fC03 i1="13" i2="X" l="ENG"><s0>Lanthanum alloy</s0><s5>20</s5></fC03><fC03 i1="13" i2="X" l="SPA"><s0>Lantano aleación</s0><s5>20</s5></fC03><fC03 i1="14" i2="X" l="FRE"><s0>Nickel alliage</s0><s5>21</s5></fC03><fC03 i1="14" i2="X" l="ENG"><s0>Nickel alloy</s0><s5>21</s5></fC03><fC03 i1="14" i2="X" l="SPA"><s0>Níquel aleación</s0><s5>21</s5></fC03><fC03 i1="15" i2="X" l="FRE"><s0>Alliage LaNiMnAlCoFe</s0><s4>INC</s4><s5>52</s5></fC03><fC03 i1="16" i2="X" l="FRE"><s0>Al Co Fe La Mn Ni</s0><s4>INC</s4><s5>53</s5></fC03><fC03 i1="17" i2="X" l="FRE"><s0>8245F</s0><s2>PAC</s2><s4>INC</s4><s5>56</s5></fC03><fC03 i1="18" i2="X" l="FRE"><s0>8245A</s0><s2>PAC</s2><s4>INC</s4><s5>57</s5></fC03><fC07 i1="01" i2="X" l="FRE"><s0>Composé minéral</s0><s5>48</s5></fC07><fC07 i1="01" i2="X" l="ENG"><s0>Inorganic compound</s0><s5>48</s5></fC07><fC07 i1="01" i2="X" l="SPA"><s0>Compuesto inorgánico</s0><s5>48</s5></fC07><fC07 i1="02" i2="X" l="FRE"><s0>Métal transition alliage</s0><s5>49</s5></fC07><fC07 i1="02" i2="X" l="ENG"><s0>Transition metal alloy</s0><s5>49</s5></fC07><fC07 i1="02" i2="X" l="SPA"><s0>Metal transición aleación</s0><s5>49</s5></fC07><fC07 i1="03" i2="X" l="FRE"><s0>Lanthanide alliage</s0><s5>50</s5></fC07><fC07 i1="03" i2="X" l="ENG"><s0>Rare earth metal alloy</s0><s5>50</s5></fC07><fC07 i1="03" i2="X" l="SPA"><s0>Lantánido aleación</s0><s5>50</s5></fC07><fN21><s1>349</s1></fN21><fN82><s1>PSI</s1></fN82></pA></standard></inist><affiliations><list><country><li>France</li><li>Tunisie</li></country><region><li>Gouvernorat de Tunis</li></region><settlement><li>Tunis</li></settlement><orgName><li>Université de Tunis</li></orgName></list><tree><country name="Tunisie"><region name="Gouvernorat de Tunis"><name sortKey="Khaldi, C" sort="Khaldi, C" uniqKey="Khaldi C" first="C." last="Khaldi">C. Khaldi</name></region><name sortKey="Lamloumi, J" sort="Lamloumi, J" uniqKey="Lamloumi J" first="J." last="Lamloumi">Jilani Lamloumi</name><name sortKey="Mathlouthi, H" sort="Mathlouthi, H" uniqKey="Mathlouthi H" first="H." last="Mathlouthi">H. Mathlouthi</name></country><country name="France"><noRegion><name sortKey="Percheron Guegan, A" sort="Percheron Guegan, A" uniqKey="Percheron Guegan A" first="A." last="Percheron-Guegan">A. Percheron-Guegan</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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